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We employ ultrafast pump-probe spectroscopy to directly monitor electron tunneling between discrete orbital states in a pair of spatially separated quantum dots. Immediately after excitation, several peaks are observed in the pump-probe…

We present the design, fabrication and discuss the performance of a new combined high-resolution Scanning Tunneling and thermopower Microscope (STM/SThEM). We also describe the development of the electronic control, the user interface, the…

Tailoring nanoparticles composition and morphology is of particular interest for improving their performance for catalysis. A challenge of this approach is that the nanoparticles optimized initial structure often changes during use.…

Conventional quantum transport methods can provide quantitative information on spin, orbital, and valley states in quantum dots, but often lack spatial resolution. Scanning tunneling microscopy, on the other hand, provides exquisite spatial…

Nuclear spins owe their long-lived magnetic states to their excellent isolation from the environment. At the same time, a finite degree of interaction with their surroundings is necessary for reading and writing the spin state. Therefore,…

We introduce the concept of Plasmonic Parametric Resonance (PPR) as a novel way to amplify high angular momentum plasmonic modes of nanoparticles by means of a simple uniform optical pump. In analogy with parametric resonance in dynamical…

Optics · Physics 2018-02-13 Alessandro Salandrino

On the spin-valve-like ferromagnet/spin glass/ferromagnet (FM/SG/FM) structure, the tunneling current is dominated by resistance switch (RS) instead of the local density of states according to the conventional tunneling theory. Here we show…

A scanning tunneling microscope (STM) can probe the inelastic spin excitations of single magnetic atoms in a surface via spin-flip assisted tunneling. A particular and intriguing case is the Mn dimer case. We show here that the existing…

Mesoscale and Nanoscale Physics · Physics 2022-08-31 F. Delgado , J. Fernández-Rossier

Recent experimental conductance measurements performed on paramagnetic molecular adsorbates on a superconducting surface, using superconducting scanning tunneling microscopy techniques, are theoretically investigated. For low temperatures,…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 P. Berggren , J. Fransson

We consider fluctuations of the electronic spin due to coupling to nuclear spin. Noise spectroscopy of an electronic spin can be revealed in the Scanning Tunnelling Microscope (STM). We argue that the noise spectroscopy of electronic spin…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 A. V. Balatsky , J. Fransson , D. Mozyrsky , Yishay Manassen

We present a broadband microwave setup for electrically detected magnetic resonance (EDMR) based on microwave antennae with the ability to apply arbitrarily shaped pulses for the excitation of electron spin resonance (ESR) and nuclear…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 F. M. Hrubesch , G. Braunbeck , A. Voss , M. Stutzmann , M. S. Brandt

We describe a simple experimental method to detect electron paramagnetic resonance (EPR) in polycrystalline 2,2-diphenyl-1-picrylhydrazyl (DPPH) sample, the standard g-marker for EPR spectroscopy, without using a cavity resonator or a…

Materials Science · Physics 2021-04-23 Lee Yong Heng , Ushnish Chaudhuri , Ramanathan Mahendiran

Localized spin states in conventional superconductors at low temperatures are expected to have long decoherence time due to the strong suppression of spin relaxation channels. We propose a scanning tunneling microscopy (STM) experiment…

Superconductivity · Physics 2007-05-23 Jurij Smakov , Ivar Martin , Alexander V. Balatsky

Recently developed electronic pre-resonance stimulated Raman scattering (epr-SRS) microscopy, in which the Raman signal of a dye is significantly boosted by setting the incident laser frequency near the electronic excitation energy, has…

Chemical Physics · Physics 2023-03-10 Jiajun Du , Xuecheng Tao , Tomislav Begušić , Lu Wei

A multi-high-frequency electron paramagnetic resonance method is used to probe the magnetic excitations of a dimer of single-molecule magnets. The measured spectra display well resolved quantum transitions involving coherent superposition…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 S. Hill , R. S. Edwards , N. Aliaga-Alcalde , G. Christou

We report the first study of the micro-SQUID response of a molecular system to electromagnetic radiation. The advantages of our micro-SQUID technique in respect to pulsed electron paramagnetic resonance (EPR) techniques consist in the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 W. Wernsdorfer , A. Mueller , D. Mailly , B. Barbara

Using a Magnetic Resonace Force Microscope, we have performed ferromagnetic resonance (FMR) spectroscopy on parametric magnons created by 4-wave process. This is achieved by measuring the differential response to a small source modulation…

Materials Science · Physics 2011-11-09 G. De Loubens , V. V. Naletov , Vincent Charbois , Olivier Klein , V. S. Tiberkevich , Andrei Slavin

We describe a fully ultra-high vacuum compatible scanning tunneling microscope (STM) optimized for radio-frequency signals. It includes in-situ exchangeable tips adapted to high frequency cabling and a standard sample holder, which offer…

Mesoscale and Nanoscale Physics · Physics 2013-02-27 Christian Saunus , Jan Raphael Bindel , Marco Pratzer , Markus Morgenstern

Electron neutral collision frequency is measured using both grounded and floating hairpin resonator probes in a 27 MHz parallel plate capacitively coupled plasma (CCP). Operating conditions are 0.1-2 Torr (13.3-267 Pa) in Ar, He, and Ar-He…

Plasma Physics · Physics 2017-09-11 David J Peterson , Philip Kraus , Thai Cheng Chua , Lynda Larson , Steven C Shannon

We propose an atom-superposition-based method for simulating spin-polarized scanning tunneling microscopy (SP-STM) from first principles. Our approach provides bias dependent STM images in high spatial resolution, with the capability of…

Materials Science · Physics 2011-11-28 Krisztián Palotás , Werner A. Hofer , László Szunyogh