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The real-time spin dynamics and the spin noise spectra are calculated for p and n-charged quantum dots within an anisotropic central spin model extended by additional nuclear electric quadrupolar interactions (QC) and augmented by…

Mesoscale and Nanoscale Physics · Physics 2015-11-18 Johannes Hackmann , Frithjof B. Anders , Philipp Glasenapp , Alex Greilich , Manfred Bayer

Single nuclear spins in the solid state have long been envisaged as a platform for quantum computing, due to their long coherence times and excellent controllability. Measurements can be performed via localised electrons, for example those…

Among the potential spin qubit candidates, yttrium phthalocyanine double-decker (YPc$_2$) features a diamagnetic metal ion core that stabilizes the molecular structure, while its magnetic properties arise primarily from an unpaired electron…

The presence of long-range quantum spin correlations underlies a variety of physical phenomena in condensed matter systems, potentially including high-temperature superconductivity. However, many properties of exotic strongly correlated…

Experimental and theoretical studies of the dynamic magnetization in swept magnetic fields of the orthorhombic SrY$_2$O$_4$ single-crystals doped with the Dy$^{3+}$ Kramers ions (0.01 and 0.5 at.%) with natural abundances of even and odd Dy…

Hyperfine splitting in Bi$^{82+}$ and Pb$^{81+}$ ions was calculated using continuum RPA approach with effective residual forces. To fix the parameters of the theory the nuclear magnetic dipole moments of two one- particle and two one-hole…

Nuclear Theory · Physics 2009-11-07 V. F. Dmitriev , R. A. Sen'kov

We present magnetization measurements on the single molecule magnet Mn6, revealing various tunnel transitions inconsistent with a giant-spin description. We propose a dimeric model of the molecule with two coupled spins S=6, which involves…

Mesoscale and Nanoscale Physics · Physics 2008-10-06 S. Bahr , C. J. Milios , L. F. Jones , E. K. Brechin , V. Mosser , W. Wernsdorfer

Ultra-cold alkali atoms trapped in two distinct hyperfine states in an external magnetic field can mimic magnetic systems of spin 1/2 particles. We describe the spin-dependent effective interaction as a spin-spin interaction. As a…

Statistical Mechanics · Physics 2011-11-09 D. H. Santamore , Eddy Timmermans

We present the first quantum mechanical study of hyperfine effects in the rotational cluster states of a symmetric triatomic molecule H$_2$S. Rotational clusters arise from spontaneous symmetry breaking induced by high-angular-momentum…

Atomic and Molecular Clusters · Physics 2025-03-27 Andrey Yachmenev , Guang Yang

The coherent spin dynamics of electrons are investigated for CsPbI$_3$ perovskite nanocrystals in a glass matrix using time-resolved Faraday ellipticity. In nanocrystals with a diameter of about 11 nm, the Larmor precession frequency has a…

The physical properties of magnetic nanoparticles have been investigated with focus on the influence of dipolar interparticle interaction. For weakly coupled nanoparticles, thermodynamic perturbation theory is employed to derive analytical…

Materials Science · Physics 2016-08-31 Petra E. Jönsson

We have analyzed effects of the hyperfine interaction on electric dipole spin resonance when the amplitude of the quantum-dot motion becomes comparable or larger than the quantum dot's size. Away from the well known small-drive regime, the…

Mesoscale and Nanoscale Physics · Physics 2016-05-04 Stefano Chesi , Li-Ping Yang , Daniel Loss

One-dimensional metal-organic chains often possess a complex magnetic structure susceptible to be modified by a alteration of their chemical composition. The possibility to tune their magnetic properties provides an interesting playground…

The transferred hyperfine interaction between nuclear and electron spins in an heavy fermion material depends on the hybridization between the $f$-electron orbitals and those surrounding a distant nucleus. In CeMIn$_5$ (M=Rh, Ir, Co), both…

Strongly Correlated Electrons · Physics 2021-08-04 P. Menegasso , J. C. Souza , I. Vinograd , Z. Wang , S. P. Edwards , P. G. Pagliuso , N. J. Curro , R. R. Urbano

Carbon based systems are prominent candidates for a solid-state spin-qubit due to weak spin-orbit and hyperfine interactions in combination with a low natural abundance of spin carrying isotopes. We consider the effect of the hyperfine…

Mesoscale and Nanoscale Physics · Physics 2012-08-03 Moritz Fuchs , Valentin Rychkov , Björn Trauzettel

Decoherence caused by nuclear field fluctuations is a fundamental obstacle to the realization of quantum information processing using single electron spins. Alternative proposals have been made to use spin qubits based on valence band holes…

Mesoscale and Nanoscale Physics · Physics 2013-02-19 E. A. Chekhovich , A. B. Krysa , M. Hopkinson , P. Senellart , A. Lemaitre , M. S. Skolnick , A. I. Tartakovskii

Single molecule magnets distinguish themselves in the field of quantum magnetism through the ability to combine fundamental research with promising applications, the evolution of quantum spintronics in the last decade exemplifying the…

Mesoscale and Nanoscale Physics · Physics 2021-10-04 Gheorghe Taran , Edgar Bonet , Wolfgang Wernsdorfer

Hyperfine-induced electric dipole contributions may significantly increase probabilities of otherwise very weak electric octupole and magnetic quadrupole atomic clock transitions (e.g. transitions between $s$ and $f$ electron orbitals).…

Atomic Physics · Physics 2016-06-01 V. A. Dzuba , V. V. Flambaum

We present a theoretical study of the time-dependent laser alignment of molecules taking into account the hyperfine coupling due to nuclear-quadrupole interactions. The coupling of nuclear spins to the overall angular momentum of molecules…

Chemical Physics · Physics 2020-06-18 Linda V. Thesing , Andrey Yachmenev , Rosario González-Férez , Jochen Küpper

The motivation to develop materials for quantum technologies has put exploration of novel quantum states of matter at the focus of several research fields, with particular efforts towards understanding and controlling the behaviour of…

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