Related papers: Photon echo from localized excitons in semiconduct…
We report a theoretical description and experimental implementation of a novel two-dimensional coherent excitation spectroscopy based on quasi-steady-state photoinduced absorption measurement of a long-lived nonlinear population. We have…
Based on new obtained analytical results, the main properties of photon echo quantum memory protocols are analysed and discussed together with recently achieved experimental results. The main attention is paid to studying the influence of…
Nonlinear optical processes in low dimensional materials are often weak or symmetry forbidden, limiting their use in nanoscale light sources and on chip frequency conversion. Here, we show that combining two weakly nonlinear systems,…
We theoretically propose a biphoton entanglement-enhanced multidimensional spectroscopic technique as a probe for the dissipative polariton dynamics in the ultrafast regime. It is applied to the cavity-confined monomeric photosynthetic…
The elementary optical excitations in two dimensional semiconductors hosting itinerant electrons are attractive and repulsive polarons -- excitons that are dynamically screened by electrons. Exciton-polarons have hitherto been studied in…
We demonstrate that electron-phonon interaction in quantum dots embedded in one-dimensional systems leads to pronounced, non-Markovian decoherence of optical transitions. The experiments we present focus on the lineshape of…
We present a detailed analysis of exciton-photon interaction in a microcavity made out of a photonic crystal slab. Here we have analyzed a disk-like quantum dot where an exciton is formed. Excitonic eigen-functions in addition to their…
The exponential growth of photonic quantum technologies is driving the demand of tools for measuring the quality of their information carriers. One of the most prominent is Stimulated Emission Tomography (SET), which uses classical coherent…
We demonstrate that semiconductor quantum dots can be excited efficiently in a resonant three-photon process, whilst resonant two-photon excitation is highly suppressed. Time-dependent Floquet theory is used to quantify the strength of the…
Resonant laser excitation of a two-level system with subsequent single-photon emission can be used to generate single photons with high indistinguishability or Hong-Ou-Mandel (HOM) visibility. However, spectral overlap between excitation…
Since dissipative processes are ubiquitous in semiconductors, characterizing how electronic and thermal energy transduce and transport at the nanoscale is vital for understanding and leveraging their fundamental properties. For example, in…
The manipulation of coupled quantum excitations is of fundamental importance in realizing novel photonic and optoelectronic devices. We use electroluminescence to probe plasmon-exciton coupling in hybrid structures consisting of a nanoscale…
Femtosecond (fs)-resolved photoemission electron micrographs of single and few-layer MoSe$_2$ track exciton dynamics in this model 2D quantum material system with joint nanometer (nm)-fs resolution. We illustrate the latter using two-photon…
The possibility to store optical information is important for classical and quantum communication. Atoms or ions as well as color centers in crystals offer suitable two-level systems for absorbing incoming photons. To obtain a reliable…
Semiconductors in all dimensionalities ranging from 0D quantum dots and molecules to 3D bulk crystals support bound electron-hole pair quasiparticles termed as excitons. Over the past two decades, the emergence of a variety of…
Femtosecond core-level transient absorption spectroscopy is utilized to investigate photoinduced dynamics of the charge density wave in 1T-TiSe2 at the Ti M2,3 edge (30-50 eV). Photoexcited carriers and phonons are found to primarily induce…
We study theoretically optomechanical damping and amplification spectra for vibrations interacting with excitonic polaritons in a zero-dimensional microcavity. We demonstrate, that the spectra strongly depend on the ratio of the…
We study the role of electron-phonon scattering for a pulse-triggered quantum dot single-photon source which utilizes a modified version of stimulated Raman adiabatic passage and cavity-coupling. This on-demand source is coherently pumped…
Phonon damping is the main source of pure dephasing in the solid state, limiting many fundamental quantum effects to low temperature observations. Here we show how excitons in semiconductors can be totally decoupled from the phonon bath,…
Quantum applications of solid state systems base upon generation and control of coherent electronic excitations. Prominent examples are exciton states in semiconductors excitable by photons. The high oscillator strength of electric-dipole…