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We show that the neutron diffuse scattering in relaxor ferroelectric (1-x)PbZn$_{1/3}$Nb$_{2/3}$O$_{3}$ - x PbTiO$_{3}$ (x=0.07) consists of two components. The first component is strictly elastic but extended in q-space and grows below 600…

Materials Science · Physics 2019-08-12 G. -M. Rotaru , S. N. Gvasaliya , B. Roessli , S. Kojima , S. G. Lushnikov , P. Günter

Ionic-pair equal-time displacement correlations in relaxor lead magnesium niobate, $Pb(Mg_{1/3}Nb_{2/3})O_{3}$, have been investigated at room temperature in terms of an x-ray diffuse scattering technique. Functions of the distinct…

Materials Science · Physics 2009-10-31 Naohisa Takesue , Yasuhiko Fujii , Hoydoo You

Numerous authors have referred to room-temperature magnetic switching of large electric polarizations as The Holy Grail of magnetoelectricity.We report this long-sought effect using a new physical process of coupling between magnetic and…

Materials Science · Physics 2009-02-24 Ashok Kumar , G. L. Sharma , R. S. Katiyar R. Pirc , R. Blinc J. F. Scott

The low-energy part of the vibration spectrum in PbMg$_{1/3}$Nb$_{2/3}$O$_3$ (PMN) relaxor ferroelectric has been studied by neutron scattering above and below the Burns temperature, T$_d$. The transverse acoustic and the lowest transverse…

Materials Science · Physics 2007-05-23 S N Gvasaliya , B Roessli , R A Cowley , P Hubert , S G Lushnikov

Relaxor ferroelectrics are a class of materials that are widely perceived as deriving their exotic properties from structural heterogeneities. Understanding the microscopic origin of the superior electromechanical response requires…

Temperature dependent studies of the 1/2(hk0) superlattice reflections \alpha spots by synchrotron x-ray scattering measurements were performed in (PMN) and (PMN-xPT) with Ti doping x<0.32 single crystals. Separation of the \alpha spots…

Materials Science · Physics 2009-11-10 A. Tkachuk , Haydn Chen

The stability of the disordered glassy phase in the relaxors PbMg1/3Nb2/3O3 and (PbMg1/3Nb2/3O3)0.88(PbTiO3)0.12, called PMN and PMN-PT, was investigated by preparing partially polarized samples and allowing them to age at zero field in the…

Materials Science · Physics 2009-11-13 Eugene V. Colla , Derek Vigil , John Timmerwilke , M. B. Weissman , D. D. Viehland , Brahim Dkhil

The dynamical behavior of field-induced ferroelectric phase transitions in compositions of PbMg1/3Nb2/3O3(1-x)-PbTiO3(x) (PMN-PT) near the morphotropic phase boundary (MPB) was investigated using several electric-field application…

Materials Science · Physics 2026-04-07 Shivjeet Chanan , Joseph Kerchenfaut , Eduard Illin , Eugene V. Colla

Using neutron pair distribution function (PDF) analysis over the temperature range from 1000 K to 15 K, we demonstrate the existence of local polarization and the formation of medium-range, polar nanoregions (PNRs) with local rhombohedral…

Disordered Systems and Neural Networks · Physics 2009-11-10 I. -K. Jeong , T. W. Darling , J. K. Lee , Th. Proffen , R. H. Heffner , J. S. Park , K. S. Hong , W. Dmowski , T. Egami

We have investigated the magnetic ground-state of the multiferroic relaxor ferroelectric \pfn with $\mu$SR spectroscopy and neutron scattering. We find that a transition to a partially disordered phase occurs below T=20 K that coexists with…

Materials Science · Physics 2009-09-13 G. -M. Rotaru , B. Roessli , A. Amato , S. N. Gvasaliya , C. Mudry , S. G. Lushnikov , T. A. Shaplygina

Structural phase transformations of [110] electric field cooled Pb(Mg1/3Nb2/3)O3-30%PbTiO3 (PMN-30%PT) crystals have been performed by x-ray diffraction in a field-cooled (FC) condition. A phase sequence of…

