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We demonstrate precision measurement and control of inhomogeneous broadening in a multi-ion clock consisting of three $^{176}$Lu$^+$ ions. Microwave spectroscopy between hyperfine states in the $^3D_1$ level is used to characterise…

We devise a perturbation-immune version of Ramsey's method of separated oscillatory fields. Spectroscopy of an atomic clock transition without compromising the clock's accuracy is accomplished by actively balancing the spectroscopic…

Atomic Physics · Physics 2018-02-14 Christian Sanner , Nils Huntemann , Richard Lange , Christian Tamm , Ekkehard Peik

We develop a method of modified hyper-Ramsey spectroscopy in optical clocks, achieving complete immunity to the frequency shifts induced by the probing fields themselves. Using particular pulse sequences with tailored phases, frequencies,…

Atomic Physics · Physics 2016-01-27 R. Hobson , W. Bowden , S. A. King , P. E. G. Baird , I. R. Hill , P. Gill

We evaluate the feasibility of using magnetic-dipole (M1) transitions in highly-charged ions as a basis of an optical atomic clockwork of exceptional accuracy. We consider a range of possibilities, including M1 transitions between clock…

Atomic Physics · Physics 2015-06-23 V. I. Yudin , A. V. Taichenachev , A. Derevianko

In this work, the peculiarities of Ramsey resonance and its sensitivity to the light shift from an optically dense medium of cold atoms are investigated. We considered different composite pulse protocols for clock spectroscopy such as…

Atomic Physics · Physics 2019-07-26 K. A. Barantsev , T. Zanon-Willette , A. N. Litvinov

Hyper-Ramsey protocols effectively reduce AC-Stark shifts in probing ultra-narrow optical clock transitions but they remain sensitive to laser intensity noise, decoherence, frequency drifts, and low-frequency perturbations. We address these…

Atomic Physics · Physics 2025-12-25 T. Zanon-Willette , B. Ilikj , D. Wilkowski , B. Darquié , N. V. Vitanov

We experimentally investigate an optical frequency standard based on the $^2S_{1/2} (F=0)\to {}^2F_{7/2} (F=3)$ electric octupole (\textit{E}3) transition of a single trapped $^{171}$Yb$^+$ ion. For the spectroscopy of this strongly…

Atomic and Molecular Clusters · Physics 2016-02-15 N. Huntemann , C. Sanner , B. Lipphardt , Chr. Tamm , E. Peik

We evaluate the electric quadrupole moments of the ${^1}\!S_0$ and ${^3}\!P_0$ clock states of $^{27}$Al$^+$ and $^{115}$In$^+$. To capture all dominant contributions, our analysis extends through third order of perturbation theory and…

Atomic Physics · Physics 2017-04-11 K. Beloy , D. R. Leibrandt , W. M. Itano

The stability of an optical atomic clock is a critical figure of merit for almost all clock applications. To this end, much optical atomic clock research has focused on reducing clock instability by increasing the atom number, lengthening…

Atomic Physics · Physics 2023-12-21 Xin Zheng , Jonathan Dolde , Shimon Kolkowitz

We report on an absolute frequency measurement of the ${\rm Lu}^{+}\,(^{3}\rm D_1)$ standard frequency which is defined as the hyperfine-average of $^{1}\rm S_0$ to $^{3}\rm D_1$ optical clock transitions in $^{176}{\rm Lu}^{+}$. The…

Atomic Physics · Physics 2026-01-12 Zhao Zhang , Qi Zhao , Qin Qichen , N. Jayjong , M. D. K. Lee , K. J. Arnold , M. D. Barrett

We develop an universal method to significantly suppress probe-induced shifts in any types of atomic clocks using the Ramsey spectroscopy. Our approach is based on adaptation of the synthetic frequency concept [V. I. Yudin, et al., Phys.…

Atomic Physics · Physics 2016-11-15 V. I. Yudin , A. V. Taichenachev , M. Yu. Basalaev , T. Zanon-Willette

We study and characterize a quasi-continuous dynamical decoupling (QCDD) scheme that effectively suppresses dominant frequency shifts in a multi-ion optical clock. Addressing the challenge of inhomogeneous frequency shifts in such systems,…

Atomic Physics · Physics 2024-08-13 Nitzan Akerman , Roee Ozeri

We present non-standard optical Ramsey schemes that use pulses individually tailored in duration, phase, and frequency to cancel spurious frequency shifts related to the excitation itself. In particular, the field shifts and their…

Hyperfine-induced electric dipole contributions may significantly increase probabilities of otherwise very weak electric octupole and magnetic quadrupole atomic clock transitions (e.g. transitions between $s$ and $f$ electron orbitals).…

Atomic Physics · Physics 2016-06-01 V. A. Dzuba , V. V. Flambaum

The next generation of atomic frequency standards based on an ensemble of neutral atoms or a single-ion will provide very stringent tests in metrology, applied and fundamental physics requiring a new step in very precise control of external…

Atomic Physics · Physics 2016-07-07 T. Zanon-Willette , M. Minissale , V. I. Yudin , A. V. Taichenachev

We report precision measurement of the unperturbed ${^{3}}D_1$ microwave transition frequencies in $^{176}\mathrm{Lu}^+$ to a fractional uncertainty of $4\times10^{-14}$. We find the $|F,m_F\rangle=|8,0\rangle$ to $|7,0\rangle$ hyperfine…

Atomic Physics · Physics 2025-10-09 M. D. K. Lee , Qi Zhao , Qin Qichen , Zhao Zhang , N. Jayjong , K. J. Arnold , M. D. Barrett

We consider hyperfine-mediated effects for clock transitions in $^{176}$Lu$^+$. Mixing of fine structure levels due to the hyperfine interaction bring about modifications to Land\'e $g$-factors and the quadrupole moment for a given state.…

Atomic Physics · Physics 2020-09-08 Zhiqiang Zhang , K. J. Arnold , R. Kaewuam , M. S. Safronova , M. D. Barrett

We introduce a scheme to coherently suppress second-rank tensor frequency shifts in atomic clocks, relying on the continuous rotation of an external magnetic field during the free atomic state evolution in a Ramsey sequence. The method…

Atomic Physics · Physics 2020-10-07 R. Lange , N. Huntemann , C. Sanner , H. Shao , B. Lipphardt , Chr. Tamm , E. Peik

Current optical atomic clocks do not utilize their resources optimally. In particular, an exponential gain in sensitivity could be achieved if multiple atomic ensembles were to be controlled or read-out individually, even without…

Measurement science now connects strongly with engineering of quantum coherence, many-body states, and entanglement. To scale up the performance of an atomic clock using a degenerate Fermi gas loaded in a three-dimensional optical lattice,…

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