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The electronic excitation occurring on adsorbates at ultrafast time scales from optical lasers that initiate surface chemical reactions is still an open question. Here, we report the ultrafast temporal evolution of X-ray absorption…

High peak power ultrafast lasers are widely used in nonlinear spectroscopy but often limit its spectral resolution because of the broad frequency bandwidth of ultrashort laser pulses. Improving the resolution by achieving spectrally narrow…

Optics · Physics 2009-11-13 Stanislav O. Konorov , Xiaoji G. Xu , John W. Hepburn , Valery Milner

Controlling nonequilibrium responses in optically driven quantum materials is essential for advancing applications in energy conversion, ultrafast electronics, and quantum computation. Nonlinear optical spectroscopy serves as a powerful…

BAL QSOs are notoriously faint X-ray sources, presumably due to extreme intrinsic absorption. However, several objects have begun to appear through the obscuration with recent X-ray observations by Chandra and ASCA. Where enough counts are…

Astrophysics · Physics 2007-05-23 S. C. Gallagher , W. N. Brandt , G. Chartas , G. P. Garmire

Measuring the phase of light is fundamental to optical imaging, sensing, and signal processing applications. Conventional optical phase measurements rely on multipath configurations, bulky interferometric setups, and computationally…

We have tested the new experimental techniques in the M\"ossbauer spectroscopy with Synchrotron M\"ossbauer Source by using the polarization analysis of the reflected radiation. In particular we have shown that the dichroic components in…

Mesoscale and Nanoscale Physics · Physics 2018-03-28 Marina Andreeva , Roman Baulin , Aleksandr Chumakov , Tatiyana Kiseleva , Rudolf Rüffer

Quantum networks using photonic channels require control of the interactions between the photons, carrying the information, and the elements comprising the nodes. In this work we theoretically analyse the spectral properties of an optical…

Quantum Physics · Physics 2021-12-23 Tom Schmit , Luigi Giannelli , Anders S. Sørensen , Giovanna Morigi

X-ray photon correlation spectroscopy (XPCS) allows for the resolution of dynamic processes within a material across a wide range of length and time scales. X-ray speckle visibility spectroscopy (XSVS) is a related method that uses a single…

Numerical Analysis · Mathematics 2023-01-09 Shaswat Mohanty , Christopher B. Cooper , Hui Wang , Mengning Liang , Wei Cai

We proposed remote spectroscopy approach consisted in luminescence light utilization. During interaction with different targets ultrashort UV laser pulse generates broadband spectrum light, which can be applied for remote spectroscopy…

Two-photon excitation spectroscopy is a nonlinear technique that has gained rapidly in interest and significance for studying the complex energy-level structure and transition probabilities of materials. While the conventional spectroscopy…

Quantum Physics · Physics 2022-11-23 Yuanyuan Chen , Roberto de J. León-Montiel , Lixiang Chen

We develop a means for speckle-based phase imaging of the projected thickness of a single-material object, under the assumption of illumination by spatially random time-independent x-ray speckles. These speckles are generated by passing x…

Femtosecond transient soft X-ray Absorption Spectroscopy (XAS) is a very promising technique that can be employed at X-ray Free Electron Lasers (FELs) to investigate out-of-equilibrium dynamics for material and energy research. Here we…

Existing computational spectral imaging systems typically rely on coded aperture and beam splitters that block a substantial fraction of incident light, degrading reconstruction quality under light-starved conditions. To address this…

Computer Vision and Pattern Recognition · Computer Science 2026-03-17 Jiuyun Zhang , Zhan Shi , Linsen Chen , Xun Cao

Optical microscopy is without a doubt an essential component of life science research, but many objects of interest in biology are transparent. Chemical or immunological dyes, which can often be toxic, fluorescent transgenes, which require…

Optics · Physics 2012-09-11 Quintin Tyrell Davis

New experimental techniques based on non-linear ultrafast spectroscopies have been developed over the last few years, and have been demonstrated to provide powerful probes of quantum dynamics in different types of molecular aggregates,…

A novel method and experimental configuration are proposed that allow the collection of high-quality X-ray absorption spectroscopy (XAS) data in transmission mode on a standard laboratory diffractometer. This configuration makes use of…

Instrumentation and Detectors · Physics 2025-09-23 Milen Gateshki , Charalampos Zarkadas , Detlef Beckers

Purpose: Spectral imaging is a method in medical x-ray imaging to extract information about the object constituents by the material-specific energy dependence of x-ray attenuation. The authors have investigated a photon-counting spectral…

Medical Physics · Physics 2021-01-21 Erik Fredenberg , Magnus Hemmendorff , Bjorn Cederstrom , Magnus Aslund , Mats Danielsson

We present a novel extraction algorithm for spectral phase interferometry for direct field reconstruction (SPIDER) for the so-called X-SPIDER configuration. Our approach largely extends the measurable time windows of pulses without…

Quantum correlation, such as entanglement and squeezing have shown to improve phase estimation in interferometric setups on one side, and non-interferometric imaging scheme of amplitude object on the other. In the last case, quantum…

We describe an experiment to measure the emitted real-time electric field from an ultrafast third-order nonlinear optical interaction in molecules, using a phase-tracked spectral interferometry scheme. By combining a software lock-in…

Optics · Physics 2025-03-11 Siddhant Pandey , Francis Walz , Niranjan Shivaram
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