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Transport and non-equilibrium magnetization in monolayers of magnetic molecules subject to a bias voltage are considered. We apply a master-equation approach going beyond the sequential-tunneling approximation to study the Coulomb-blockade…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Florian Elste , Carsten Timm

We have used a combined dynamic scanning tunneling and atomic force microscope to study the organisation of weakly bound adsorbed molecules on a graphite substrate. Specifically we have acquired images of islands of the perylene derivative…

Materials Science · Physics 2009-11-13 N. Berdunov , A. J. Pollard , P. H. Beton

The interplay between magnetism, band topology, and electronic correlation in low dimensions has been a fascinating subject of research. Here, we propose two-dimensional (2D) material systems which demonstrate such an interesting interplay.…

Materials Science · Physics 2020-12-24 Bo Tai , Weikang Wu , Xiaolong Feng , Yalong Jiao , Jianzhou Zhao , Yunhao Lu , Xian-Lei Sheng , Shengyuan A. Yang

The magnetic tetrapyrrole molecules (such as porphyrins and phthalocyanines) with an active transition metal atom in their centre are currently intensively studied as prosperous potential elements of devices for high-density information…

Materials Science · Physics 2022-10-06 Aleksei Koshevarnikov , Tomi Ketolainen , Jacek A. Majewski

Electrically manipulating the quantum properties of nano-objects, such as atoms or molecules, is typically done using scanning tunnelling microscopes and lateral junctions. The resulting nanotransport path is well established in these model…

We study the spin-orbit torque (SOT) effective fields in Cr/CoFeAl/MgO and Ru/CoFeAl/MgO magnetic heterostructures using the adiabatic harmonic Hall measurement. High-quality perpendicular-magnetic-anisotropy CoFeAl layers were grown on Cr…

Materials Science · Physics 2016-03-15 Zhenchao Wen , Junyeon Kim , Hiroaki Sukegawa , Masamitsu Hayashi , Seiji Mitani

The structural and magnetic properties of spinel compounds $CoB_2O_4$ (B=Cr,Mn and Fe) are studied using the DFT+U method and generalized gradient approximation (GGA). We concentrate on understanding the trends in the properties of these…

Strongly Correlated Electrons · Physics 2016-09-21 Debashish Das , Rajkumar Biswas , Subhradip Ghosh

The equiatomic quaternary Heusler alloy CoFeCrAl is a candidate material for spin-gapless semiconductors (SGSs). However, to date, there have been no experimental attempts at fabricating a junction device. This paper reports a fully…

Based on the standard tight-binding model of the graphene $\pi$-band electronic structure, the extended H\"uckel model for the adsorbate and graphene carbon atoms, and spin splittings estimated from density functional theory (DFT), the…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Alireza Saffarzadeh , George Kirczenow

Using first-principles calculations we demonstrate sizable exchange coupling between a magnetic molecule and a magnetic substrate via a graphene layer. As a model system we consider cobaltocene (CoCp$_2$) adsorbed on graphene deposited on…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 Simone Marocchi , Paolo Ferriani , Nuala Mai Caffrey , Franca Manghi , Stefan Heinze , Valerio Bellini

The tris pyrazolyl borate ligand imposes a rigid scaffold around Fe( ii ) ensuring a robust magnetic anisotropy when the molecules assembled as monolayers suffer from the dissymmetric environment of the substrate/vacuum interface.

We investigate transport through 6 to 10 nm thin epitaxial GaAs(001) barriers sandwiched between polycrystalline iron films. Apart from a pronounced tunneling magnetoresistance effect (TMR) at low magnetic fields we observe a distinct…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 M. Zenger , J. Moser , W. Wegscheider , D. Weiss , T. Dietl

We report the emergence of adsorption-induced magnetism from heterohelicene molecules on a non-magnetic Cu(100) surface. Spin-polarized low-energy electron microscopy (SP-LEEM) measurements reveal spin-dependent electron reflectivity for…

The electronic structure and magnetic properties of the graphene/Fe/Ni(111) system were investigated via combination of the density functional theory calculations and electron-spectroscopy methods. This system was prepared via intercalation…

Materials Science · Physics 2017-09-13 M. Weser , E. N. Voloshina , K. Horn , Yu. S. Dedkov

Magnetic properties of nanometer thick Co films intercalated at the graphene/Ir(111) interface are investigated using spin-polarized low-energy electron microscopy (SPLEEM) and Auger electron spectroscopy. We show that the graphene top…

Materials Science · Physics 2014-04-04 N. Rougemaille , A. T. N'Diaye , J. Coraux , C. Vo-Van , O. Fruchart , A. K. Schmid

Controlling magnetic anisotropy energy (MAE) in two-dimensional (2D) ferromagnetic materials is crucial for designing novel spintronic devices. Using first-principles calculations, we systematically investigate the magnetic properties of…

Materials Science · Physics 2024-11-22 Xunwu Hu , Dao-Xin Yao , Kun Cao

Recently, magnetic tunnel junctions with perpendicular magnetized electrodes combined with exchange bias films have attracted large interest. In this paper we examine the tunnel magnetoresistance of…

One of the key factors behind the rapid evolution of molecular spintronics is the efficient realization of spin manipulation of organic molecules with a magnetic center. The spin state of such molecules may depend crucially on the…

We investigate a well defined heterostructure constituted by magnetic Fe layers sandwiched between graphene (Gr) and Ir(111). The challenging task to avoid Fe-C solubility and Fe-Ir intermixing has been achieved with atomic controlled Fe…

Thin van der Waals (vdW) layered magnetic materials disclose the possibility to realize vdW heterostructures with new functionalities. Here we report on the realization and investigation of tunneling spin valves based on van der Waals…

Mesoscale and Nanoscale Physics · Physics 2018-06-15 Zhe Wang , Deepak Sapkota , Takashi Taniguchi , Kenji Watanabe , David Mandrus , Alberto F. Morpurgo