Related papers: Echo Spectroscopy in multi-level quantum-mechanica…
In this work we present a hypothesis that spectral response of atoms or molecules to a pulse of electromagnetic radiation with fast rising or falling fronts would contain a unique emission line that is located approximately near the…
The response of an arbitrary closed quantum system to a partially coherent electric field is investigated, with a focus on the transient coherences in the system. As a model we examine, both perturbatively and numerically, the coherences…
An excitable semiconductor micropillar laser with delayed optical feedback is able to regenerate pulses by the excitable response of the laser. It has been shown that almost any pulse sequence can, in principle, be excited and regenerated…
We study the impact of inter-pulse phase fluctuation in free-electron X-ray laser on the signal in the photon echo spectroscopy, which is one of the simplest non-linear spectroscopic methods. A two-pulse echo model is considered with…
Two-level systems (TLS) are the major source of dephasing of spin qubits in numerous quantum computing platforms. In spite of much effort, it has been difficult to substantially mitigate the effects of this noise or, in many cases, to fully…
While calculations and measurements of single-particle spectral properties often offer the most direct route to study correlated electron systems, the underlying physics may remain quite elusive, if information at higher particle levels is…
We show that particle detectors, such as 2-level atoms, in non-inertial motion (or in gravitational fields) could be used to build quantum gates for the processing of quantum information. Concretely, we show that through suitably chosen…
Dipole-coupled subwavelength quantum emitter arrays respond cooperatively to external light fields as they may host collective delocalized excitations (a form of excitons) with super- or subradiant character. Deeply subwavelength…
We examine the potential-energy curves and polarization of the dipole moments of two static polar molecules under the influence of an external dc electric field and their anisotropic dipole-dipole interaction. We model the molecules as…
In this paper we present an ab initio real-time analysis of free polarization decay and photon echo in extended systems. As a prototype material, we study bulk GaAs driven by ultra-short laser pulses of 10 fs (energy spread of 0.4 eV), with…
How atoms and electrons in a molecule move during a chemical reaction and how rapidly energy is transferred to or from the surroundings can be studied with flashes of laser light. However, despite prolonged efforts to develop various…
The control and manipulation of quantum-entangled non-local states is a crucial step for the development of quantum information processing. A promising route to achieve such states on a wide scale is to couple solid-state quantum emitters…
We investigate the ultracold collisions of rotationally excited dipolar molecules in free-space, taking the hetero-nuclear bi-alkali molecule of KRb as an example. We show that we can sharply tune the elastic, inelastic and reactive rate…
The use of rotational degrees of freedom of quantum systems in quantum technologies is limited by environmental effects under decoherence mechanism. Here, we study the mechanism of decoherence based on a new formalism of elastic scattering…
We analyze theoretically the interplay between the torsional and the rotational motion of an aligned biphenyl-like molecule. To do so, we consider a transition between two electronic states with different internal torsional potentials,…
Understanding and controlling the electronic as well as ro-vibrational motion and, thus, the entire chemical dynamics in molecules is the ultimate goal of ultrafast laser and imaging science. In photochemistry, laser-induced dissociation…
High-harmonic spectroscopy driven by circularly-polarized laser pulses and their counter-rotating second harmonic is a new branch of attosecond science which currently lacks quantitative interpretations. We extend this technique to the…
Ultrachirped pulses for which the frequency chirp is of the order of the transition frequency of a two-level atom are examined. When the chirp is large enough, the resonance may be crossed twice, for positive and negative quadrature…
The resonant quantum dynamics of an excited two-level emitter is investigated via classical modulation of its transition frequency while simultaneously the radiator interacts with a broadband electromagnetic field reservoir. The frequency…
Spectra of Thomson and Compton radiation, emitted during electron scattering off an intense laser beam, are calculated using the frameworks of classical and strong-field quantum electrodynamics, respectively. Both approaches use a…