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Ionization of atoms and molecules by absorption of a light pulse results in electron wavepackets carrying information on the atomic or molecular structure as well as on the dynamics of the ionization process. These wavepackets can be…

Two-photon excitation spectroscopy is a nonlinear technique that has gained rapidly in interest and significance for studying the complex energy-level structure and transition probabilities of materials. While the conventional spectroscopy…

Quantum Physics · Physics 2022-11-23 Yuanyuan Chen , Roberto de J. León-Montiel , Lixiang Chen

We study resonant two-photon ionization of helium atoms via the $1s3p$, $1s4p$ and $1s5p^1$P$_1$ states using the 15$^\mathrm{th}$ harmonic of a titanium-sapphire laser for the excitation and a weak fraction of the laser field for the…

We present numerical simulations of ultrafast multiphoton ionization dynamics in a two-dimensional atomic model driven by co- and counterrotating circularly polarized single-color and bichromatic carrier envelope phase (CEP) stable…

Atomic Physics · Physics 2020-07-15 T. Bayer , Ch. Philipp , K. Eickhoff , M. Wollenhaupt

We extend the semiclassical two-step model for strong-field ionization that describes quantum interference and accounts for the Coulomb potential beyond the semiclassical perturbation theory to the hydrogen molecule. In the simplest case of…

Atomic Physics · Physics 2019-03-27 N. I. Shvetsov-Shilovski , M. Lein , K. Tőkési

The light emission from a scanning tunneling microscope operated on a Ag(111) surface at 6 K is analyzed from low conductances to values approaching the conductance quantum. Optical spectra recorded at a sample voltages V reveal emission…

Mesoscale and Nanoscale Physics · Physics 2018-09-11 Peter-Jan Peters , Fei Xu , Kristen Kaasbjerg , Gianluca Rastelli , Wolfgang Belzig , Richard Berndt

We present a theory that efficiently describes the quantum dynamics of an electronic excitation that is coupled to a continuous, highly structured phonon environment. Based on a stochastic approach to non-Markovian open quantum systems, we…

Quantum Physics · Physics 2009-11-05 Jan Roden , Alexander Eisfeld , Wolfgang Wolff , Walter T. Strunz

We developed a new method to calculate two-photon processes in quantum mechanics that replaces the infinite summation over the intermediate states by a perturbation expansion. This latter consists of a series of commutators that involve…

Quantum Physics · Physics 2018-04-25 Filippo Fratini , Laleh Safari , Pedro Amaro , José-Paulo Santos

Attosecond photoionisation time delays reveal information about the potential energy landscape an outgoing electron wavepacket probes upon ionisation. In this study we experimentally quantify, for the first time, the dependence of the time…

We present the first demonstration of two-photon double ionization of neon using an intense extreme ultraviolet (XUV) attosecond pulse train (APT) in a photon energy regime where both direct and sequential mechanisms are allowed. For an APT…

Attosecond interferometry in a two-color field is central to attosecond metrology and spectroscopy. In this technique, a photoelectron wave packet is released when a single photon from an extreme ultraviolet comb is absorbed. The wave…

Owing to its numerical simplicity, a two-dimensional two-electron model atom, with each electron moving in one direction, is an ideal system to study non-perturbatively a fully correlated atom exposed to a laser field. Frequently made…

Atomic Physics · Physics 2009-10-30 D. Bauer

We investigate dynamics of atomic and molecular systems exposed to intense, shaped chaotic fields and a weak femtosecond laser pulse theoretically. As a prototype example, the photoionization of a hydrogen atom is considered in detail. The…

Quantum Physics · Physics 2015-05-18 Kamal P Singh , Jan M Rost

Exchange correlation plays an important role in double-ionization of complex atoms by ultrashort laser pulse. In this work, we investigate two-photon double inner-shell electron ionization of neon induced by an attosecond extreme…

Atomic Physics · Physics 2019-06-05 Jianpeng Liu , Yongqiang Li , Jianmin Yuan

A new theoretical approach to the description of the attosecond streaking measurements of atomic photoionization is presented. It is a fully quantum mechanical description based on numerical solving of the time-dependent Schroedinger…

Atomic Physics · Physics 2007-05-23 A. K. Kazansky , N. M. Kabachnik

The radiation of photons by electrons is investigated in the framework of quantum electrodynamics up to the second order in the coupling constant $e$. The $N$-particle, coherent, and thermal initial states are considered and the forms of…

High Energy Physics - Theory · Physics 2022-09-08 P. O. Kazinski , T. V. Solovyev

Ionization by relativistically intense short laser pulses is studied in the framework of strong-field quantum electrodynamics. Distinctive patterns are found in the energy probability distributions of photoelectrons. Except of the already…

Atomic Physics · Physics 2018-03-14 F. Cajiao Vélez , J. Z. Kamiński , K. Krajewska

A variational treatment for a two-electron quantum dot (the artificial helium atom) is proposed which leads to exact answer for the ground state energy. Depending on the magnetic field value the singlet-triplet and triplet-triplet…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Subinoy Das , Pallab Goswami , J. K. Bhattacharjee

We analyze atomic photoexcitation into the discrete states by twisted photons, or photons carrying extra orbital angular momentum along their direction of propagation. From the angular momentum and parity considerations, we are able to…

Atomic Physics · Physics 2018-03-07 Andrei Afanasev , Carl E. Carlson , Maria Solyanik

A new approach is laid out to investigate the two photon atomic transitions. It is based on application of the finite basis solutions constructed from the Bernstein Polynomial (B-Polynomial) sets. We show that such an approach provides a…

Mathematical Physics · Physics 2015-05-28 P. Amaro , A. Surzhykov , F. Parente , P. Indelicato , J. P. Santos