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The presence of dynamical heterogeneities, i.e. nanometer-scale regions containing molecules rearranging cooperatively at very different rates compared to the bulk, is increasingly being recognized as crucial in our understanding of the…

Disordered Systems and Neural Networks · Physics 2015-06-25 Horacio E. Castillo , Azita Parsaeian

In this paper we investigate, both analytically and numerically, the emergence of a kinetic glass transition in two different model systems: a uniformly heated granular gas and a molecular fluid with nonlinear drag. Despite the profound…

Soft Condensed Matter · Physics 2024-04-25 A. Patrón , B. Sánchez-Rey , A. Prados

We study bidisperse colloidal suspensions confined within glass microcapillary tubes to model the glass transition in confined cylindrical geometries. We use high speed three-dimensional confocal microscopy to observe particle motions for a…

Soft Condensed Matter · Physics 2013-02-28 Nabiha Saklayen , Gary L. Hunter , Kazem V. Edmond , Eric R. Weeks

Many investigations shed light on various correlations between structure and dynamics in supercooled liquids; however, a general relation between structure and dynamics remains elusive. This molecular dynamics simulation study identifies…

Soft Condensed Matter · Physics 2023-08-16 D. C. Thakur , Sandeep Kushawah , Jalim Singh , Anna Varughese , Prasanth P. Jose

Recent theoretical advances have led to the creation of a unified phase diagram for the thermal glass and athermal jamming transitions. This diagram makes clear that, while related, the mode-coupling---or dynamic---glass transition is…

Soft Condensed Matter · Physics 2017-09-20 Peter Morse , Eric Corwin

The viscosity of glass-forming liquids increases by many orders of magnitude if their temperature is lowered by a mere factor of 2-3 [1,2]. Recent studies suggest that this widespread phenomenon is accompanied by spatially heterogeneous…

Disordered Systems and Neural Networks · Physics 2015-05-28 Walter Kob , Sandalo Roldan-Vargas , Ludovic Berthier

The emergence of nanoscience has increased the importance of experiments able to probe the very local structure of materials, especially for disordered and heterogeneous systems. This is technologically important; for example, the nanoscale…

Soft Condensed Matter · Physics 2015-05-13 R. Casalini , C. M. Roland

We here discuss the results of 3d MonteCarlo simulations of a minimal lattice model for gelling systems. We focus on the dynamics, investigated by means of the time autocorrelation function of the density fluctuations and the particle mean…

Soft Condensed Matter · Physics 2007-05-23 E. Del Gado , A. Fierro , L. de Arcangelis , A. Coniglio

Active glasses refer to a class of driven non-equilibrium systems that share remarkably similar dynamical behavior as conventional glass-formers in equilibrium. Glass-like dynamical characteristics have been observed in various biological…

Soft Condensed Matter · Physics 2024-12-24 Subhodeep Dey , Smarajit Karmakar

The dynamical facilitation scenario, by which localized relaxation events promote nearby relaxation events in an avalanching process, has been suggested as the key mechanism connecting the microscopic and the macroscopic dynamics of…

Soft Condensed Matter · Physics 2015-11-03 Raffaele Pastore , Antonio Coniglio , Massimo Pica Ciamarra

The dynamics of dense particle packings near the jamming transition is characterized by correlated particle motion. The growth of dynamical heterogeneities, or strong spatial variations in the motion of the particles constituting the…

Soft Condensed Matter · Physics 2024-09-12 Rajkumar Biswas , Anoop Mutneja , Smarajit Karmakar , Ranjini Bandyopadhyay

The dynamical arrest of gels is the consequence of a well defined structural phase transition, leading to the formation of a spanning cluster of bonded particles. The dynamical glass transition, instead, is not accompanied by any clear…

Soft Condensed Matter · Physics 2016-07-21 Raffaele Pastore , Antonio de Candia , Anallisa Fierro , Massimo Pica Ciamarra , Antonio Coniglio

We use molecular dynamics computer simulations to investigate the relaxation dynamics of a binary Lennard-Jones liquid confined in a narrow pore. We find that the average dynamics is strongly influenced by the confinement in that time…

Statistical Mechanics · Physics 2009-10-31 Peter Scheidler , Walter Kob , Kurt Binder

The collective behaviour of statistical systems close to critical points is characterized by an extremely slow dynamics which, in the thermodynamic limit, eventually prevents them from relaxing to an equilibrium state after a change in the…

Statistical Mechanics · Physics 2009-07-13 Andrea Gambassi

We analyze data from confocal microscopy experiments of a colloidal suspension to validate predictions of rapid sporadic events responsible for structural relaxation in a glassy sample. The trajectories of several thousand colloidal…

Soft Condensed Matter · Physics 2011-12-08 J. Ariel Rodriguez Fris , Gustavo A. Appignanesi , Eric R. Weeks

Many systems, including polymers and molecular liquids, when adequately cooled and/or compressed, solidify into a disordered solid, i.e., a glass. The~transition is not abrupt, featuring progressive decrease of the microscopic mobility and…

Soft Condensed Matter · Physics 2019-11-19 Francesco Puosi , Antonio Tripodo , Dino Leporini

Driven granular systems readily form glassy phases at high particle volume fractions and low driving amplitudes. We use computer simulations of a driven granular glass to evidence a re-entrance melting transition into a fluid state, which,…

Soft Condensed Matter · Physics 2013-02-19 Jan Plagge , Claus Heussinger

We develop the elastically collective nonlinear Langevin equation theory of bulk relaxation of glass-forming liquids to investigate molecular mobility under compression conditions. The applied pressure restricts more molecular motion and…

Soft Condensed Matter · Physics 2020-04-24 Anh D. Phan , Agnieszka Jedrzejowska , Marian Paluch , Katsunori Wakabayashi

We present molecular dynamics simulations on the slow dynamics of a mixture of big and small soft-spheres with a large size disparity. Dynamics are investigated in a broad range of temperature and mixture composition. As a consequence of…

Soft Condensed Matter · Physics 2009-11-11 Angel J. Moreno , Juan Colmenero

The mode-coupling theory of the glass transition treats the dynamics of supercooled liquids in terms of two-point density correlation functions. Here we consider a generalized, hierarchical formulation of schematic mode-coupling equations…

Statistical Mechanics · Physics 2014-11-27 Liesbeth M. C. Janssen , Peter Mayer , David R. Reichman