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Perovskite SrIrO3 (SIO) films epitaxially deposited with a thickness of about 60 nm on various substrate materials display nearly strain-relieved state. Films grown on orthorhombic (110) DyScO3 (DSO) are found to display untwinned bulk-like…

Strongly Correlated Electrons · Physics 2018-09-19 K. R. Kleindienst , K. Wolff , J. Schubert , R. Schneider , D. Fuchs

We investigated the electronic structure of the SrTiO$_3$/LaAlO$_3$ superlattice (SL) by resonant soft x-ray scattering. The (003) peak, which is forbidden for our "ideal" SL structure, was observed at all photon energies, indicating…

We have measured photoemission spectra of SrTiO3/LaTiO3 superlattices with a topmost SrTiO3 layer of variable thickness. Finite coherent spectral weight with a clear Fermi cut-off was observed at chemically abrupt SrTiO3/LaTiO3 interfaces,…

The resistivity of the two dimensional electron gas that forms at the interface of strontium titanate with various oxides is sensitive to irradiation with visible light. In this letter we present data on the interface between the band gap…

Superconductivity · Physics 2019-09-23 D. Arnold , D. Fuchs , K. Wolff , R. Schäfer

Interface effects on the ferroelectric behavior of PbTiO$_3$ ultrathin films deposited on SrTiO$_3$ substrate are investigated using an interatomic potential approach with parameters fitted to first-principles calculations. We find that the…

Materials Science · Physics 2009-11-11 M Sepliarsky , M. G. Stachiotti , R. L. Migoni

We investigate energetic stability and dissociation dynamics of water adsorption at the LaAlO3 surface of the n-type LaAlO3/SrTiO3 (LAO/STO) interface and its effect on electronic properties of the interface by carrying out first-principles…

Materials Science · Physics 2015-06-15 Yun Li , Jaejun Yu

The temperature dependence of the electrical resistivity of the heterostructures consisting of single crystalline LaMnO$_3$ samples with different crystallographic orientations covered by the epitaxial ferroelectric…

Strongly Correlated Electrons · Physics 2017-10-20 D. P. Pavlov , I. I. Piyanzina , V. M. Mukhortov , A. M. Balbashov , D. A. Tayurskii , I. A. Garifullin , R. F. Mamin

The coupling between the electrical transport properties of La2/3Sr1/3MnO3 (LSMO) thin films and structural phase transitions of SrTiO3 (STO) substrates at Ts = 105 K has been investigated. We found that the electrical resistivity of LSMO…

Materials Science · Physics 2017-02-28 Zhaoliang Liao , Rongying Jin , E. W. Plummer , Jiandi Zhang

A two-dimensional electron liquid is formed at the n-type interface between SrTiO3 and LaAlO3. Here we report on Kelvin probe microscopy measurements of the electronic compressibility of this electron system. The electronic compressibility…

Strongly Correlated Electrons · Physics 2012-08-14 V. Tinkl , M. Breitschaft , C. Richter , J. Mannhart

We report on the synthesis of high quality La$_{1/3}$Sr$_{2/3}$FeO$_3$ (LSFO) thin films using the pulsed laser deposition technique on both SrTiO$_3$ (STO) and LaAlO$_3$ (LAO) substrates (100)-oriented. From X-Ray diffraction (XRD)…

Materials Science · Physics 2009-11-07 W. Prellier , B. Mercey

A combined experimental and theoretical investigation of the electronic structure of the archetypal oxide heterointerface system LaAlO3 on SrTiO3 is presented. High-resolution, hard x-ray photoemission is used to uncover the occupation of…

Thin film synthesis methods developed over the past decades have unlocked emergent interface properties ranging from conductivity to ferroelectricity. However, our attempts to exercise precise control over interfaces are constrained by a…

Materials Science · Physics 2017-11-15 Steven R. Spurgeon , Peter V. Sushko , Ryan B. Comes , Scott A. Chambers

The surface termination of (100)-oriented LaAlO3 (LAO) single crystals was examined by atomic force microscopy and optimized to produce a single-terminated atomically flat surface by annealing. Then the atomically flat STO film was achieved…

Materials Science · Physics 2012-05-09 Z. Q. Liu , Z. Huang , W. M. Lü , K. Gopinadhan , X. Wang , A. Annadi , T. Venkatesan , Ariando

We investigate the effect of the laser parameters of pulsed laser deposition on the film stoichiometry and electronic properties of LaAlO_3/SrTiO_3 (001) heterostructures. The La/Al ratio in the LaAlO_3 films was varied over a wide range…

Materials Science · Physics 2015-06-15 H. K. Sato , C. Bell , Y. Hikita , H. Y. Hwang

We have studied the electronic properties of the 2D electron liquid present at the LaAlO$_3$/SrTiO$_3$ interface in series of samples prepared at different growth temperatures. We observe that interfaces fabricated at 650{\deg}C exhibit the…

Materials Science · Physics 2015-03-20 A. Fête , C. Cancellieri , D. Li , D. Stornaiuolo , A. D. Caviglia , S. Gariglio , J. -M. Triscone

Hard x-ray photoelectron spectroscopy (HAXPES) and variable kinetic energy x-ray photoelectron spectroscopy (VKE-XPS) analyses have been performed on 10 unit cell La$_{(1-{\delta})}$Al$_{(1+{\delta})}$O$_3$ films, with La:Al ratios of 1.1,…

Materials Science · Physics 2015-06-24 C. Weiland , G. E. Sterbinsky , A. K. Rumaiz , C. S. Hellberg , J. C. Woicik , S. Zhu , D. G. Schlom

The ability to control materials properties through interface engineering is demonstrated by the appearance of conductivity at the interface of certain insulators, most famously the {001} interface of the band insulators LaAlO$_{3}$ and…

We present a first-principles study of the electronic structures and properties of ideal (atomically sharp) LaAlO3/SrTiO3 (001) heterointerfaces and their variants such as a new class of quantum well systems. We demonstrate the…

Materials Science · Physics 2015-05-19 Hanghui Chen , Alexie M. Kolpak , Sohrab Ismail-Beigi

The effect of growth conditions on the structural and electronic properties of the polar/non-polar LaCrO$_3$/SrTiO$_3$ (LCO/STO) interface has been investigated. The interface is either insulating or metallic depending on growth conditions.…

Materials Science · Physics 2019-06-04 A. H. Al-Tawhid , J. R. Frick , D. B. Dougherty , D. P. Kumah

LaNiO$_3$ (LNO) is an intriguing member of the rare-earth nickelates in exhibiting a metal-insulator transition for a critical film thickness of about 4 unit cells [Son et al., Appl. Phys. Lett. 96, 062114 (2010)]; however, such thin films…