Materials Science · Physics 2009-11-11 Hu Cao , Feiming Bai , Naigang Wang , Jiefang Li , D. Viehland , Guangyong Xu , Gen Shirane

Neutron inelastic scattering measurements of the polar TO phonon mode in the cubic relaxor Pb(Mg1/3Nb2/3)O3, at room temperature, reveal anomalous behavior similar to that recently observed in the Pb(Zn1/3Nb2/3)_{0.92}Ti_{0.08}O3 system in…

Materials Science · Physics 2009-10-31 P. M. Gehring , S. B. Vakhrushev , G. Shirane

We report a neutron scattering study of a ferroelectric phase transition in Sr$_{0.61}$Ba$_{0.39}$Nb$_2$O$_6$ (SBN-61). The ferroelectric polarization is along the crystallographic $c$-axis but the transverse acoustic branch propagating…

Materials Science · Physics 2014-02-10 S. N. Gvasaliya , R. A. Cowley , L. I. Ivleva , S. G. Lushnikov , B. Roessli , A. Zheludev

The relaxor ferroelectric PbMg1/Nb2/3O3 was investigated by means of broad-band dielectric and Fourier Transform Infrared (FTIR) transmission spectroscopy in the frequency range from 1 MHz to 15 THz at temperatures between 20 and 900 K…

Materials Science · Physics 2009-11-10 S. Kamba , M. Kempa , V. Bovtun , J. Petzelt , K. Brinkman , N. Setter

The relaxor ferroelectric (PbMn$_{1/3}$Nb$_{2/3}$O$_3$)$_{1-x}$(PbTiO$_3$)$_{x}$, $x=0.1$, (PMN/PT(90/10)) is found to exhibit several regimes of complicated aging behavior. Just below the susceptibility peak there is a regime exhibiting…

Materials Science · Physics 2009-11-11 Lambert K. Chao , Eugene V. Colla , M. B. Weissman

<001> oriented 0.7Pb(Mg1/3Nb2/3)O3-0.3PbTiO3 single crystals were poled under different electric fields, i.e. Epoling=4 kV/cm and Epoling=13 kV/cm. In addition to the temperature-dependent dielectric constant measurement, X-ray diffraction…

Materials Science · Physics 2009-11-07 Ke-Pi Chen , Xiao-Wen Zhang , Hao-Su Luo

A first-principles-based model is developed to investigate the influence of lead vacancies on the properties of relaxor ferroelectric Pb(Sc1/2Nb1/2)O3 (PSN). Lead vacancies generate large, inhomogeneous, electric fields that reduce barriers…

Materials Science · Physics 2009-11-11 L. Bellaiche , Jorge Iniguez , Eric Cockayne , B. P. Burton

We present a quantitative analysis of the phonon lineshapes obtained by neutron inelastic scattering methods in the relaxor ferroelectric Pb(Mg1/3Nb2/3)O3 (PMN). Differences in the shapes and apparent positions of the transverse acoustic…

Materials Science · Physics 2009-11-07 S. Wakimoto , C. Stock , Z. -G. Ye , W. Chen , P. M. Gehring , G. Shirane

Taking into account the long-ranged spin interactions due to weak localization effects in disordered itinerant ferromagnets the scattering of both electrons and neutrons on critical spin fluctuations near quantum phase transition is…

Disordered Systems and Neural Networks · Physics 2015-06-25 Y. N. Skryabin , A. V. Chukin

High-energy x-ray diffraction experiments peformed on rhombohedral (1-x)Pb(Zn1/3Nb2/3)O3-xPbTiO3(PZN-xPT) crystals with x= 4.5 and 8% show that an electric field applied along the [001] direction induces the tetragonal phase, as proposed by…

Materials Science · Physics 2009-11-07 B. Noheda , Z. Zhong , D. E. Cox , G. Shirane , S-E. Park , P. Rehring