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We provide analytical and numerical insights into the phase diagram and other properties of the extended Kitaev-Heisenberg model on the honeycomb lattice in the {\it easy-plane} limit, in which interactions are only between spin components…

Strongly Correlated Electrons · Physics 2023-01-20 P. A. Maksimov , A. L. Chernyshev

We present a thorough experimental study of the three-dimensional hyperhoneycomb Kitaev magnet $\beta$-Li$_2$IrO$_3$, using a combination of inelastic neutron scattering (INS), time-domain THz spectroscopy, and heat capacity measurements.…

The magnetism of Kitaev materials has been widely studied, but their charge properties and the coupling to other degrees of freedom are less known. Here we investigate the charge states of $\alpha$-RuCl$_3$, a promising Kitaev quantum spin…

Strongly Correlated Electrons · Physics 2024-08-27 Xiaohu Zheng , Zhengxin Liu , Cuiwei Zhang , Huaxue Zhou , Chongli Yang , Youguo Shi , Katsumi Tanigaki , Rui-Rui Du

Cobaltates with 3$d$ based layered honeycomb structure were recently proposed as Kitaev magnets and putative candidates to host the long-sought Kitaev spin liquid. Here we present inelastic neutron scattering results down to 50 mK for…

Strongly Correlated Electrons · Physics 2023-01-18 Alaric L. Sanders , Richard A. Mole , Jiatu Liu , Alex J. Brown , Dehong Yu , Chris D. Ling , Stephan Rachel

Inelastic and elastic neutron scattering is used to study spin correlations in the quasi-one dimensional quantum antiferromagnet IPA-CuCl3 in strong applied magnetic fields. A condensation of magnons and commensurate transverse long-range…

Strongly Correlated Electrons · Physics 2007-05-23 A. Zheludev , V. O. Garlea , T. Masuda , H. Manaka , L. -P. Regnault , E. Ressouche , B. Grenier , J. -H. Chung , Y. Qiu , K. Habicht , K. Kiefer , M. Boehm

We report magnetization and neutron diffraction studies on crystal and magnetic structures of Ir- and Rh-substituted honeycomb lattice $\alpha$-RuCl$_3$. The iridium or rhodium atoms are distributed at the Ru site with little structural…

Materials Science · Physics 2023-10-05 Zachary Morgan , Iris Ye , Colin L. Sarkis , Xiaoping Wang , Stephen Nagler , Jiaqiang Yan

A quantum spin-liquid might be realized in $\alpha$-RuCl$_{3}$, a honeycomb-lattice magnetic material with substantial spin-orbit coupling. Moreover, $\alpha$-RuCl$_{3}$ is a Mott insulator, which implies the possibility that novel exotic…

Mott insulators with strong spin-orbit coupling display a strongly anisotropic response to applied magnetic fields. This applies in particular to Kitaev materials, with $\alpha$-RuCl$_3$ and Na$_2$IrO$_3$ representing two important…

Strongly Correlated Electrons · Physics 2020-10-06 Eric C. Andrade , Lukas Janssen , Matthias Vojta

The layered compound $\alpha$-RuCl$_3$ is composed of a honeycomb lattice of magnetic Ru$^{3+}$ ions with the $4d^5$ electronic state. We have investigated the magnetic properties of $\alpha$-RuCl$_3$ via magnetization and specific heat…

Strongly Correlated Electrons · Physics 2015-06-24 Yumi Kubota , Hidekazu Tanaka , Toshio Ono , Yasuo Narumi , Koichi Kindo

Recently considerable excitement has arisen due to the experimental observation of a field-induced spin liquid phase in the compound $\alpha$-RuCl$_3$. However, the nature of this putative spin liquid phase and the relevant microscopic…

Strongly Correlated Electrons · Physics 2019-10-23 Yi-Fan Jiang , Thomas P. Devereaux , Hong-Chen Jiang

The Mott insulator a-RuCl3, featuring the intertwined interplay of spin-orbit coupling (SOC) and Kitaev spin correlations, provides an unparalleled platform for probing quantum many-body physics. Using scanning tunneling…

Strongly Correlated Electrons · Physics 2025-11-10 Wei Yue , Xiaohu Zheng , Chongli Yang , Kun Peng , Rui-Rui Du

We report a neutron scattering study of the metallic triangular lattice antiferromagnet PdCrO$_2$. Powder neutron diffraction measurements confirm that the crystalline space group symmetry remains $R\bar{3}m$ below $T_N$. This implies that…

We report inelastic neutron scattering measurements of the spin dynamics in the layered hexagonal magnet 2H-AgNiO2 which has stacked triangular layers of antiferromagnetically-coupled Ni2+ spins (S=1) ordered in a collinear alternating…

Strongly Correlated Electrons · Physics 2009-03-25 E. M. Wheeler , R. Coldea , E. Wawrzynska , T. Sorgel , M. Jansen , M. M. Koza , J. Taylor , P. Adroguer , N. Shannon

$\alpha$-RuCl$_3$ is a promising candidate material to realize the so far elusive quantum spin liquid ground state. However, at low temperatures, the coexistence of different exchange interactions couple the effective pseudospins into an…

Cu2(pymca)3(ClO4) (pymca: pyrimidine-2-carboxylate) consists of a slightly distorted honeycomb lattice of Cu2+ spins, which shows no long-range magnetic order down to 0.6 K. A magnetization study revealed 1/3 and 2/3 plateau phases [A.…

Strongly Correlated Electrons · Physics 2025-08-11 Masaaki Matsuda , Alexander I. Kolesnikov , Zentaro Honda , Tokuro Shimokawa , Sho Inoue , Yasuo Narumi , Masayuki Hagiwara

Using inelastic neutron scattering, we have observed a quasi-one-dimensional dispersive magnetic excitation in the frustrated triangular-lattice spin-2 chain oxide Ca3Co2O6. At the lowest temperature (T = 1.5 K), this magnon is…

Strongly Correlated Electrons · Physics 2013-12-17 Anil Jain , P. Y. Portnichenko , Hoyoung Jang , G. Jackeli , G. Friemel , A. Ivanov , A. Piovano , S. M. Yusuf , B. Keimer , D. S. Inosov

Pursuing the exotic quantum spin liquid (QSL) state in the Kitaev material $\alpha$-RuCl$_3$ has intrigued great research interest recently. A fascinating question is on the possible existence of field-induced QSL phase in this compound.…

Strongly Correlated Electrons · Physics 2023-09-14 Xu-Guang Zhou , Han Li , Yasuhiro H. Matsuda , Akira Matsuo , Wei Li , Nobuyuki Kurita , Gang Su , Koichi Kindo , Hidekazu Tanaka

We report a comparative neutron single crystal diffraction study of the structural and magnetic properties of layered halides CrCl$_3$ and $\alpha$-RuCl$_3$, which host a honeycomb arrangement of transition metal ions with distinct…

Strongly Correlated Electrons · Physics 2026-05-13 Zachary Morgan , Iris Ye , Jiasen Guo , Michael A McGuire , Jiaqiang Yan

The spin-orbit assisted Mott insulator $\alpha$-RuCl3 is proximate to the coveted quantum spin liquid (QSL) predicted by the Kitaev model. In the search for the pure Kitaev QSL, reducing the dimensionality of this frustrated magnet by…

As one of the most promising Kitaev quantum-spin-liquid (QSL) candidates, $\alpha$-RuCl$_3$ has received a great amount of attention. However, its ground state exhibits a long-range zigzag magnetic order, which defies the QSL phase.…