Related papers: Hyperfine and quadrupole interactions for Dy isoto…
An attractive feature of magnetic adatoms and molecules for nanoscale applications is their superparamagnetism, the preferred alignment of their spin along an easy axis preventing undesired spin reversal. The underlying magnetic anisotropy…
Resonant soft x-ray Bragg diffraction at the Dy M4,5 edges has been exploited to study Dy multipole motifs in DyB2C2. Our results are explained introducing the intra-atomic quadrupolar interaction between the core 3d and valence 4f shell.…
Compared to electrons, holes in InAs quantum dots have a significantly weaker hyperfine interaction that leads to less dephasing from nuclear spins. Thus many recent studies have suggested that nuclear spins are unimportant for hole spin…
This thesis contains a thorough investigation of the quantum spin dynamics in Mn12-ac and Mn6 Single-molecule magnets. In particular, we have investigated the interplay between quantum tunneling of magnetization and nuclear spin dynamics in…
Understanding the decoherence of electron spins in semiconductors due to their interaction with nuclear spins is of fundamental interest as they realize the central spin model and of practical importance for using electron spins as qubits.…
A promising platform for quantum information processing is that of silicon impurities, where the quantum states are manipulated by magnetic resonance. Such systems, in abstraction, can be considered as a nucleus of arbitrary spin coupled to…
The unique isomeric transition at 7.8 eV in $~^{229}\mathrm{Th}$ has a magnetic dipole ($M1$) and an electric quadrupole ($E2$) multipole mixing. So far, the $E2$ component has been widely disregarded. Here, we investigate the nuclear…
Strong hyperfine coupling in a 0.2% Holmium doped LiYF_4 single crystal induces staircaselike hysteresis loops of the magnetization at very low temperatures. The field sweep rate dependence of hysteresis loops allows the study of two…
We investigate theoretically the hyperfine-induced dephasing of two-electron-spin states in a double quantum dot with a finite singlet-triplet splitting J. In particular, we derive an effective pure dephasing Hamiltonian, which is valid…
We investigate the influence of interaction between tunneling particles and disorder on their avoided-level-crossing transitions in the fast-sweep limit. Whereas the results confirm expectations based on the mean-field arguments that…
We apply an elementary measurement scheme to calculate the electronic triplet-singlet transition mediated by hyperfine interaction in a double quantum dot. We show how the local character of the hyperfine interaction and the nuclear…
Hyperfine structures of $^{211}$Fr due to the interactions of magnetic dipole ($\mu$), electric quadrupole ($Q$) and magnetic octupole ($\Omega$) moments with the electrons are investigated using the relativistic coupled-cluster (RCC)…
We revisited the electronic structure parameters used to interpret the hyperfine structure of neutral polonium. We used a computational scheme that treats relativistic and high-order electronic correlation effects within the coupled cluster…
We present an expression for the operator of the electric quadrupole hyperfine interaction which takes into account finite nuclear size. We compare the results obtained with the use of this operator with those obtained in the standard…
Hyperfine interactions couple nuclear and electronic degrees of freedom. The present work explores how hyperfine coupling within the Tm ions in TmVO$_4$ single crystals affects an electronic ferroquadrupole ordered ground state and its…
Nuclear magnetic resonance gyroscopes that detect rotation as a shift in the precession frequency of nuclear spins, have attracted a lot of attentions. Under a feedback-generated drive, the precession frequency is supposed to be dependent…
We study the exchange interaction between two hole-spin qubits in a double quantum dot setup in a silicon nanowire in the presence of magnetic and electric fields. Based on symmetry arguments we show that there exists an effective spin that…
We discuss low-temperature properties of magnets with integer spin and large single-ion easy-plane anisotropy $D$ in transverse magnetic field $h$. Considering the exchange interaction between spins as a perturbation and using the diagram…
Atomic spectroscopy is used to search for the space-time variation of fundamental constants which may be due to an interaction with scalar and pseudo-scalar (axion) dark matter. In this letter, we study the effects which are produced by the…
We report a systematic study of the hyperfine interaction between the electron spin of a single nitrogen-vacancy (NV) defect in diamond and nearby $^{13}$C nuclear spins, by using pulsed electron spin resonance spectroscopy. We isolate a…