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The spintronic properties of magnetic molecules have attracted significant scientific attention. Special emphasis has been placed on the qubit for quantum information processing. The single molecule magnet, bis(phthalocyaninato (Pc))…

Electrochemical strains are a ubiquitous feature of solid state ionic devices ranging from ion batteries and fuel cells to electroresistive and memristive memories. Recently, we proposed a scanning probe microscopy (SPM) based approach,…

Materials Science · Physics 2015-06-03 A. N. Morozovska , E. A. Eliseev , S. V. Kalinin

The role of the tip in inelastic electron tunneling spectroscopy (IETS) performed with scanning tunneling microscopes (STM) is theoretically addressed via first-principles simulations of vibrational spectra of single carbon monoxide (CO)…

Mesoscale and Nanoscale Physics · Physics 2011-04-12 Aran Garcia-Lekue , Daniel Sanchez-Portal , Andres Arnau , Thomas Frederiksen

We herein estimate the effect of lattice defects on the line shape of electron paramagnetic resonance (EPR) signals from a single crystal of the S=10 single-molecule magnet Mn$_{12}$ with the external magnetic field along the crystal c…

Condensed Matter · Physics 2009-11-07 Kyungwha Park , N. S. Dalal , P. A. Rikvold

The Quantum Twisting Microscope (QTM) is a groundbreaking instrument that enables energy- and momentum-resolved measurements of quantum phases via tunneling spectroscopy across twistable van der Waals heterostructures. In this work, we…

We present a novel method that combines spin resonance spectroscopy with transmission electron microscopy (TEM), enabling localized in-situ detection of microwave (MW)-driven spin excitations. Our approach utilizes continuous wave MW…

Understanding the interaction of charge carriers with lattice vibrations in the quasi-equilibrium regime is crucial for semiconductor functionality. However, the structural signatures of these interactions are often too subtle for…

Materials Science · Physics 2026-03-11 Guy Reuveni , Maya Levy Greenberg , Matan Menahem , Olle Hellman , Omer Yaffe

On-chip Electron Spin Resonance (ESR) of magnetic molecules requires the ability to precisely position nanosized samples in antinodes of the electro-magnetic field for maximal magnetic interaction. A method is developed to entrap…

Mesoscale and Nanoscale Physics · Physics 2009-08-28 N. Groll , S. Bertaina , M. Pati , N. S. Dalal , I. Chiorescu

We report a new technique of scanning capacitance microscopy at microwave frequencies. A near field scanning microwave microscope probe is kept at a constant height of about 1nm above the samplewith the help of Scanning Tunneling Microscope…

Materials Science · Physics 2007-05-23 Atif Imtiaz , Steven M. Anlage

Recent radio frequency scanning tunneling spectroscopy (rf-STS) experiments have demonstrated nuclear and electron spin excitations up to $\pm12\hbar$ in a single molecular spin quantum dot (qudot). Despite the profound experimental…

In this paper, we present a rapidly-prototyped, costefficient, 3D-printed quasioptical sample holder for improving the signal-to-noise ratio (SNR) in modern, resonator-free, highfield electron paramagnetic resonance (EPR) spectrometers.…

Instrumentation and Detectors · Physics 2024-01-04 Antonin Sojka , Brad D. Price , Mark S. Sherwin

Electron Spin Resonance (ESR) can microscopically probe both conduction electrons (ce) and local moment (LM) spin systems in different materials. A ce spin resonance (CESR) is observed in metallic systems based on light elements or with…

Strongly Correlated Electrons · Physics 2009-08-04 L. M. Holanda , J. M. Vargas , C. Rettori , S. Nakatsuji , K. Kuga , Z. Fisk , S. B. Oseroff , P. G. Pagliuso

Detecting the photons emitted from single quantum objects is highly desired to diagnose nano-scale devices. It has been, however, believed very difficult to sense single atoms in optical spectroscopy due to the inferior detection…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Kazu Suenaga , Toshiya Okazaki , Eiji Okunishi , Syo Matsumura

We propose a new technique for the detection of single atoms in ultracold quantum gases. The technique is based on scanning electron microscopy and employs the electron impact ionization of trapped atoms with a focussed electron probe.…

Statistical Mechanics · Physics 2007-05-23 T. Gericke , C. Utfeld , N. Hommerstad , H. Ott

Quantum tunnelling of electrons can be confined to the sub-cycle time scale of strong light fields, contributing decisively to the extreme time resolution of attosecond science. Because tunnelling also enables atomic-scale spatial…

Creating a quantum-coherent architecture at the atomic scale has long been an ambition in quantum science and nanotechnology. This ultimate length scale requires the use of fundamental quantum properties of atoms, such as the spin of…

The molecular dark state participates in many important photon-induced processes, yet is typically beyond the optical-spectroscopic measurement due to the forbidden transition dictated by the selection rule. In this work, we propose to use…

Quantum Physics · Physics 2021-11-09 Guohui Dong , Zhubin Hu , Xiang Sun , Hui Dong

We have developed a broadband scanning tunnelling microscope capable of conventional, low frequency (<10 kHz), microscopy as well spectroscopy and shot-noise detection at 1 MHz. After calibrating our AC circuit on a gold surface, we…

Mesoscale and Nanoscale Physics · Physics 2018-09-28 Freek Massee , Quan Dong , Antonella Cavanna , Yong Jin , Marco Aprili

The Electron Paramagnetic Spectroscopy (EPR) is the most direct and powerful method for the detection and identification of free radicals and other species with unpaired electrons. Statistics disorders are a common gynaecological disorder…

Electric Scanning Probe Microscopies are used to characterize the surface behavior of ferroelectric materials. The effects of local charge density on the chemistry and physics of ferroelectric surfaces are investigated. The kinetics and…

Materials Science · Physics 2007-05-23 Sergei V. Kalinin , Dawn A. Bonnell
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