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We develop the method of Ramsey spectroscopy with the use of an additional field compensating the frequency shifts of clock optical transitions. This method in combination with the method of magnetically induced excitation of strongly…

Atomic Physics · Physics 2008-10-22 A. V. Taichenachev , V. I. Yudin , C. W. Oates , Z. W. Barber , L. Hollberg

We present a new interrogation scheme for the next generation of quantum clocks to suppress frequency-shifts induced by laser probing fields themselves based on Generalized Hyper-Ramsey resonances. Sequences of composite laser pulses with…

Atomic Physics · Physics 2016-04-19 Thomas Zanon-Willette , Emeric de Clercq , Ennio Arimondo

Ramsey interferometry is a cornerstone technique for precise measurement of time and frequency in modern clocks. The Ramsey experiments are typically done in optically dilute samples of atoms to improve homogeneity and avoid back-action of…

Quantum Physics · Physics 2025-05-20 S. A. Moiseev , K. I. Gerasimov , M. M. Minnegaliev , I. V. Brekotkin , E. S. Moiseev

Laser decoherence limits the stability of optical clocks by broadening the observable resonance linewidths and adding noise during the dead time between clock probes. Correlation spectroscopy avoids these limitations by measuring correlated…

We present a novel method for engineering an optical clock transition that is robust against external field fluctuations and is able to overcome limits resulting from field inhomogeneities. The technique is based on the application of…

Atomic Physics · Physics 2019-12-03 Nati Aharon , Nicolas Spethmann , Ian D. Leroux , Piet O. Schmidt , Alex Retzker

Increasing coherent interrogation times is central to advancing the precision of optical clocks. Synchronous differential optical clock comparisons have now demonstrated atomic coherence times that far exceed the coherence time of the clock…

High precision spectroscopy of the $^1S_0$-to-${^1}D_2$ clock transition of $^{176}$Lu is reported. Measurements are performed with Hertz level precision with the accuracy of the hyperfine-averaged frequency limited by the calibration of an…

Atomic Physics · Physics 2019-03-06 R. Kaewuam , T. R. Tan , K. J. Arnold , M. D. Barrett

We present the experimental realization of a continuous dynamical decoupling scheme which suppresses leading frequency shifts in a multi-ion frequency reference based on $^{40}\mathrm{Ca}^+$. By near-resonant magnetic coupling of the…

Rapid progress in the precision and accuracy of optical atomic clocks over the last decade has advanced the frontiers of timekeeping, metrology, and quantum science. However, the stabilities of most optical clocks remain limited by the…

Atomic Physics · Physics 2022-03-09 Xin Zheng , Jonathan Dolde , Varun Lochab , Brett N. Merriman , Haoran Li , Shimon Kolkowitz

We report the first laser spectroscopy of the $^1$S$_0$ to $^3$D$_1$ clock transition in $^{175}$Lu$^+$. Clock operation is demonstrated on three pairs of Zeeman transitions, one pair from each hyperfine manifold of the $^3$D$_1$ term. We…

Atomic Physics · Physics 2017-03-07 Kyle J. Arnold , R. Kaewuam , A. Roy , E. Paez , S. Wang , M. D. Barrett

Quantum engineering of time-separated Raman laser pulses in three-level systems is presented to produce an ultra-narrow optical transition in bosonic alkali-earth clocks free from light shifts and with a significantly reduced sensitivity to…

Atomic Physics · Physics 2015-03-26 T. Zanon-Willette , S. Almonacil , E. de Clercq , A. D. Ludlow , E. Arimondo

We show that by averaging over transitions to multiple hyperfine levels, quadrupole shifts and dominant Zeeman effects exactly cancel whenever the nuclear spin, I, is at least as large as the total electronic angular momentum, J. The…

Quantum Physics · Physics 2014-11-04 M. D. Barrett

Accurate measurements of different transition frequencies between atomic levels of the electronic and hyperfine structure over time are used to investigate temporal variations of the fine structure constant $\alpha$ and the…

Atomic Physics · Physics 2014-12-01 N. Huntemann , B. Lipphardt , Chr. Tamm , V. Gerginov , S. Weyers , E. Peik

We study the Ho$^{14+}$ ion as a candidate for extremely accurate and stable optical atomic clock which is sensitive to the time variation of the fine structure constant. We demonstrate that the proposed system has all desired features…

Atomic Physics · Physics 2015-03-05 V. A. Dzuba , V. V. Flambaum , Hidetoshi Katori

Determining light shift in Raman-Ramsey interference is important for the development of atomic frequency standards based on a vapor cell. We have accurately calculated light shift in Raman-Ramsey interference using the density-matrix…

Optics · Physics 2015-06-23 G. S. Pati , Z. Warren , N. Yu , M. S. Shahriar

We present and implement a non-destructive detection scheme for the transition probability readout of an optical lattice clock. The scheme relies on a differential heterodyne measurement of the dispersive properties of lattice-trapped atoms…

Atomic Physics · Physics 2017-09-13 G. Vallet , E. Bookjans , U. Eismann , S. Bilicki , R. Le Targat , J. Lodewyck

We present a method that uses radio-frequency pulses to cancel the quadrupole shift in optical clock transitions. Quadrupole shifts are an inherent inhomogeneous broadening mechanism in trapped ion crystals, limiting current optical ion…

Quantum Physics · Physics 2019-06-12 Ravid Shaniv , Nitzan Akerman , Tom Manovitz , Yotam Shapira , Roee Ozeri

Multi-ion optical clocks offer the possibility of overcoming the low signal-to-noise ratio of single-ion clocks, while still providing low systematic uncertainties. We present simultaneous spectroscopy of up to four ${}^{115}$In${}^+$ clock…

Numerous few-electron atomic systems are considered which can be used effectively for observing a potential variation of the fine-structure constant $\alpha$ and the electron-proton mass ratio $m_e/m_p$. We examine optical magnetic dipole…

We perform high resolution spectroscopy on $^{176}$Lu$^+$ including the $^1S_0\leftrightarrow{^3}D_1$ and $^1S_0\leftrightarrow{^3}D_2$ clock transitions. Hyperfine structures and optical frequencies relative to the $^1S_0$ ground state of…

Atomic Physics · Physics 2019-01-09 R. Kaewuam , A. Roy , T. R. Tan , K. J. Arnold , M. D. Barrett