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We report measurements and theoretical analysis of resonant spin tunneling in randomly oriented nanospheres of a molecular magnet. Amorphous nanospheres of Mn$_{12}$ acetate have been fabricated and characterized by chemical, infrared, TEM,…

Mesoscale and Nanoscale Physics · Physics 2015-07-30 S. Lendinez , R. Zarzuela , J. Tejada , M. W. Terban , S. J. L. Billinge , J. Espin , I. Imaz , D. Maspoch , E. M. Chudnovsky

The capacity to externally manipulate magnetic properties is highly desired from both fundamental and technological perspectives, particularly in the development of magnetoelectronics and spintronics devices. Here, using first-principles…

Materials Science · Physics 2024-02-27 Rui-Qi Wang , Tian-Min Lei , Yue-Wen Fang

We investigate the structure, chemical bonding, electronic properties, and magnetic behavior of a three-dimensional graphitic network in aba and aaa stacking with intercalated transition metal atoms (Mn, Fe, Co, Ni, and Cu). Using density…

Mesoscale and Nanoscale Physics · Physics 2012-07-03 T. P. Kaloni , M. Upadhyay Kahaly , U. Schwingenschlögl

A detailed study of the ground state of the Coulomb system $(\al \al e e)$ which corresponds to the $He_2^{2+}$ molecular ion in a magnetic field $B=0-4.414 \times 10^{13} $ G in parallel configuration (infinitely massive $\al-$particles…

Astrophysics · Physics 2008-11-26 A. V. Turbiner , N. L. Guevara

Density functional theory and nonequilibrium Green's function calculations have been used to explore spin-resolved transport through the high-spin state of an iron(II)sulfur single molecular magnet. Our results show that this molecule…

Materials Science · Physics 2017-04-25 Sherif Abdulkader Tawfik , Leigh Weston , X. Y. Cui , Simon Ringer , Catherine Stampfl

We propose cotunneling as the microscopic mechanism that makes possible inelastic electron spectroscopy of magnetic atoms in surfaces for a wide range of systems, including single magnetic adatoms, molecules and molecular stacks. We…

Mesoscale and Nanoscale Physics · Physics 2011-08-26 F. Delgado , J. Fernández-Rossier

The electronic structure and magnetism of a new magnetic intercalation compound (Li0.8Fe0.2)OHFeSe are investigated theoretically. The electronic structure calculations predict that the Fe in the (Li,Fe)OH intercalated layer is in +2…

Strongly Correlated Electrons · Physics 2017-02-14 Da-Yong Liu , Zhe Sun , Liang-Jian Zou

We present a detailed first principles study on the magnetic structure of an Fe monolayer on different surfaces of 5d transition metals. We use the spin-cluster expansion technique to obtain parameters of a spin model, and predict the…

Materials Science · Physics 2014-05-06 E. Simon , K. Palotás , B. Ujfalussy , A. Deák , G. M. Stocks , L. Szunyogh

The magnetic structure of a Cr monolayer on a W(110) substrate is investigated by means of first-principles calculations based on the noncollinear spin density functional theory (DFT). As magnetic ground state we find a long-period…

Materials Science · Physics 2016-01-26 Bernd Zimmermann , Marcus Heide , Gustav Bihlmayer , Stefan Blügel

Discontinuous magnetic multilayers [CoFe/Al2O3] are studied by use of magnetometry, susceptometry and numeric simulations. Soft ferromagnetic Co80Fe20 nanoparticles are embedded in a diamagnetic insulating a-Al2O3 matrix and can be…

Materials Science · Physics 2010-09-13 O. Petracic , X. Chen , S. Bedanta , W. Kleemann , S. Sahoo , S. Cardoso , P. P. Freitas

Motivated in part by experiments performed by M.H. Pan et al. (nanoletters, v.5, p 83, 2005), we have undertaken a theoretical study of the the magnetic properties of two-monolayer thick Co nanoplatelets with an equilateral triangular…

Other Condensed Matter · Physics 2009-11-11 T. O. Strandberg , C. M. Canali , A. H. MacDonald

The low temperature spin dynamics of a Fe8 Single-Molecule Magnet was studied under circularly polarized electromagnetic radiation allowing us to establish clearly photon-assisted tunneling. This effect, while linear at low power, becomes…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 L. Sorace , W. Wernsdorfer , C. Thirion , A. -L. Barra , M. Pacchioni , D. Mailly , B. Barbara

Graphene is expected to complement todays Si-based information technology. In particular, magnetic molecules in contact with graphene constitute a tantalizing approach towards organic spin electronics because of the reduced conductivity…

Materials Science · Physics 2013-04-18 C. F. Hermanns , K. Tarafder , M. Bernien , A. Krüger , Y. -M. Chang , P. M. Oppeneer , W. Kuch

Recent experimental advances in scanning tunneling microscopy make the measurement of the conductance spectra of isolated and magnetically coupled atoms on nonmagnetic substrates possible. Notably these spectra are characterized by a…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Aaron Hurley , Nadjib Baadji , Stefano Sanvito

All van der Waals (vdW) Fe3GeTe2/Cr2Ge2Te6/graphite magnetic heterojunctions have been fabricated via mechanical exfoliation and stacking, and their magnetotransport properties are studied in detail. At low bias voltages large negative…

Materials Science · Physics 2022-10-26 Honglei Feng , Gang Shi , Dayu Yan , Yong Li , Youguo Shi , Yang Xu , Peng Xiong , Yongqing Li

We present a study of the electronic structure and magnetism of Co$_2$MnAl, CoMnVAl and their heterostructure. We employ a combination of density-functional theory and dynamical mean-field theory (DFT+DMFT). We find that Co$_2$MnAl is a…

Materials Science · Physics 2018-01-12 Igor Di Marco , Andreas Held , Samara Keshavarz , Yaroslav O. Kvashnin , Liviu Chioncel

Spin-electronic devices are poised to become part of mainstream microelectronic technology .Downsizing them, however, faces the intrinsic difficulty that as ferromagnets become smaller, it becomes more difficult to stabilize their magnetic…

The structure and magnetic properties of Co clusters, comprising from 26 to 2700 atoms, self-organized or not on the graphene/Ir(111) moir\'e, were studied in situ with the help of scanning tunneling microscopy and X-ray magnetic circular…

HRTEM, nano-beam electronic diffraction, energy dispersive X-rays scanning spectroscopy, Vibrating Sample Magnetometry (VSM) and FerroMagnetic Resonance (FMR) techniques are used in view of comparing (static and dynamic) magnetic and…

We have used spin-polarized scanning tunneling spectroscopy to observe the spin-polarization state of individual Fe and Cr atoms adsorbed onto Co nanoislands. Both of these magnetic adatoms exhibit stationary out-of-plane spin-polarization…

Materials Science · Physics 2009-11-13 Y. Yayon , V. W. Brar , L. Senapati , S. C. Erwin , M. F. Crommie