Related papers: High-resolution spectroscopy on cold electrically …
$^{133}\text{Ba}^+$ has been identified as an attractive ion for quantum information processing due to the unique combination of its spin-1/2 nucleus and visible wavelength electronic transitions. Using a microgram source of radioactive…
We demonstrate optical cycling and sub-Doppler laser cooling of a cryogenic buffer-gas beam of calcium monohydride (CaH) molecules. We measure vibrational branching ratios for laser cooling transitions for both excited electronic states A…
Cold, neutral hydroxyl radicals are Stark decelerated and confined within a magnetic trap consisting of two permanent ring magnets. The OH molecules are trapped in the ro-vibrational ground state at a density of $\sim10^{6}$ cm$^{-3}$ and…
We describe an approach to optically trapping small, chemically stable molecules at cryogenic temperatures by buffer-gas loading a deep optical dipole trap. The ~10 K trap depth will be produced by a tightly-focused, 1064-nm cavity capable…
Direct frequency comb spectroscopy of trapped ions is demonstated for the first time. It is shown that the 4s^2S_(1/2)-4p^2P_(3/2) transition in calcium ions can be excited directly with a frequency comb laser that is upconverted to 393 nm.…
We investigate the effect of far-off-resonant trapping light on ultracold bosonic RbCs molecules. We use kHz-precision microwave spectroscopy to measure the differential AC Stark shifts between the ground and first excited rotational levels…
We report a magneto-optical trap of strontium monohydroxide (SrOH) containing 2000(600) molecules at a temperature of 1.2(3) mK. The lifetime is 91(9) ms, which is limited by decay to optically unaddressed vibrational states. This provides…
The rotational spectrum of the formaldehyde isotopologue H$_2$C$^{17}$O was investigated between 0.56 and 1.50 THz using a sample of natural isotopic composition. In addition, transition frequencies were determined for H$_2$C$^{18}$O and…
We study the influence of a scanning nano-electrode on fluorescence excitation spectra of single terrylene molecules embedded in thin p-terphenyl films at cryogenic temperatures. We show that applied voltages less than 10 V can result in…
We present a model as well as experimental results for a surface electrode radio-frequency Paul trap that has a circular electrode geometry well-suited for trapping of single ions and two-dimensional planar ion crystals. The trap design is…
Heavy polar molecules can be used to measure the electric dipole moment of the electron, which is a sensitive probe of physics beyond the Standard Model. The value is determined by measuring the precession of the molecule's spin in a plane…
We propose a novel Sisyphus cooling scheme for atoms confined in a far off resonance optical dipole trap. Utilizing the differential trap-induced AC Stark shift, two electronic levels of the atom are resonantly coupled by a cooling laser…
The electronic energy level structure of yttrium monoxide (YO) provides a long-lived, low-lying $^{2}\Delta$ state ideal for high-precision molecular spectroscopy, narrowline laser cooling at the single photon-recoil limit, and studying…
Recently, the extremely sensitive torsion-rotation transitions in methanol have been used to set a tight constraint on a possible variation of the proton-to-electron mass ratio over cosmological time scales. In order to improve this…
We report the sympathetic cooling and Coulomb crystallization of molecular ions above the surface of an ion-trap chip. N$_2^+$ and CaH$^+$ ions were confined in a surface-electrode radiofrequency ion trap and cooled by the interaction with…
To provide constraints on the chemical processes responsible for the observed columns of organic species, we used NOEMA to observe the sight line toward NRAO150 in the 2mm spectral window. We targeted the low excitation lines of o-H2CO…
Carbon monoxide molecules in their electronic, vibrational, and rotational ground state are highly attractive for trapping experiments. The optical or ac electric traps that can be envisioned for these molecules will be very shallow,…
The precise measurement of transition frequencies in cold, trapped molecules has applications in fundamental physics, and extremely high accuracies are desirable. We determine suitable candidates by considering simple molecules with a…
We demonstrate significantly improved magneto-optical trapping of molecules using a very slow cryogenic beam source and RF modulated and DC magnetic fields. The RF MOT confines $1.1(3) \times 10^5$ CaF molecules at a density of $4(1) \times…
We have demonstrated a high temperature vapor cell for absorption spectroscopy on the Ca intercombination line. The cell uses a dual chamber design to achieve the high temperatures necessary for an optically dense vapor while avoiding the…