Related papers: Synthesis of ultrafast waveforms using coherent Ra…
We measure the time-energy correlation of broadband, spontaneously generated four wave mixing (FWM), and demonstrate novel time-frequency coupling effects; specifically, we observe a power-dependent splitting of the correlation in both…
Octave-spanning, 12.5 fs, (1.9 cycle) pulses with 115 {\mu}J energy in the short-wavelength mid-infrared spectral range (1-2.5 {\mu}m) have been generated via phase-mismatched cascaded nonlinear frequency conversion using organic DAST…
Optical waveguides made from periodically poled materials provide high confinement of light and enable the generation of new wavelengths via quasi-phase-matching, making them a key platform for nonlinear optics and photonics. However, such…
We discuss a novel method for generating octave-spanning supercontinua and few-cycle pulses in the important mid-IR wavelength range. The technique relies on strongly phase-mismatched cascaded second-harmonic generation (SHG) in mid-IR…
Collinear phase-matched optical rectification is studied in ZnGeP$_{2}$ pumped with near-infrared light. The pump-intensity dependence is presented for three crystal lengths (0.3, 1.0 and 3.0 mm) to determine the effects of linear optical…
We observe an optical filtering effect in four-wave mixing (FWM) process based on a cold atomic gas. The side peaks appear at the edges of pulse of generated optical field, and they propagate through the atomic media without absorption. The…
We report on single electronic spins coupled to the motion of mechanical resonators by a novel mechanism based on crystal strain. Our device consists of single-crystalline diamond cantilevers with embedded Nitrogen-Vacancy center spins.…
We present a numerical parametric study of single-cycle electromagnetic pulse generation in a DAST/SiO2 multilayer structure via collinear optical rectification of 800 nm femtosecond laser pulses. It is shown that modifications of the…
Excited-state vibrational dynamics in molecules can be studied by an electronically off-resonant Raman process induced by a probe pulse with variable delay with respect to an actinic pulse. We establish the connection between several…
Time-domain analysis of harmonic fields with sub-cycle resolution is now experimentally viable due to the emergence of sensitive, on-chip techniques for petahertz-scale optical-field sampling. We demonstrate how such a time-domain,…
We present a general and versatile technique of population transfer based on {\it parallel adiabatic passage} by femtosecond shaped pulses. Their amplitude and phase are specifically designed to optimize the adiabatic passage corresponding…
Diamond has superlative material properties for a broad range of quantum and electronic technologies. However, heteroepitaxial growth of single crystal diamond remains limited, impeding integration and evolution of diamond-based…
Phase-coherent pulsed driving of passive optical fiber resonators enable the generation of ultrashort dissipative Raman solitons with durations well below 100~fs. The existence and characteristics of such solitons critically depends on the…
We present two methods for efficient detection of chiral molecules based on sequences of single pulses and Raman pulse pairs. The chiral molecules are modelled by a closed-loop three-state system with different signs in one of the couplings…
We report measurements of phase-matched nonlinear x-ray and optical sum-frequency generation from single-crystal silicon using sub-resonant 0.95 eV laser pulses and 9.5 keV hard x-ray pulses from the LCLS free-electron laser. The…
I present a detailed derivation of wideband optical pulses interacting with a Raman transition in the kind of scheme currently used to generate the ultra broadband light fields needed to create ultrashort pulses. In contrast to the usual…
Ultrashort laser pulses enable attosecond-scale measurements and drive breakthroughs across science and technology, but their routine use hinges on reliable pulse characterization. Frequency-Resolved Optical Gating (FROG) is a leading…
We study high order harmonics generation (HHG) in crystalline silicon and diamond subjected to near and mid-infrared laser pulses. We employ time-dependent density functional theory and solve the time-dependent Kohn-Sham equation in the…
We generate mode-locked picosecond pulses near 1110 nm by spectrally slicing and reamplifying an octave-spanning supercontinuum source pumped at 1550 nm. The 1110 nm pulses are near transform-limited, with 1.7 ps duration over their 1.2 nm…
Atom interferometric sensors and quantum information processors must maintain coherence while the evolving quantum wavefunction is split, transformed and recombined, but suffer from experimental inhomogeneities and uncertainties in the…