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Quantum coherence is highly involved in photochemical functioning of complex molecular systems. Co-existence and intermixing of electronic and/or vibrational coherences, while never unambiguously identified experimentally, has been proposed…
We have demonstrated that a rather weak external optical feedback with delay can lead to the mode switching of the counterpropogating modes. The delay time should be longer then any system characteristic time. The equations describing the…
Coherent two-dimensional spectroscopy in IR or visible region is very effective for studying correlations, energy relaxation/transfer pathways in complex multi-chromophore or multi-mode systems. However it is usually restricted up to…
We demonstrate that the coupling of excitonic and vibrational motion in biological complexes can provide mechanisms to explain the long-lived oscillations that have been obtained in non linear spectroscopic signals of different…
Ultrafast lasers have become one of the most powerful tools in coherent nonlinear optical spectroscopy. Short pulses enable direct observation of fast molecular dynamics, whereas broad spectral bandwidth offers ways of controlling nonlinear…
Multi-qubit quantum sensors are rapidly emerging as platforms that extend the capabilities of conventional single-qubit sensing. In this work we show how suitable pulse sequences applied to a two-qubit sensor enable separate extraction of…
The theory of the ultrashort laser pulse scattered by metallic nanoparticles in the region of surface plasmon resonances is developed in the framework of kinetic approach. For the spheroidal particles, the dependence of the light scattering…
We have observed multi-photon resonances in a system with a spin 3/2 irradiated simultaneously by a multiple pulse radiofrequency sequence and a low frequency field swept in the range 0-80 kHz. The used excitation scheme allowed us to…
The angular momentum of molecules, or, equivalently, their rotation in three-dimensional space, is ideally suited for quantum control. Molecular angular momentum is naturally quantized, time evolution is governed by a well-known Hamiltonian…
Is it possible to infer the time evolving quantum state of a multichromophoric system from a sequence of two-dimensional electronic spectra (2D-ES) as a function of waiting time? Here we provide a positive answer for a tractable model…
Given the wide range of applications of time-domain spectroscopy, and particularly THz time-domain spectroscopy, the modelling of a probe pulse propagating through a multilayered structure is often required. Due to the fact that the…
The at-will control of quantum states is a primary goal of quantum science and technology. The celebrated Hahn echo exemplifies such quantum-state control based on a time-reversal process in a few-level system. Here, we propose a different…
We show that the precise preparation of a quantum superposition between three rotational states of an ultracold dipolar molecule generates controllable interferences in their two-body scattering dynamics and collisional rate coefficients,…
We investigate the influence of a stochastically fluctuating step-barrier potential on bimolecular reaction rates by exact analytical theory and stochastic simulations. We demonstrate that the system exhibits a new resonant reaction…
Chiral molecules with broken parity symmetries can be modeled as quantum systems with cyclic-transition structures. By using these novel properties, we design two-step laser pulses to distinguish left- and right-handed molecules from the…
We investigate the ultrafast optical response of the one-dimensional half-filled extended Hubbard model exposed to two successive laser pulses. By using the time-dependent Lanczos method, we find that following the first pulse, the…
The ability to coherently spectrally manipulate quantum information has the potential to improve qubit rates across quantum channels and find applications in optical quantum computing. In this paper we present experiments that use a…
We report on magneto-oscillations in differential resistivity of a two-dimensional electron system subject to intense microwave radiation. The period of these oscillations is determined not only by microwave frequency but also by its…
We characterize the coherent dynamics of a two-level quantum emitter driven by a pair of symmetrically-detuned phase-locked pulses. The promise of dichromatic excitation is to spectrally isolate the excitation laser from the quantum…
With analytical treatment, the classical dynamics of an ultrarelativistic electron in two counter-propagating circularly polarized strong laser beams with either co-rotating or counter-rotating direction are considered. Assuming that the…