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Related papers: The pyrochlore Ho2Ti2O7: Synthesis, crystal growth…

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Strontium titanate (SrTiO$_{3}$, STO) stands out as a promising material for various electronic applications thanks to its exceptional dielectric properties. Molecular beam epitaxy is one of the few techniques which allows epitaxial growth…

The synthesis of stoichiometric and epitaxial pyrochlore iridate thin films presents significant challenges yet is critical for unlocking experimental access to novel topological and magnetic states. Towards this goal, we unveil an in-situ…

Mm-sized LiMn$_{1-x}$Fe$_x$PO$_4$ single crystals with $0\leq x \leq 1$ were grown by means of the traveling floating-zone technique at elevated Argon pressure of 30~bar. For the various doping levels, the growth process was optimized with…

Strongly Correlated Electrons · Physics 2017-02-07 Christoph Neef , Hubert Wadepohl , Hans-Peter Meyer , Rüdiger Klingeler

Highly crystalline TiO2 nanostructures were prepared through a facile inorganic acid-assisted hydrothermal treatment of hexagonal-structured assemblies of nanocrystalline titiania templated by cetyltrimethylammonium bromide (Hex-ncTiO2/CTAB…

Materials Science · Physics 2012-11-20 Shuxi Dai , Yanqiang Wu , Toshio Sakai , Zuliang Du , Hideki Sakai , Masahiko Abe

The compound CaV2O4 contains V^{+3} cations with spin S = 1 and has an orthorhombic structure at room temperature containing zigzag chains of V atoms running along the c-axis. We have grown single crystals of CaV2O4 and report…

High-quality Bi$_{2+x}$Sr$_{2-x}$CuO$_{6+\delta}$(0$<$x$\leq$0.5) single crystals have been grown successfully using the travelling-solvent floating-zone(TSFZ) technique. The samples with $x >$ 0.05 are in the underdoped level. The…

Superconductivity · Physics 2009-11-11 Huiqian Luo , Lei Fang , Gang Mu , Hai-Hu Wen

Although materials that exhibit nearest-neighbor-only antiferromagnetic interactions and geometrical frustration theoretically should not magnetically order in the absence of disorder, few such systems have been observed experimentally. One…

Strongly Correlated Electrons · Physics 2016-08-31 S. -W. Han , J. S. Gardner , C. H. Booth

This study reports atomic-scale characterization of structural defects in Yb2Ti2O7, a pyrochlore oxide whose subtle magnetic interactions is prone to small perturbations. Due to discrepancies in the reported magnetic ground states, it has…

Strongly Correlated Electrons · Physics 2018-10-29 Zahra Shafieizadeh , Yan Xin , Seyed M. Koohpayeh , Qing Huang , Haidong Zhou

Tb2Ti2O7, a pyrochlore system, has garnered significant interest due to its intriguing structural and physical properties and their dependence on external physical parameters. In this study, utilizing high-brilliance synchrotron X-ray…

High resolution X-ray powder-diffraction experiments on a well-characterized polycrystalline sample of the spin liquid Tb2Ti2O7 reveal that it shows normal positive thermal-expansion above 4 K, which does not agree with the intriguing…

Strongly Correlated Electrons · Physics 2011-12-14 Kazuki Goto , Hiroshi Takatsu , Tomohiro Taniguchi , Hiroaki Kadowaki

To investigate excess-hydrolysis of titanium alkoxides, TiO2 powders were fabricated from titanium-tetra-isopropoxide using 6:1 and 100:1 H2O:Ti (r) ratios. Powders were dried and fired at a range of temperatures ( up to 800 C).…

Materials Science · Physics 2014-10-31 Dorian A. H. Hanaor , Ilkay Chironi , Inna Karatchevtseva , Gerry Triani , Charles C. Sorrell

Spin ice materials are the model systems that have a zero-point entropy as \textit{T} $\rightarrow$ 0 K, owing to the frozen disordered states. Here, we chemically alter the well-known spin ice Ho$_{2}$Ti$_{2}$O$_{7}$ by replacing Ti sites…

Strongly Correlated Electrons · Physics 2022-04-20 Sheetal , A. Elghandour , R. Klingeler , C. S. Yadav

Synthesis and crystal structures are described for the compounds Ln2(Ti2-xLnx)O7-x/2, where Ln = Tb, Dy, Ho, Er, Tm, Yb, Lu, and x ranges from 0 to 0.67. Rietveld refinements on X-ray powder diffraction data indicate that in Tb and Dy…

Strongly Correlated Electrons · Physics 2009-08-11 G. C. Lau , B. D. Muegge , T. M. McQueen , E. L. Duncan , R. J. Cava

Motivated by the variation in reported lattice parameters of floating-zone-grown Nd$_{2}$Zr$_{2}$O$_{7}$ crystals, we have performed a detailed study of the relationship between synthesis environment, structural disorder, and magnetic…

We report the growth of mm-sized Pmnb-Li2FeSiO4 single crystals by means of the optical floating-zone method at high argon pressure and describe the conditions required for a stable growth process. The crystal structure is determined and…

Recent experimental results have emphasized two aspects of Tb2Ti2O7 which have not been taken into account in previous attempts to construct theories of Tb2Ti2O7: the role of small levels of structural disorder, which appears to control the…

Strongly Correlated Electrons · Physics 2016-05-04 M. Ruminy , L. Bovo , E. Pomjakushina , M. K. Haas , U. Stuhr , A. Cervellino , R. J. Cava , M. Kenzelmann , T. Fennell

Nanotubed titanic acid (H2Ti2O4(OH)2) was prepared from nanotubed sodium titanate (Na2Ti2O4(OH)2) by an ion exchange reaction in a pH=1 HCl solution. The effect of annealing temperature on the morphology, structure and photocatalytic…

Materials Science · Physics 2010-09-16 Min Zhang , Zhensheng Jin , Jingwei Zhang , Xinyong Guo , Jianjun Yang , Wei Li , Xiaodong Wang , Zhijun Zhang

Reduced titanium dioxide has recently attracted large attention, particularly for its unique co-catalyst-free H$_2$ heterogeneous photocatalytic application. The enhanced photocatalytic activity of the reduced TiO$_2$ was previously…

We present the structural, magnetic, thermal and ab-plane electronic transport properties of single crystals of CaCu1.7As2 grown by the self-flux technique that were investigated by powder x-ray diffraction, magnetic susceptibility chi,…

Superconductivity · Physics 2013-08-20 V. K. Anand , D. C. Johnston

We report the growth of YFe2O4-\delta\ single crystals by the optical floating zone method, showing for the first time the same magnetization as highly stoichiometric (\delta = 0.00) powder samples and sharp superstructure reflections in…

Materials Science · Physics 2015-08-13 Thomas Mueller , Joost de Groot , Joerg Strempfer , Manuel Angst