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For decades, most research on high harmonic generation (HHG) considered matter as quantum but light as classical, leaving the quantum-optical nature of the harmonics an open question. Here we explore the quantum properties of high…

Quantum Physics · Physics 2023-11-21 Matan Even Tzur , Michael Birk , Alexey Gorlach , Ido Kaminer , Michael Krueger , Oren Cohen

The order of high harmonics emitted by an atom in an intense laser field is limited by the so-called cutoff frequency. Solving the time-dependent Schr\"odinger equation, we show that this frequency can be increased considerably by a…

Atomic Physics · Physics 2016-09-08 Carla Figueira de Morisson Faria , Jan-Michael Rost

We theoretically study the high-harmonic generation (HHG) in one-dimensional spin systems. While in electronic systems the driving by AC electric fields produces radiation from the dynamics of excited charges, we consider here the situation…

Strongly Correlated Electrons · Physics 2019-05-24 Shintaro Takayoshi , Yuta Murakami , Philipp Werner

A second plateau in the harmonic spectra of laser-driven two-electron atoms is observed both in the numerical solution of a low-dimensional model helium atom and using an extended strong field approximation. It is shown that the harmonics…

Atomic Physics · Physics 2009-11-13 P. Koval , F. Wilken , D. Bauer , C. H. Keitel

When a laser pulse impinges on a molecule which is invariant under certain symmetry operations selection rules for harmonic generation (HG) arise. In other words: symmetry controls which channels are open for the deposition and emission of…

Atomic Physics · Physics 2009-11-07 D. Bauer , F. Ceccherini

By deriving the 3/2 dimensional Hamiltonian equations for electrons in the intense laser radiation and quasi-static transverse electric and longitudinal magnetic fields, the electron heating mechanisms are examined both for low harmonic…

Plasma Physics · Physics 2019-07-24 Yanzeng Zhang , Sergei Krasheninnikov

High harmonic generation (HHG) from semiconductors and insulators has become a very active area of research due to its great potential for developing compact HHG devices. Here we show that by growing monolayers (ML) of insulators on…

Atomic Physics · Physics 2016-12-28 Néstor F. Aguirre , Fernando Martín

Harmonic generation is a general characteristic of driven nonlinear systems, and serves as an efficient tool for investigating the fundamental principles that govern the ultrafast nonlinear dynamics. In atomic gases, high-harmonic radiation…

The combination of high-order harmonic generation (HHG) with resonant XUV excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process is investigated theoretically. In this setup, the…

Atomic Physics · Physics 2023-01-10 Christian Buth , Markus C. Kohler , Joachim Ullrich , Christoph H. Keitel

We present a comprehensive theoretical investigation of high-order harmonic generation in H$_2^+$ molecular ions within a quantum optical framework. Our study focuses on characterizing various quantum optical and quantum information…

High-order harmonic generation (HHG) enables the up-conversion of intense infrared or visible femtosecond laser pulses into extreme-ultraviolet attosecond pulses. However, the highly nonlinear nature of the process results in low conversion…

We study high order harmonics generation (HHG) in crystalline silicon and diamond subjected to near and mid-infrared laser pulses. We employ time-dependent density functional theory and solve the time-dependent Kohn-Sham equation in the…

Materials Science · Physics 2022-08-31 David Freeman , Shunsuke Yamada , Atsushi Yamada , Kazuhiro Yabana , Anatoli Kheifets

We present theoretical studies of high-order harmonic generation (HHG) driven by plasmonic fields in two-electron atomic systems. Comparing the two-active electron and single-active electron approximation models of the negative hydrogen ion…

Atomic Physics · Physics 2016-11-03 A. Chacón , M. F. Ciappina , M. Lewenstein

The atomic response to an ultra-intense driving field produces a characteristic high-harmonic spectrum featuring a rapid drop in intensity for the lower harmonics, followed by a plateau and a sharp cutoff. This response vanishes for…

Quantum Physics · Physics 2026-01-06 Lidija Petrovic , Philipp Stammer , Maciej Lewenstein , Javier Rivera-Dean

At the core of attosecond science lies the ability to generate laser pulses of sub-femtosecond duration. In tabletop devices the process relies on high-harmonic generation, where a major challenge is to obtain high yields and high cutoff…

Atomic Physics · Physics 2014-11-05 J. Solanpää , J. A. Budagosky , N. I. Shvetsov-Shilovski , A. Castro , A. Rubio , E. Räsänen

High-order harmonic generation in multiphoton ionization regime is studied theoretically to examine the resonant effects of the generating particle. We solve the time-dependent Schr\"odinger equation for In+ in the laser field by expanding…

Atomic Physics · Physics 2023-12-12 Alexander I. Magunov , Vasily V. Strelkov

High harmonic generation (HHG) in solids has emerged as a powerful spectroscopic method for resolving ultrafast electron dynamics and band structure properties across a wide range of materials. However, quantitative HHG studies require…

Optics · Physics 2025-12-16 S. Mandal , P. Kumar , Z. Pi , H. Y. Kim , M. Zhan , E. Goulielmakis

Together with one of its variants, the recently proposed phase-merging enhanced harmonic generation (PEHG) free-electron lasers (FELs) have been systematically studied in this paper. Different form the standard-HGHG, a transverse gradient…

Accelerator Physics · Physics 2015-06-18 Chao Feng , Haixiao Deng , Dong Wang , Zhentang Zhao

We theoretically investigate high-order harmonic generation (HHG) and its ellipticity in gapped graphene, driven by a femtosecond short-pulse laser at various orientation angles, employing the two-band density-matrix equations within the…

Atomic Physics · Physics 2025-05-21 Xinru Song , Xiaoyu Bu , Xiaohui Zhao , Rongxiang Zhang , Shang Wang , Fulong Dong

High-order harmonic generation via single-slit diffraction of relativistic laser pulses is investigated. Using fully kinetic 2D and 3D particle-in-cell simulations, we show that interesting optical phenomena emerge, including the generation…

Plasma Physics · Physics 2025-05-07 Longqing Yi
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