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Raman spectroscopy is employed to probe directly the soft rotation and tilting modes, which are two primary order parameters predicted in the hybrid improper ferroelectric material Ca$_3$Mn$_2$O$_7$. We observe a giant softening of the…

Strongly Correlated Electrons · Physics 2018-04-04 A. Glamazda , D. Wulferding , P. Lemmens , B. Gao , S. -W. Cheong , K. -Y. Choi

A detailed investigation using variable temperature powder neutron diffraction demonstrates that BiFeO3 undergoes a phase transition from the ferroelectric alpha phase (rhombohedral, R3c) to a paraelectric beta phase (orthorhombic, Pbnm)…

Materials Science · Physics 2009-08-21 Donna C. Arnold , Kevin S. Knight , Finlay D. Morrison , Philip Lightfoot

Single crystals of Ca(Fe1-xRux)2As2 (0<x<0.065) and Ca1-yLay(Fe0.973Ru0.027)2As2 (0<y<0.2) have been synthesized and studied with respect to their structural, electronic and magnetic properties. The partial substitution of Fe by Ru induces…

Strongly Correlated Electrons · Physics 2015-12-23 K. Zhao , C. Stingl , R. S. Manna , C. Q. Jin , P. Gegenwart

In this work, the potential to exploit Aurivillius higher order composition (n=6) given by Bi4Ti3O12-3BiFeO3 as single phase and high temperature magnetoelectric materials are well explored by elaborately studying the concerned structure…

Materials Science · Physics 2022-12-20 K. R. S. Preethi Meher , K. B. R. Varma

Ferroelectrics show a phase transition to a paraelectric phase at a well-defined transition temperature. Introducing disorder makes this transition diffuse, and the system becomes a relaxor. Since the degree of (dis-)order is usually…

We present a combined high-resolution x-ray diffraction and x-ray resonant magnetic scattering (XRMS) study of as-grown BaFe2As2. The structural/magnetic transitions must be described as a two-step process. At T_S = 134.5 K we observe the…

A sequence of structural transitions occurring in the quasi-one-dimensional (1D) 3d1 system BaVS3 at low temperature was investigated by high resolution synchrotron X-ray diffraction. The orthorhombic Cmc21 structure of the…

Strongly Correlated Electrons · Physics 2009-11-10 S. Fagot , P. Foury-Leylekian , S. Ravy , J. P. Pouget , M. Anne , G. Popov , M. V. Lobanov , M. Greenblatt

Lattice modulation and magnetic structures in magnetoelectric compounds Tb1-xDyxMnO3 have been studied around the ferroelectric (FE) Curie temperature T_C by x-ray and neutron diffraction. Temperature-independent modulation vectors through…

Strongly Correlated Electrons · Physics 2009-11-11 T. Arima , A. Tokunaga , T. Goto , H. Kimura , Y. Noda , Y. Tokura

Neutron scattering has been used to study the magnetic correlations and long wavelength spin dynamics of La1-xCaxMnO3 in the ferromagnetic regime (0<=x<1/2). For x=1/3 (Tc=250K) where the magnetoresistance effects are largest the system…

Condensed Matter · Physics 2009-10-28 J. W. Lynn , R. W. Erwin , J. A. Borchers , Q. Huang , A. Santoro , J-L. Peng , Z. Y. Li

Most transition-metal trihalides are dimorphic. The representative chromium-based triad, CrCl3, CrBr3, CrI3, is characterized by the low-temperature phase adopting the trigonal BiI3 type while the structure of the high-temperature phase is…

Pressure induced phase transitions of MIAgIIF3 perovskites where M = K, Rb, Cs, have been predicted theoretically for the first time for pressures up to 100 GPa. The sequence of phase transitions for M = K and Rb consists of an orthorhombic…

Materials Science · Physics 2022-04-01 Łukasz Wolański , Marvin Metzelaars , Jan van Leusen , Paul Kögerler , Wojciech Grochala

We report a structural phase transition found at Ts = 200 K in a pyrochlore oxide Cd2Re2O7 which shows superconductivity at Tc = 1.0 K. X-ray diffractionexperiments indicate that the phase transition is of the second order, from a…

Superconductivity · Physics 2009-11-07 M. Hanawa , J. Yamaura , Y. Muraoka , F. Sakai , Z. Hiroi

Although the structural phase transitions in single-crystal hybrid methyl-ammonium (MA) lead halide perovskites (MAPbX3, X = Cl, Br, I) are common phenomena, they have never been observed in the corresponding nanocrystals. Here we…

Applied Physics · Physics 2020-04-08 Yuri D. Glinka , Rui Cai , Xian Gao , Dan Wu , Rui Chen , Xiao Wei Sun

In order to better understand the reconstructive ferroelectric-paraelectric transition of Bi2WO6, which is unusual within the Aurivillius family of compounds, we performed first principles calculations of the dielectric and dynamical…

Materials Science · Physics 2015-06-04 Hania Djani , Eric Bousquet , Abdelhafid Kellou , Philippe Ghosez

The subtle interplay of randomness and quantum fluctuations at low temperatures gives rise to a plethora of unconventional phenomena in systems ranging from quantum magnets and correlated electron materials to ultracold atomic gases.…

Disordered Systems and Neural Networks · Physics 2014-01-15 L. Demko , S. Bordacs , T. Vojta , D. Nozadze , F. Hrahsheh , C. Svoboda , B. Dora , H. Yamada , M. Kawasaki , Y. Tokura , I. Kezsmarki

Detailed measurements of the magnetic and transport properties of the two La1-xCaxMnO3 (x = 0.18, x = 0.20) single crystals straddling the compositional metal-insulator transition boundary (0.18 < xc < 0.22) are summarized. The analysis of…

Strongly Correlated Electrons · Physics 2009-01-15 Wanjun Jiang , X. Z. Zhou , K. Glazyrin , Y. Mukovskii , Gwyn Williams

We report systematic studies of structural, microstructural and transport properties of Y1-xCaxBa2Cu3O7-d bulk samples with 0.20 x 0.0. The partial substitution of Ca2+ at Y3+ site in YBa2Cu3O7-d leads towards slightly overdoped regime,…

Superconductivity · Physics 2009-11-10 Rajiv Giri , H. K. Singh , O. N. Srivastava , V. P. S. Awana , Anurag Gupta , B. V. Kumaraswamy , H. Kishan

We report the observation of a phase transition in a KTaO$_3$ crystal, corresponding to a paraelectric-to-ferroelectric transition. The crystal was placed inside a copper cavity to form a dielectric-loaded microwave cavity, and the…

Materials Science · Physics 2025-07-23 Zijun C. Zhao , Jeremy F. Bourhill , Maxim Goryachev , Aleksey Sadekov , Michael E. Tobar

We report the discovery of structural phase transitions and superconductivity in the full Heusler compounds $X$Pd$_2$Sn ($X$ = Ti, Zr, Hf), by means of electrical transport, magnetic susceptibility, specific heat and x-ray diffraction…

Superconductivity · Physics 2023-03-07 Hang Su , Feng Du , Rui Li , Shuaishuai Luo , Yuxuan Chen , Jiyong Liu , Ye Chen , Chao Cao , Michael Smidman , Huiqiu Yuan

Lead-free (K0.48Na0.48Li0.04)(Nb1-xTax)O3 (KNLNT-x) ceramics were synthesized to study the effects of Li and Ta substitution on phase transition behavior, microstructure, and ferroelectric, dielectric, and piezoelectric properties. X-ray…