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Motivated by the possibility of an intermediate U(1) quantum spin liquid phase in out-of-plane magnetic fields and enhanced magnetic fluctuations in exfoliated {\alpha}-RuCl3 flakes, we study magneto-Raman spectra of exfoliated multilayer…

In recent years, a lot of effort has been devoted to the quest for experimental realizations of Kitaev interactions in spin systems. Recently, many materials have been synthesized which seem to realize extended Kitaev models, where Kitaev…

Strongly Correlated Electrons · Physics 2019-06-05 Maria Laura Baez

TlCuCl$_3$ has a singlet ground state with the excitation gap $\Delta =0.65$ meV. The magnetic excitations in TlCuCl$_3$ have been investigated by means of neutron inelastic scattering experiments. The constant-$\it{\pmb Q}$ energy scan…

Strongly Correlated Electrons · Physics 2007-05-23 A. Oosawa , T. Kato , H. Tanaka , K. Kakurai , M. Mueller , H. -J. Mikeska

We investigate the effects of hydrostatic pressure on $\alpha$-RuCl$_3$, a prototypical material for the Kitaev spin model on a honeycomb lattice with a possible spin-liquid ground state. Using ultrasound measurements at pressures up to…

Strongly Correlated Electrons · Physics 2025-03-07 A. Hauspurg , Susmita Singh , T. Yanagisawa , V. Tsurkan , J. Wosnitza , Wolfram Brenig , Natalia B. Perkins , S. Zherlitsyn

In this study, we reanalyze the magnetic interactions in the Kitaev spin liquid candidate materials Na$_2$IrO$_3$, $\alpha$-RuCl$_3$, and $\alpha$-Li$_2$IrO$_3$ using nonperturbative exact diagonalization methods. These methods are more…

Strongly Correlated Electrons · Physics 2016-07-06 Stephen M. Winter , Ying Li , Harald O. Jeschke , Roser Valenti

RuCl$_3$ was likely the first ever deliberately synthesized ruthenium compound, following the discovery of the $_{44}$Ru element in 1844. For a long time it was known as an oxidation catalyst, with its physical properties being discrepant…

Strongly Correlated Electrons · Physics 2025-09-04 Marius Möller , P. A. Maksimov , Shengtao Jiang , Steven R. White , Roser Valenti , A. L. Chernyshev

Magnetic dilution of a well-established Kitaev candidate system is realized in the substitutional Ru$_{1-x}$Rh$_x$Cl$_3$ series ($x = 0.02-0.6$). Optimized syntheses protocols yield uniformly-doped single crystals and polycrystalline…

Strongly Correlated Electrons · Physics 2023-01-10 G. Bastien , E. Vinokurova , M. Lange , K. K. Bestha , L. T. Corredor , G. Kreutzer , A. Lubk , Th. Doert , B. Buchner , A. Isaeva , A. U. B. Wolter

In $\alpha$-RuCl$_3$, an external magnetic field applied within the honeycomb plane can induce a transition from a magnetically ordered state to a disordered state that is potentially related to the Kitaev quantum spin liquid. In zero…

We provide a theory of triplon dynamics in the valence bond solid ground state of the coupled spin-ladders modelled for BiCu$_2$PO$_6$. Utilizing the recent high quality neutron scattering data [Nature Physics (2015), DOI:…

Strongly Correlated Electrons · Physics 2016-06-20 Kyusung Hwang , Yong Baek Kim

We examine the role of spin-orbit coupling in the electronic structure of $\alpha$-RuCl3, in which Ru ions in 4d5 configuration form a honeycomb lattice. The measured optical spectra exhibit a clear optical gap and excitations within the…

Strongly Correlated Electrons · Physics 2014-08-06 K. W. Plumb , J. P. Clancy , L. Sandilands , V. Vijay Shankar , Y. F. Hu , K. S. Burch , Hae-Young Kee , Young-June Kim

We explore the potential experimental realization of the mixed-spin Kitaev model in materials such as Zr$_{0.5}$Ru$_{0.5}$Cl$_3$, where spin-1/2 and spin-3/2 ions occupy distinct sublattices of a honeycomb lattice. By developing a…

Strongly Correlated Electrons · Physics 2025-05-09 Willian Natori , Yang Yang , Hui-Ke Jin , Johannes Knolle , Natalia B. Perkins

The recent neutron-scattering data for spin-wave dispersion in $\rm Ho Mn O_3$ are well described by an anisotropic Hubbard model on a triangular lattice with a planar (XY) spin anisotropy. Best fit indicates that magnetic excitations in…

Strongly Correlated Electrons · Physics 2015-06-25 Saptarshi Ghosh , Avinash Singh

The ruthenium halide $\alpha$-RuCl$_{3}$ is a promising candidate for a Kitaev spin liquid. However, the microscopic model describing $\alpha$-RuCl$_{3}$ is still debated partly because of a lack of analogue materials for…

We report inelastic neutron scattering measurements on Na2IrO3, a candidate for the Kitaev spin model on the honeycomb lattice. We observe spin-wave excitations below 5 meV with a dispersion that can be accounted for by including…

$\alpha$-RuCl$_3$ is a candidate Kitaev material that exhibits zigzag antiferromagnetic ordering below 7 K. One contentious issue regarding this material is its bulk structure in the low-temperature phase. Recently, it has become generally…

Materials Science · Physics 2026-01-27 Seung-Ju Hong , Tae Yun Kim , Cheol-Hwan Park

Single-crystal neutron inelastic scattering was performed in order to investigate the magnetic excitations in the spin gap system TlCuCl$_3$. The constant-${\bf Q}$ energy scan profiles were collected in the $a^*-c^*$ plane. Three…

Condensed Matter · Physics 2007-05-23 A. Oosawa , T. Kato , H. Tanaka , H. Uekusa , Y. Ohashi , K. Nakajima , M. Nishi , K. Kakurai

Novel ground states might be realized in honeycomb lattices with strong spin-orbit coupling. Here we study the electronic structure of ${\alpha}$-RuCl$_3$, in which the Ru ions are in a d5 configuration and form a honeycomb lattice, by…

Strongly Correlated Electrons · Physics 2016-09-21 A. Koitzsch , C. Habenicht , E. Mueller , M. Knupfer , B. Buechner , H. Kandpal , J. van den Brink , D. Nowak , A. Isaeva , Th. Doert

Motivated by recent experiments on $\alpha$-RuCl$_3$, we investigate a possible quantum spin liquid ground state of the honeycomb-lattice spin model with bond-dependent interactions. We consider the $K-\Gamma$ model, where $K$ and $\Gamma$…

Strongly Correlated Electrons · Physics 2018-02-15 Matthias Gohlke , Gideon Wachtel , Youhei Yamaji , Frank Pollmann , Yong Baek Kim

What is the correct low-energy spin Hamiltonian description of $\alpha$-RuCl$_3$? The material is a promising Kitaev spin liquid candidate, but is also known to order magnetically, the description of which necessitates additional…

Strongly Correlated Electrons · Physics 2020-01-13 Pontus Laurell , Satoshi Okamoto

Dimethylammonium copper (II) chloride (also known as DMACuCl3 or MCCL) is a low dimensional S=1/2 quantum spin system proposed to be an alternating ferro-antiferromagnetic chain with similar magnitude ferromagnetic (FM) and…

Strongly Correlated Electrons · Physics 2009-11-11 M. B. Stone , W. Tian , G. E. Granroth , M. D. Lumsdena , J-H. Chung , D. G. Mandrusa , S. E. Nagler