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We present the theory, implementation, and benchmarking of a real-time time-dependent density functional theory (RT-TDDFT) module within the RMG code, designed to simulate the electronic response of molecular systems to external…

Atomically precise metal nanoclusters bridge the molecular and bulk regimes, but designing bimetallic motifs with targeted stability and reactivity remains challenging. Here we combine density functional theory (DFT) and physics-grounded…

The formalism of density functional theory (DFT) can be easily extended to the time dependent case (TDDFT). However, while in the static case the theory is well established and is expected to be, at least in principle, an exact approach for…

Condensed Matter · Physics 2007-05-23 Sandro Stringari

Background: Heavy-ion fusion reactions at energies near the Coulomb barrier are influenced by couplings between the relative motion and nuclear intrinsic degrees of freedom of the colliding nuclei. The time-dependent Hartree-Fock (TDHF)…

Nuclear Theory · Physics 2016-03-23 D. Bourgin , C. Simenel , S. Courtin , F. Haas

We present an implementation of time-dependent density-functional theory (TDDFT) in the linear response formalism enabling the calculation of low energy optical absorption spectra for large molecules and nanostructures. The method avoids…

Time-dependent density functional theory (TDDFT) is a widely used method to investigate electron dynamics under external time-dependent perturbations such as laser fields. In this work, we present a machine learning approach to accelerate…

Materials Science · Physics 2025-12-02 Karan Shah , Attila Cangi

A new alternate method for evaluating linear response theory is formally developed, and results are presented. This method involves the time-evolution of the system using TDHF and is constructed directly on top of a static Hartree-Fock…

Nuclear Theory · Physics 2009-11-11 A. S. Umar , V. E. Oberacker

The number and properties of the neutrons and photons emitted in nuclear fission are directly related to the excitation energy of the fission fragments when they are formed at scission. Though not observable experimentally because of the…

Nuclear Theory · Physics 2025-10-09 Antonio Bjelčić , Nicolas Schunck , Marc Verriere

We carried out a simulation of heavy ion collision using a time-dependent density functional theory. We call it the canonical-basis time-dependent Hartree-Fock-Bogoliubov theory (Cb-TDHFB) which can describe nuclear dynamics in…

Nuclear Theory · Physics 2015-06-12 Shuichiro Ebata

In this contribution, current status and future prospects of our ongoing project is summarized. In the inner crust of neutron stars, a variety of crystalline structures may emerge, as a result of competition of Coulomb and nuclear…

Nuclear Theory · Physics 2023-10-11 Kazuyuki Sekizawa , Kenta Yoshimura

Coupling of cluster and deformed structures are important for dynamics of nuclear structure. Threshold energy has been discussed to explain cluster structures coupling to deformed states but relation between threshold energy and excitation…

Nuclear Theory · Physics 2019-06-12 Yasutaka Taniguchi

The nucleonic localization function has been used for a decade to study the formation of alpha-particles in nuclei, by providing a measure of having nucleons of a given spin in a single place. However, differences in interpretation remain,…

Nuclear Theory · Physics 2023-01-11 E. Khan , L. Heitz , F. Mercier , J. -P. Ebran

We present a theoretical description of femtosecond laser induced dynamics of the hydrogen molecule and of singly ionised sodium dimers, based on a real-space, real-time, implementation of time-dependent density functional theory (TDDFT).…

Condensed Matter · Physics 2007-05-23 Alberto Castro , M. A. L. Marques , Julio A. Alonso , George F. Bertsch , Angel Rubio

Using a theory of large amplitude collective motion, the adiabatic self-consistent collective coordinate method, we derive reaction path for the fusion process at sub-barrier energies. The collective Hamiltonian to describe the fusion…

Nuclear Theory · Physics 2019-01-30 Kai Wen , Takashi Nakatsukasa

This chapter provides a basic introduction to excited-state extensions of density functional theory (DFT), including time-dependent (TD-)DFT in both its linear-response and its explicitly time-dependent formulations. As applied to the…

Chemical Physics · Physics 2023-05-02 John M. Herbert

Background: Multinucleon transfer (MNT) and quasifission (QF) processes are dominant processes in low-energy collisions of two heavy nuclei. They are expected to be useful to produce neutron-rich unstable nuclei. Nuclear dynamics leading to…

Nuclear Theory · Physics 2016-05-25 Kazuyuki Sekizawa , Kazuhiro Yabana

We illustrate the formation of a thin-long structure of heavy nuclei by three-nucleus simultaneous collisions within time-dependent density functional theory. The impact parameter dependence for such formation is systematically demonstrated…

Nuclear Theory · Physics 2013-02-19 Yoritaka Iwata , Kei Iida , Naoyuki Itagaki

We analyze the details of mass exchange in the vicinity of the Coulomb barrier for heavy-ion collisions involving neutron-rich nuclei using the time-dependent Hartree-Fock (TDHF) theory. We discuss the time-dependence of transfer and show…

Nuclear Theory · Physics 2008-11-26 A. S. Umar , V. E. Oberacker , J. A. Maruhn

A microscopic mean-field description of heavy ions fusion is performed in the framework of the Time-Dependent Hartree-Fock (TDHF) theory using a Skyrme interaction with the SLy4d parametrization. A good agreement with experiments is…

Nuclear Theory · Physics 2008-03-11 Cédric Simenel , Benoît Avez

Microscopic methods and tools to describe nuclear dynamics have considerably been improved in the past few years. They are based on the time-dependent Hartree-Fock (TDHF) theory and its extensions to include pairing correlations and quantum…

Nuclear Theory · Physics 2018-09-13 C. Simenel , A. S. Umar