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A single crystal of lead-zirconate-titanate (PZT), composition Pb(Zr0.80Ti0.20)O3, was studied by polarized-Raman scattering as a function of temperature. Raman spectra reveal that the local structure deviates from the average structure in…

Materials Science · Physics 2015-06-23 J. Frantti , Y. Fujioka , A. Puretzky , Y. Xie , Z. -G. Ye , C. Parish , A. M. Glazer

We have recently predicted and subsequently verified experimentally by specific heat measurements that EuTiO3 undergoes a structural phase transition at elevated temperature TS = 282 K. The origin of the phase transition has been attributed…

Materials Science · Physics 2012-05-25 J. Köhler , R. Dinnebier , A. Bussmann-Holder

SrTiO$_{3}$, a quantum paraelectric, becomes a metal with a superconducting instability after removal of an extremely small number of oxygen atoms. It turns into a ferroelectric upon substitution of a tiny fraction of strontium atoms with…

The temperature-dependent phase transitions in Ruddlesden-Popper oxides with perovskite bilayers have been under increased scrutiny in recent years due to the so-called hybrid improper ferroelectricity that some chemical compositions…

Materials Science · Physics 2021-12-08 Gabriel Clarke , Dominik Daisenberger , X. Luo , S. W. Cheong , Nicholas C. Bristowe , Mark S. Senn

Ferroelectricity in hafnia is often regarded as a breakthrough discovery in ferroelectrics, potentially able to revolutionize the whole field. Despite increasing interests, a comprehensive understanding of the many factors driving the…

Materials Science · Physics 2021-06-16 Francesco Delodovici , Paolo Barone , Silvia Picozzi

The precise crystal structure of La3Ni2O7 in its high-pressure superconducting state has been a subject of intense debate, with proposed models including both orthorhombic and tetragonal symmetries. Using high-pressure Raman spectroscopy…

Superconductivity · Physics 2025-11-20 Hengyuan Zhang , Jielong Zhang , Mengwu Huo , Junfeng Chen , Deyuan Hu , Dao-Xin Yao , Hualei Sun , Kun Cao , Meng Wang

We have carried out the powder x-ray diffraction and dielectric studies on multiferroic particulate composite xNi0.9Zn0.1Fe2O4/(1-x)PbZr0.52Ti0.48O3 with x=0.15, 0.30, 0.45, 0.60, 0.75 and 0.90 to explore the structural and ferroelectric…

Materials Science · Physics 2014-02-20 Rishikesh Pandey , Braj Raj Meena , Akhilesh Kumar Singh

We have conducted a detailed high-pressure (HP) investigation on $Eu-$doped $BaTiO_3$ using angle-resolved x-ray diffraction, Raman spectroscopy, dielectric permittivity and dc resistance measurements. The x-ray diffraction data analysis…

Materials Science · Physics 2023-04-04 Mrinmay Sahu , Bishnupada Ghosh , Bobby Joseph , Goutam Dev Mukherjee

SrTiO$_{3}$ undergoes a cubic-to-tetragonal phase transition at 105K. This antiferrodistortive transition is believed to be in competition with incipient ferroelectricity. Substituting strontium by isovalent calcium induces a ferroelectric…

We have studied the phase diagram of La$_{1-x}$Ca$_{x}$MnO$_{3}$ for $0.5\leq x\leq 0.9$ using neutron powder diffraction and magnetization measurements. At 300 K all samples are paramagnetic and single phase with crystallographic symmetry…

Strongly Correlated Electrons · Physics 2009-11-07 M. Pissas , G. Kallias

Despite their structural similarities, SrBi$_2$Ta$_2$O$_9$ (SBT) and SrBi$_2$Nb$_2$O$_9$ (SBN) undergo a different sequence of phase transitions. The phase diagram of SBT as a function of the temperature includes an intermediate phase…

Materials Science · Physics 2015-05-13 Urko Petralanda , I. Etxebarria

Lithium doped sodium niobate is an ecofriendly piezoelectric material that exhibits a variety of structural phase transitions with composition and temperature. We have investigated the phase stabilities of an important composition…

We present local structural evidence supporting the presence of charge inhomogeneities in the CuO2 planes of underdoped La2-xSrxCuO4. High-resolution atomic pair distribution functions have been obtained from neutron powder diffraction data…

Superconductivity · Physics 2016-08-31 E. S. Bozin , G. H. Kwei , H. Takagi , S. J. L. Billinge

Understanding the polarization switching mechanisms at play in ferroelectric materials is crucial for their exploitation in electronic devices. The conventional centrosymmetric reference structure-based mechanism which accounts for…

Theoretical {\em ab initio} and experimental methods were used to investigate the $x$Bi(Zn,Ti)O$_3$-(1-$x$)PbTiO$_3$ (BZT-PT) solid solution. We find that hybridization between Zn 4$p$ and O 2$p$ orbitals allows the formation of short,…

The structural phase transformations of 0.7Pb(Mg1/3Nb2/3)O3-0.3PbTiO3 (PMN-30%PT) have been studied using x-ray diffraction (XRD) and neutron scattering as a function of temperature and electric field. We observe the phase transformational…

Materials Science · Physics 2009-11-10 Feiming Bai , Naigang Wang , Jiefang Li , D. Viehland , P. M. Gehring , Guangyong Xu , G. Shirane

Structural, electronic and magnetic properties of polycrystalline La2-xCaxCoMnO6 (0 $\leq$ x $\leq$ 0.75) compounds are investigated by x-ray diffraction and magnetometry. All the samples have an orthorhombic structure and show a slight…

Materials Science · Physics 2022-05-11 J. R. Jesus , L. Bufaiçal , E. M. Bittar

Bilayer antiferromagnets CrX$_{3}$ (X $=$ Cl, Br, and I) are promising materials for spintronics and optoelectronics that are rooted in their peculiar electronic structures. However, their bands are often hybridized from the interlayer…

Optics · Physics 2024-02-20 Y. Q. Liu , M. S. Si , G. P. Zhang

Quantum paraelectrics are materials in which a long-range ferroelectric/antiferroelectric order is suppressed by quantum fluctuations, i.e. zero-point motion of the lattice prevents condensation of the soft polar phonon mode even at T = 0…

Strongly Correlated Electrons · Physics 2019-08-06 Ivica M. Bradarić , Feodor V. Kusmartsev

Oxide heterointerfaces constitute a rich platform for realizing novel functionalities in condensed matter. A key aspect is the strong link between structural and electronic properties, which can be modified by interfacing materials with…

Materials Science · Physics 2021-07-09 T. C. van Thiel , J. Fowlie , C. Autieri , N. Manca , M. Šiškins , D. Afanasiev , S. Gariglio , A. D. Caviglia