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Imaginary-time time-dependent Density functional theory (it-TDDFT) has been proposed as an alternative method for obtaining the ground state within density functional theory (DFT) which avoids some of the difficulties with convergence…

Computational Physics · Physics 2021-11-09 John McFarland , Efstratios Manousakis

Time-dependent density functional theory (TDDFT) is a standard approach for calculating optical excitations of molecules and solids, while ensemble DFT (EDFT) is a promising alternative under development. We introduce ensemble TDDFT…

Chemical Physics · Physics 2026-05-22 Kimberly J. Daas , Steven Crisostomo , Kieron Burke

A mixed quantum-classical approach to simulate the coupled dynamics of electrons and nuclei in nanoscale molecular systems is presented. The method relies on a second order expansion of the Lagrangian in time-dependent density functional…

Chemical Physics · Physics 2009-11-10 T. A. Niehaus , D. Heringer , B. Torralva , Th. Frauenheim

The saddle-to-scission dynamics of the induced fission process is explored using a microscopic finite-temperature model based on time-dependent nuclear density functional theory (TDDFT), that allows to follow the evolution of local…

Nuclear Theory · Physics 2023-07-27 B. Li , D. Vretenar , Z. X. Ren , T. Nikšić , J. Zhao , P. W. Zhao , J. Meng

The formation of correlated structures is of importance in many diverse contexts such as strongly coupled plasmas, soft matter, and even biological mediums. In all these contexts the dynamics are mainly governed by electrostatic…

Plasma Physics · Physics 2023-06-07 Mamta Yadav , Priya Deshwal , Srimanta Maity , Amita Das

We propose a computationally efficient approach to the nonadiabatic time-dependent density functional theory (TDDFT) which is based on a representation of the frequency-dependent exchange correlation kernel as a response of a set of damped…

Mesoscale and Nanoscale Physics · Physics 2019-12-18 Dmitry R. Gulevich , Yaroslav V. Zhumagulov , Alexei V. Vagov , Vasili Perebeinos

Quantum embedding methods have recently developed significantly to model large molecular structures. This work proposes a novel wave function theory in density functional theory (WTF-in-DFT) embedding scheme based on pair-coupled cluster…

Chemical Physics · Physics 2024-01-10 Rahul Chakraborty , Katharina Boguslawski , Paweł Tecmer

The theoretical understanding of plasmon behavior is crucial for an accurate interpretation of inelastic scattering diagnostics in many experiments. We highlight the utility of linear-response time-dependent density functional theory…

Materials Science · Physics 2021-03-17 Kushal Ramakrishna , Attila Cangi , Tobias Dornheim , Andrew Baczewski , Jan Vorberger

The electric dipole (E1) strength functions have been systematically calculated based on the time-dependent density functional theory (TDDFT), using the finite amplitude method and the real-time approach to the TDDFT with pairing…

Nuclear Theory · Physics 2017-08-23 Shuichiro Ebata , Tsunenori Inakura , Takashi Nakatsukasa

Fragmentation dynamics in the Coulomb explosion of hydrocarbons, specifically methane, ethane, propane, and butane, are investigated using time dependent density functional theory (TDDFT) simulations. The goal of this work is to elucidate…

Chemical Physics · Physics 2024-10-11 Samuel S. Taylor , Kálmán Varga , Károly Mogyorósi , Viktor Chikán , Cody Covington

In this paper we demonstrate the performance of several density-based methods in predicting the inversion of S$_1$ and T$_1$ states of a few N-heterocyclic fused ring molecules (popularly known as INVEST molecules) with an eye to identify a…

Chemical Physics · Physics 2024-08-12 Shamik Chanda , Subhasish Saha , Sangita Sen

We report on a general method for the calculation of the frequency-dependent optical response of clusters based upon time-dependent density functional theory (TDDFT). The implementation is done using explicit propagation in the time domain…

Materials Science · Physics 2009-11-07 Argyrios Tsolakidis , Daniel Sanchez-Portal , Richard M. Martin

We demonstrate that the microscopic Time-dependent Hartree-Fock (TDHF) theory provides an important approach to shed light on the nuclear dynamics leading to the formation of superheavy elements. In particular, we discuss studying…

Nuclear Theory · Physics 2017-12-06 A. S. Umar , C. Simenel , S. Ayik

The entrance-channel mass-asymmetry dependence of the compound nucleus formation time in light heavy-ion reactions has been investigated within the framework of semiclassical dissipative collision models. the model calculations have been…

Nuclear Theory · Physics 2009-09-25 A. Szanto de Toledo , B. V. Carlson , C. Beck , M. Thoenessen

Following a previous paper [Y. Shi, Phys. Rev. C 98, 014329(2018)], we present an extension of the density-functional theory to allow for dynamic calculations based on the obtained static Hartree-Fock results. We perform extensive benchmark…

Nuclear Theory · Physics 2020-11-04 Yue Shi , Nobuo Hinohara , Bastian Schuetrumpf

To understand the true origin of flowlike signatures and applicability of hydrodynamics in small collision systems, effects of soft QCD dynamics, the sensitivity of jetlike correlations, and nonequilibrium effects, efforts are being made to…

High Energy Physics - Phenomenology · Physics 2023-09-18 Debadatta Behera , Suraj Prasad , Neelkamal Mallick , Raghunath Sahoo

Motivated by TeV-scale neutrino mass models, we propose a systematic treatment of heavy neutrino $(N)$ production at hadron colliders. Our simple and efficient modeling of the vector boson fusion (VBF) $W^\pm\gamma\rightarrow N\ell^\pm$ and…

High Energy Physics - Phenomenology · Physics 2016-09-14 Celine Degrande , Olivier Mattelaer , Richard Ruiz , Jessica Turner

In the framework of relativistic-mean-field (RMF) models, we investigate the properties of light and heavy $\Lambda$ hyperclusters emersed in nuclear matter at various densities $n_{\mathrm{gas}}$ and proton fractions $Y_p$. In particular,…

Nuclear Theory · Physics 2025-11-04 Cheng-Jun Xia , Yu-Ting Rong , Ting-Ting Sun

Molecular-level understanding of the interactions between the constituents of an atomic structure is essential for designing novel materials in various applications. This need goes beyond the basic knowledge of the number and types of…

The elliptic flow of emitted particles and fragments observed in heavy-ion reactions at high energy has become an important observable reflecting the pressure generated in the dense collision zone. More recently, the strength of the nuclear…

Nuclear Experiment · Physics 2019-08-28 W. Trautmann