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Time-dependent density-functional theory (TDDFT) is an extension of ground-state density-functional theory which allows the treatment of electronic excited states and a wide range of time-dependent phenomena in the linear and nonlinear…

Materials Science · Physics 2025-10-10 Carsten A. Ullrich

Time-dependent density-functional theory (TDDFT) is deemed to be a formally rigorous way of dealing with the time-evolution of a many-electron system at the level of electron densities rather than the underlying wavefunctions, which in turn…

Chemical Physics · Physics 2024-11-26 Jochen Schirmer

In the last 10 years, we have observed an important increase of interest in the application of time-dependent energy density functional theory (TD-EDF). This approach allows to treat nuclear structure and nuclear reaction from small to…

Nuclear Theory · Physics 2015-10-28 Denis Lacroix , Yusuke Tanimura , Guillaume Scamps , Cédric Simenel

Time-dependent density functional theory (TDDFT) is rapidly emerging as a premier method for solving dynamical many-body problems in physics and chemistry. The mathematical foundations of TDDFT are established through the formal existence…

Quantum Physics · Physics 2014-08-22 J. D. Whitfield , M. -H. Yung , D. G. Tempel , S. Boixo , A. Aspuru-Guzik

We compute nuclear response functions by solving the time-dependent A-body Schr\"odinger equation, recording the time-dependent transition moment and extracting spectral information via Fourier transforms. The solution of the time-dependent…

We propose a machine learning based approach to develop the exchange-correlation potential of time dependent density functional theory (TDDFT). The neural network projection from the time-varying electron densities to the corresponding…

Computational Physics · Physics 2020-05-20 Yasumitsu Suzuki , Ryo Nagai , Jun Haruyama

We study fusion reactions of the $^{64}$Ni+$^{64}$Ni system using the density-constrained time-dependent Hartree-Fock (TDHF) formalism. In this formalism the fusion barriers are directly obtained from TDHF dynamics. In addition, we…

Nuclear Theory · Physics 2008-11-26 A. S. Umar , V. E. Oberacker

Transition-metal nanoclusters exhibit structural and electronic properties that depend on their size, often making them superior to bulk materials for heterogeneous catalysis. However, their performance can be limited by sulfur poisoning.…

We present results of collisions of $^{90}$Zr+$^{90}$Zr and $^{96}$Zr+$^{96}$Zr obtained within time-dependent density functional theory (TDDFT) extended to superfluid systems, known as time-dependent superfluid local density approximation…

Eigenvalue problems and linear systems of equations involving large symmetric matrices are commonly solved in quantum chemistry using Krylov space methods, such as the Davidson algorithm. The preconditioner is a key component of Krylov…

Chemical Physics · Physics 2024-04-29 Zehao Zhou , Shane M. Parker

Surface energies of metal-based systems are important for determining the Wulff-constructed shapes of metal nanoparticles and understanding the stability. We have developed a coordination number-based model to predict the total energy of…

Materials Science · Physics 2025-06-19 Shyama Charan Mandal , Frank Abild-Pedersen

We propose a scheme for calculation of linear optical response of current-carrying molecular junctions for the case when electronic tunneling through the junction is much faster than characteristic time of external laser field. We discuss…

Mesoscale and Nanoscale Physics · Physics 2008-04-07 Michael Galperin , Sergei Tretiak

Using the framework of nuclear energy density functionals we examine the conditions for single-nucleon localization and formation of cluster structures in finite nuclei. We propose to characterize localization by the ratio of the dispersion…

Nuclear Theory · Physics 2015-06-05 J. -P. Ebran , E. Khan , T. Niksic , D. Vretenar

First-order nonadiabatic coupling matrix elements (fo-NACMEs) are the basic quantities in theoretical descriptions of electronically nonadiabatic processes that are ubiquitous in molecular physics and chemistry. Given the large size of…

Chemical Physics · Physics 2021-05-25 Zikuan Wang , Chenyu Wu , Wenjian Liu

The nuclear fusion is a reaction to form a compound nucleus. It plays an important role in several circumstances in nuclear physics as well as in nuclear astrophysics, such as synthesis of superheavy elements and nucleosynthesis in stars.…

Nuclear Theory · Physics 2016-07-20 K. Hagino , N. Rowley , J. M. Yao

Cluster production plays an important role in heavy-ion collisions at intermediate beam energies, where light nuclei contribute substantially to final-state yields and to other observables that are used to infer the nuclear equation of…

Nuclear Theory · Physics 2026-05-13 Oleh Savchuk , Pawel Danielewicz , William Lynch , Jérôme Margueron

The formation of weakly bound clusters in the hot and dense environment at midrapidity is one of the surprising phenomena observed experimentally in heavy-ion collisions from a low center of mass energy of a few GeV up to a…

Nuclear Theory · Physics 2024-09-20 V. Kireyeu , G. Coci , S. Glaessel , J. Aichelin , C. Blume , E. Bratkovskaya

Theoretical modeling of nucleus-nucleus collision often is based on the nucleus-nucleus potential. One of the advanced methods for constructing this potential is the semi-microscopical double-folding model with the M3Y-Paris NN-forces.…

Nuclear Theory · Physics 2023-07-26 I. I. Gontchar , M. V. Chushnyakova

Time-Dependent Density Functional Theory (TDDFT) has recently been extended to describe many-body open quantum systems (OQS) evolving under non-unitary dynamics according to a quantum master equation. In the master equation approach,…

Chemical Physics · Physics 2015-05-18 David G. Tempel , Mark A. Watson , Roberto Olivares-Amaya , Alán Aspuru-Guzik

Background: The time-dependent Hartree-Fock (TDHF) theory has been successful in describing low-energy heavy ion collisions. Recently, we have shown that multinucleon transfer processes can be reasonably described in the TDHF theory…

Nuclear Theory · Physics 2014-12-24 Kazuyuki Sekizawa , Kazuhiro Yabana
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