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Quantum magnets based on honeycomb lattices with low-coordination number offer a viable ground to realize exotic emergent quantum excitations and phenomena arising from the interplay between competing magnetic interactions, spin…

Strongly Correlated Electrons · Physics 2024-11-14 J. Khatua , M. Gomilsek , Kwang-Yong Choi , P. Khuntia

In NaNiO2, Ni3+ ions form a quasi two dimensional triangular lattice of S = 1=2 spins. The magnetic order observed below 20K has been described as an A type antiferromagnet with ferro- magnetic layers weakly coupled antiferromagnetically.…

Strongly Correlated Electrons · Physics 2009-11-11 Sophie De Brion , C. Darie , M. Hopzapfel , D. Talbayev , L. Mihaly , F. Simon , A. Janossy , G. Chouteau

We report the development of a continuous-wave and pulsed X-band electron spin resonance (ESR) spectrometer for the study of spins on ordered surfaces down to cryogenic temperatures. The spectrometer operates in ultra-high vacuum and…

The static and dynamic magnetic properties of an $S=1/2$ stacked triangular antiferromagnet RbCuCl$_{3}$ with a helical spin structure due to lattice distortion were investigated by susceptibility, high-field magnetization process and ESR…

Strongly Correlated Electrons · Physics 2009-10-31 S. Maruyama , H. Tanaka , Y. Narumi , K. Kindo , H. Nojiri , M. Motokawa , K. Nagata

The electron spin resonance spectrum of a quasi 1D S=1/2 antiferromagnet K2CuSO4Br2 was found to demonstrate an energy gap and a doublet of resonance lines in a wide temperature range between the Curie--Weiss and Ne\`{e}l temperatures. This…

Strongly Correlated Electrons · Physics 2015-10-28 A. I. Smirnov , T. A. Soldatov , K. Yu. Povarov , M. Hälg , W. E. A. Lorenz , A. Zheludev

Multi-frequency electron spin resonance (ESR) transmission spectra have been measured as function of temperature and magnetic field on single crystals of the quasi-one-dimensional spin-1 chain compound SrNi2V2O8 in the GHz frequency range.…

Strongly Correlated Electrons · Physics 2013-03-18 Zhe Wang , M. Schmidt , A. K. Bera , A. T. M. N. Islam , B. Lake , A. Loidl , J. Deisenhofer

We used electron spin resonance (ESR) combined with scanning tunneling microscopy (STM) to measure hydrogenated Ti (spin-1/2) atoms at low-symmetry binding sites on MgO in vector magnetic fields. We found strongly anisotropic g-values in…

The synthesis and characterization of a new Yb-based material Ba3Yb2Zn5O11 are reported. This material is identified as the first model system of a pseudospin-1/2 quantum antiferromagnet on "breathing" pyrochlore lattice characterized by an…

Strongly Correlated Electrons · Physics 2014-09-02 K. Kimura , S. Nakatsuji , T. Kimura

We report Eu L3-edge resonant inelastic x-ray scattering (RIXS) investigation of the electronic structure of EuB6. We observe that the RIXS spectral weight around 1.1 eV increases dramatically when the system is cooled below the…

Strongly Correlated Electrons · Physics 2011-07-07 Jungho Kim , Wei Ku , Chi-Cheng Lee , D. S. Ellis , B. K. Cho , A. H. Said , Yu. Shvyd'ko , Young-June Kim

We report experimental verification of the recently predicted collective modes of spinons, stabilized by backscattering interaction, in a model quantum spin chain material. We exploit the unique geometry of uniform Dzyaloshinskii-Moriya…

Strongly Correlated Electrons · Physics 2022-05-09 Kirill Yu. Povarov , Timofei A. Soldatov , Ren-Bo Wang , Andrey Zheludev , Alexander I. Smirnov , Oleg A. Starykh

Rare-earth doped crystals have long coherence times and the potential to provide quantum interfaces between microwave and optical photons. Such applications benefit from a high cooperativity between the spin ensemble and a microwave cavity…

We report a muSR study of LiCrO2, which has a magnetic lattice made up of a stacking of triangular Heisenberg antiferromagnetic (Cr3+, S = 3/2) layers. A static magnetically ordered state is observed below the transition temperature T_N =…

Strongly Correlated Electrons · Physics 2009-06-09 A. Olariu , P. Mendels , F. Bert , L. K. Alexander , A. V. Mahajan , A. D. Hillier , A. Amato

We explore orbital dynamics in the spin liquid candidate Ba3CuSb2O9 using multi-frequency electron spin resonance. We prepared two high quality single crystals. The crystal with a slight copper deficiency shows a structural phase transition…

Strongly Correlated Electrons · Physics 2015-12-09 Yibo Han , Masayuki Hagiwara , Takehito Nakano , Yasuo Nozue , Kenta Kimura , Mario Halim , Satoru Nakatsuji

Magnetic moments arranged at the corners of a honeycomb lattice are predicted to form a novel state of matter, Kitaev quantum spin liquid, under the influence of frustration effects between bond-dependent Ising interactions. Some layered…

Strongly Correlated Electrons · Physics 2022-03-09 Sean K. Takahashi , Jiaming Wang , Alexandre Arsenault , Mykola Abramchuk , Fazel Tafti , Philip M. Singer , Takashi Imai

Spin-orbit coupling is an important ingredient to regulate the many-body physics, especially for many spin liquid candidate materials such as rare-earth magnets and Kitaev materials. The rare-earth chalcogenides NaYbCh$_2$ (Ch = O, S, Se)…

We have performed high-field magnetization and ESR measurements on Ba$_3$CoSb$_2$O$_9$ single crystals, as a representative two-dimensional spin-1/2 Heisenberg antiferromagnet on a uniform triangular lattice, and have determined all the…

Strongly Correlated Electrons · Physics 2015-06-15 Takuya Susuki , Nobuyuki Kurita , Takuya Tanaka , Hiroyuki Nojiri , Akira Matsuo , Koichi Kindo , Hidekazu Tanaka

The interplay between spin-orbit coupling, anisotropic magnetic interaction, frustration-induced quantum fluctuations and spin correlations can lead to novel quantum states with exotic excitations in rare-earth-based quantum magnets.…

Strongly Correlated Electrons · Physics 2023-08-31 J. Khatua , Q. P. Ding , M. S. Ramachandra Rao , K. Y. Choi , A. Zorko , Y. Furukawa , P. Khuntia

We discuss the effects of an applied magnetic field on the low energy excitations in the low temperature phase of Yb4As3. We show also why the magnetic interaction of the Yb{3+} ions is nearly of an isotropic Heisenberg spin-1/2 type. A…

Materials Science · Physics 2007-05-23 Yuri Kudasov , Gennadi Uimin , Peter Fulde , Alexander Ovchinnikov

By means of density functional theory (DFT) calculations (with and without inclusion of spin-orbit (SO) coupling) we present a detailed study of the electronic structure and corresponding microscopic Hamiltonian parameters of Na2IrO3. In…

Strongly Correlated Electrons · Physics 2014-01-31 Kateryna Foyevtsova , Harald O. Jeschke , I. I. Mazin , D. I. Khomskii , Roser Valenti

Competing magnetic interactions in low-dimensional quantum magnets can lead to the exotic ground state with fractionalized excitations. Herein, we present our results on an S = 5/2 quasi-one-dimensional spin system Bi3FeMo2O12. The…