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In hybrid improper ferroelectric systems, polarization arises from the onset of successive nonpolar lattice modes. In this work, measurements and modeling were performed to determine the spatial symmetries of the phases involved in the…

Materials Science · Physics 2019-07-03 S. Liu , H. Zhang , S. Ghose , M. Balasubramanian , Zhenxian Liu , S. G. Wang , Y-S. Chen , B. Gao , J. Kim , S. -W. Cheong , T. A. Tyson

Standing on successful first principles predictions for new functional ferroelectric materials, a number of new ferroelectrics have been experimentally discovered. Utilizing trilinear coupling of two types of octahedron rotations, hybrid…

Materials Science · Physics 2015-01-27 Yoon Seok Oh , Xuan Luo , Fei-Ting Huang , Yazhong Wang , Sang-Wook Cheong

Hybrid improper ferroelectricity, where an electrical polarization can be induced via a trilinear coupling to two non-polar structural distortions of different symmetry, has recently been experimentally demonstrated for the first time in…

Materials Science · Physics 2016-10-05 Elizabeth A. Nowadnick , Craig J. Fennie

We report a detailed high-resolution powder neutron diffraction investigation of the structural behaviour of the multiferroic hexagonal polymorph of YMnO3 between room temperature and 1403 K. The study was aimed at resolving previous…

Materials Science · Physics 2015-05-19 Alexandra S. Gibbs , Kevin S. Knight , Philip Lightfoot

We have investigated the influence of Ca ions substitution on the structural and superconducting properties of (Nd1-xCax)(Ba1.6La0.4)Cu3Oz system. Magnetization, X-ray diffraction and neutron diffraction studies have been carried out on a…

Superconductivity · Physics 2010-05-14 Amish G. Joshi , R. G. Kulkarni , W. B. Yelon , Ram Prasad , M. R. Gonal

We report direct experimental evidence of antiferroelectric to paraelectric phase transition under pressure in NaNbO3 using neutron diffraction at room temperature. The paraelectric phase is found to stabilize above 8 GPa and its crystal…

Materials Science · Physics 2015-06-11 S. K. Mishra , M. K. Gupta , R. Mittal , S. L. Chaplot , Thomas Hansen

We report the phase diagram of (Ba1-xCax)(Zr0.1Ti0.9)O3 solid solution. It is found that substitution of smaller Ca ions for Ba ions can slightly increase the cubic-tetragonal(T) para-ferroelectric phase transition temperature and strongly…

Materials Science · Physics 2013-10-08 Desheng Fu , Yuto Kamai , Naonori Sakamoto , Naoki Wakiya , Hisao Suzuki , Mitsuru Itoh

Ca$_3$Ti$_2$O$_7$ is an experimentally confirmed hybrid improper ferroelectric material, in which the electric polarization is induced by a combination of the coherent TiO$_6$ octahedral rotation and tilting. In this work, we investigate…

Materials Science · Physics 2018-07-03 C. F. Li , S. H. Zheng , H. W. Wang , J. J. Gong , X. Li , Y. Zhang , K. L. Yang , L. Lin , Z. B. Yan , Shuai Dong , J. -M. Liu

A neutron scattering study of nonsuperconducting La$_{2-x}$Sr$_x$CaCu$_2$O$_6$ (x=0 and 0.2), a bilayer copper oxide without CuO chains, has revealed an unexpected tetragonal-to-orthorhombic transition with a doping dependent transition…

Superconductivity · Physics 2009-11-07 C. Ulrich , S. Kondo , M. Reehuis , H. He , C. Bernhard , C. Niedermayer , F. Bouree , P. Bourges , M. Ohl , H. M. Ronnow , H. Takagi , B. Keimer

Bulk superconductor samples of YBa2Cu3-xCoxO7-{\delta} with x = 0, 0.01, 0.03, 0.05 are synthesized by solid-state reaction route. Both x-ray diffraction and electron microscopy have been employed to study the phase identification,…

Superconductivity · Physics 2011-07-07 Sushant Gupta , R. S. Yadav , N. P. Lalla , G. D. Verma , B. Das

Perturbed angular correlation spectroscopy combined with $ab-initio$ electronic structure calculations is used to unravel the structural phase transition path from the low-temperature polar structure to the high-temperature structural phase…

We report a high resolution neutron diffraction investigation of the coupling of structural and magnetic transitions in Ba1xKxFe2As2. The tetragonal-orthorhombic and antiferromagnetic transitions are suppressed with potassium-doping,…

In this work we have investigated the orthorhombic to tetragonal phase transition in the Ba2Cu3O4Cl2 compound. This transition was observed by X-ray powder diffractometry carried out in samples heat treated between 700 and 750OC and also in…

Materials Science · Physics 2007-05-23 M. S. da Luz , C. A. M. dos Santos , B. Ferreira , A. J. S. Machado

The phase diagram of Sr_1-xEu_xTiO_3 is determined experimentally by electron paramagnetic resonance and resistivity measurements and analyzed theoretically within the self-consistent phonon approximation as a function of x ([0.03-1.0]).…

Materials Science · Physics 2013-01-28 Z. Guguchia , A. Shengelaya , H. Keller , J. Köhler , A. Bussmann-Holder

The structural phase diagram of the La1-xSrxMnO3 system in the compositional range 0.08 <= x <= 0.125 has been investigated by high-resolution synchrotron x-ray powder diffraction techniques between 20-600 K. Recent studies have reported…

Strongly Correlated Electrons · Physics 2009-10-31 D. E. Cox , T. Iglesias , E. Moshopoulou , K. Hirota , K. Takahashi , Y. Endoh

We present here the results of frequency dependent dielectric, polarization and powder X-ray powder diffraction studies in the 300 to 100K temperature range for Ba_0.55Sr_0.45TiO_3. The dielectric results indicate a succession of three…

Materials Science · Physics 2007-09-24 Satyendra Singh , Satendra Pal Singh , Dhananjai Pandey

The structural, dielectric and ferroelectric properties of lead-free (Na0.5-xKxBi0.5-xLax)TiO3 powders synthesized by sol-gel self-combustion method were investigated. Rietveld refinement of Synchrotron x-ray diffraction data confirms pure…

In scientific research, both positive and negative results play crucial role in advancing the field. Negative results provide valuable insights that can guide future experiments and prevent repeated failures. Here we present our growth…

Materials Science · Physics 2025-02-25 R. Choudhary , A. Rajapitamahuni , S. Guo , Qi. Jiang , J. -H. Chu , K. A. Mkhoyan , B. Jalan

The normal ferroelectric to paraelectric phase transition in model ferroelectric materials such as BaTiO3 is typically characterized by a sharp, well-defined dielectric constant peak at a specific transition temperature. However, under…

Materials Science · Physics 2025-10-17 Prithwiraj Ganguly , Prashant Joshi , Maneesha Puthiyoth , Dilip Sasmal , Somaditya Sen

We investigate the microstructural evolution in a ferroelectric to antiferroelectric phase transition at the morphotropic phase boundary in the Bi(1-x)SmxFeO3 system. Continuous Sm3+ substitution on the A-site induces short-range…

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