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We use nonlinear pump-probe spectroscopy to study optical excitations in a charge-tunable MoSe$_2$\WS$_2$ moir\'e heterostructure. An intense red-detuned laser pulse creates a photonic dressing of the material by introducing a large virtual…

Strongly Correlated Electrons · Physics 2025-06-02 B. Evrard , H. S. Adlong , A. A. Ghita , T. Uto , L. Ciorciaro , K. Watanabe , T. Taniguchi , M. Kroner , A. İmamoğlu

Herein, the dynamics of excitons coupled with optical phonons in a triangular system is numerically studied. By representing the excitons by quasi-spin states, the similarity between the chiral spin states and the exciton chiral states is…

Mesoscale and Nanoscale Physics · Physics 2023-05-30 Noriyuki Aoyagi , Hiroaki Matsueda , Kunio Ishida

Multi-exciton correlations shape the photo-induced response of nanostructured materials, particularly when interactions are enhanced by light confinement. Here multidimensional coherent spectroscopy is used to quantify biexciton and…

Mesoscale and Nanoscale Physics · Physics 2025-07-11 Giuseppe Fumero , Jagannath Paul , Jared K. Wahlstrand , Alan D. Bristow

We demonstrate the spatial confinement of electronic excitations in a solid state system, within novel artificial structures that can be designed having arbitrary dimensionality and shape. The excitations under study are exciton-polaritons…

Strong Coulomb interaction in atomically-thin transition metal dichalcogenides makes these systems particularly promising for studies of excitonic physics. Of special interest are the manifestations of the charged excitons, also known as…

Mesoscale and Nanoscale Physics · Physics 2020-08-26 M. M. Glazov

Harnessing the optoelectronic response of organic semiconductors requires a thorough understanding of the fundamental light-matter interaction that is dominated by the excitation of correlated electron-hole pairs, i.e. excitons. The nature…

Non-equilibrium photon correlations of coherently excited single quantum systems can reveal their internal quantum dynamics and provide spectroscopic access. Here we propose and discuss the fundamentals of a coherent photon coincidence…

Quantum Physics · Physics 2020-11-04 Matthew Otten , Tristan Kenneweg , Matthias Hensen , Stephen K. Gray , Walter Pfeiffer

Resonant excitation of the biexciton state in an InAsP quantum dot by a phase-coherent pair of picosecond pulses allows preparing time-bin entangled pairs of photons via the biexciton-exciton cascade. We show that this scheme can be…

Vibrational-electronic (vibronic) resonance and its role in energy and charge transfer has been experimentally and theoretically investigated in several photosynthetic proteins. Using a dimer modeled on a typical photosynthetic protein, we…

Chemical Physics · Physics 2020-09-03 Amitav Sahu , Jo Sony Kurian , Vivek Tiwari

Entangled photon pairs are key to many novel applications in quantum technologies. Semiconductor quantum dots can be used as sources of on-demand, highly entangled photons. The fidelity to a fixed maximally entangled state is limited by the…

Coupling to phonon modes is a primary mechanism of excitonic dephasing and energy loss in semiconductors. However, low-energy phonons in colloidal quantum dots and their coupling to excitons are poorly understood, since their experimental…

Mesoscale and Nanoscale Physics · Physics 2019-10-22 Albert Liu , Diogo B. Almeida , Wan-Ki Bae , Lazaro A. Padilha , Steven T. Cundiff

Control of the band-edge offsets at heterojunctions between organic semiconductors allows efficient operation of either photovoltaic or light-emitting diodes. We investigate systems where the exciton is marginally stable against charge…

Soft Condensed Matter · Physics 2013-09-27 Arne C. Morteani , Paiboon Sreearunothai , Laura M. Herz , Richard H. Friend , Carlos Silva

Strong coupling of two-dimensional semiconductor excitons with plasmonic resonators enables control of light-matter interaction at the subwavelength scale. Here we develop strong coupling in plasmonic nano-gap resonators that allow…

This review discusses how low-energy, valence excitations created by swift electrons can render information on the optical response of structured materials with unmatched spatial resolution. Electron microscopes are capable of focusing…

Materials Science · Physics 2012-11-13 F. J. Garcia de Abajo

We investigate both experimentally and theoretically a simple yet more robust and flexible alternative to Rabi oscillation-type biexciton preparation protocols traditionally used for semiconductor quantum dots. The quantum dot is excited by…

Quantum Physics · Physics 2015-06-22 S. Bounouar , M. Müller , A. M. Barth , M. Glässl , V. M. Axt , P. Michler

The resonant interaction between quasi-one dimensional excitons and photons is investigated. For a single isolated organic quantum wire, embedded in its single crystal monomer matrix, the strong exciton-photon coupling regime is reached.…

Strongly Correlated Electrons · Physics 2009-11-11 F. Dubin , J. Berrehar , R. Grousson , M. Schott , V. Voliotis

In this chapter we review the use of semiconductor quantum dots as sources of quantum light. Principally, we focus on resonant two-photon excitation, which is a method that allows for on-demand generation of photon pairs. We explore the…

Quantum Physics · Physics 2016-08-08 Ana Predojević

Interlayer excitons in two dimensional semiconductor heterostructures show suppressed electron-hole overlap resulting in longer radiative lifetimes as compared to intralyer excitons. Such tightly bound interlayer excitons are relevant for…

We studied the intensity of resonant Raman scattering due to optical phonons in a planar II-VI-type semiconductor microcavity in the regime of strong coupling between light and matter. Two different sets of independent experiments were…

Strongly Correlated Electrons · Physics 2009-10-20 A. Bruchhausen , L. M. Leon Hilario , A. A. Aligia , A. M. Lobos , A. Fainstein , B. Jusserand , R. Andre

Exciton-polaritons emerging from the interaction of photons and excitons in the strong coupling regime are intriguing quasiparticles for the potential exchange of energy during light-matter interaction processes such as light harvesting.…