Related papers: Synthesis of ultrafast waveforms using coherent Ra…
In this Letter, we report phase-matched four-wave mixing separated by over one-octave in a dispersion engineered crystalline microresonator. Experimental and numerical results presented here confirm that primary sidebands were generated…
Excitation of four coherent phonon modes of different symmetries has been realized in copper metaborate CuB$_2$O$_4$ via impulsive stimulated Raman scattering (ISRS). Phonons were detected by monitoring changes in the linear optical…
The time-frequency degree of freedom is a powerful resource for implementing high-dimensional quantum information processing. In particular, field-orthogonal pulsed temporal modes offer a flexible framework compatible with both…
High-harmonic spectroscopy has become an essential ingredient in probing various ultrafast electronic processes in solids with sub-cycle temporal resolution. Despite its immense importance, sensitivity of high-harmonic spectroscopy to…
We demonstrate the acquisition of stimulated Raman scattering spectra with the use of a single femtosecond pulse. High resolution vibrational spectra are obtained by shifting the phase of a narrow band of frequencies in the broadband input…
Coherent Raman scattering techniques as coherent anti-Stokes Raman scattering (CARS), offer significant advantages in terms of pixel dwell times and speed as compared to spontaneous Raman scattering for investigations of crystalline…
X-ray free-electron lasers (XFELs) of high brightness have opened new opportunities for exploring ultrafast dynamical processes in matter, enabling imaging and movies of single molecules and particles at atomic resolution. In this paper, we…
Coherent nonlinear spectroscopies and imaging in the X-ray domain provide direct insight into the coupled motions of electrons and nuclei with resolution on the electronic length and time scale. The experimental realization of such…
We propose a scheme to dynamically generate optical flux lattices with nontrivial band topology using amplitude-modulated Raman lasers and radio-frequency (rf) magnetic fields. By tuning the strength of Raman and rf fields, three distinct…
In a recent experiment [1], it was observed that a sequence of two standing wave square pulses can split a BEC at rest into +/- 2 h_bar k diffraction orders with almost 100% efficiency. By truncating the Raman-Nath equations to a 2-state…
The synthesis of ultrasmall (2-5 nm) nanodiamonds purely from adamantane at pressure of 12 GPa is reported. Their structural features have been studied by Raman spectroscopy. The unusual vibration band containing a number of pronounced…
We construct a phase-conjugate resonator which passively produces stable pulses that alternate between the probe and the conjugate colors. The requisite phase-conjugate mirror inside the resonator is constructed using non-degenerate…
Recently developed techniques for generating precisely equidistant optical frequencies over broad wavelength ranges are revolutionizing precision physical measurement [1-3]. These frequency "combs" are produced primarily using relatively…
We report the generation of a multi-octave supercontinuum spanning from 350 nm to 1700 nm with exceptional spectral flatness and high conversion efficiency to both the visible and near infrared region, by pumping a methane-filled…
We demonstrate a light-pulse atom interferometer based on the diffraction of free-falling atoms by a picosecond frequency-comb laser. More specifically, we coherently split and recombine wave packets of cold $^{87}$Rb atoms by driving…
We introduce an atomic gravimetric sequence using Raman-type composite light pulses that excites a superposition of two momentum states with the same internal level. The scheme allows the suppression of common noise, making it less…
We report on the first experimental demonstration of widely-tunable parametric sideband generation in a Kerr microresonator. Specifically, by pumping a silica microsphere in the normal dispersion regime, we achieve the generation of…
We theoretically investigate the generation of higher harmonics and the construction of a single attosecond pulse by means of two oppositely polarized sinc-shaped driver pulses. In comparison to a few-cycle Gaussian pulse of the same…
An efficient broadband sum frequency generation (SFG) technique using the two collinear optical parametric processes \omega 3=\omega 1+\omega 2 and \omega 4=\omega 1+\omega 3 is proposed. The technique uses chirped quasi-phase-matched…
We demonstrate a simple method to obtain accurate optical waveforms with a GHz-level programmable modulation bandwidth and Watt-level output power for wideband optical control of free atoms and molecules. Arbitrary amplitude and phase…