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Many nanophotonic applications require precise control and characterization of electromagnetic field properties at the nanoscale. The chiral properties of the field are among its key characteristics, yet measurement of optical chirality at…

Optics · Physics 2022-02-18 Abid Anjum Sifat , Filippo Capolino , Eric O. Potma

We propose a gain-assisted enantioselective scheme in dye-doped chiral particles, demonstrating optical pulling and pushing forces that can be tuned using externally controllable parameters. By controlling the concentration of dye molecules…

We introduce a microscopy technique that facilitates the prediction of spatial features of chirality of nanoscale samples by exploiting photo-induced optical force exerted on an achiral tip in the vicinity of the test specimen. The…

Inspired by a sea creature, we identify a robust chiral optical force that pushes the opposite enantiomers of a chiral molecule towards regions of orthogonal linear polarization in an optical field via electric dipole interactions. Our…

Optical forces can be chiral when they exhibit opposite signs for the two enantiomeric versions of a chiral molecule or particle. Such forces could be eventually used to separate enantiomers, which could find application in numerous…

The recently introduced synthetic chiral light [D. Ayuso et al, Nat. Photon. 13, 866-871 (2019)] has opened up new opportunities for ultrafast and highly efficient imaging and control of chiral matter. Here we show that the giant…

Chemical Physics · Physics 2022-05-18 David Ayuso

We propose a theoretical method for enantio-discrimination based on the light deflection effect in four-level models of chiral molecules. This four-level model consists of a cyclic three-level subsystem coupled by three strong driving…

Optics · Physics 2020-08-12 Yu-Yuan Chen , Chong Ye , Quansheng Zhang , Yong Li

We put forward an enantioselective method for chiral nanoparticles using optical tweezers. We demonstrate that the optical trapping force in a typical, realistic optical tweezing setup with circularly-polarized trapping beams is sensitive…

Optics · Physics 2019-11-07 R. Ali , F. A. Pinheiro , F. S. S. Rosa , R. S. Dutra , P. A. Maia Neto

Optical fields can exert forces of chiral nature on molecules and nanoparticles, which would prove extremely valuable in the separation of enantiomers with pharmaceutical applications, yet it is inherently complex, and the varied frameworks…

The topological response of matter to electromagnetic fields is a property in high demand in materials design and metrology due to its robustness against noise and decoherence, stimulating recent advances in ultrafast photonics. Embedding…

Nanoscopic observation of chiro-optical phenomena is essential in wide scientific areas but has measurement difficulties; hence, its physics are still unknown. Currently, in most cases, chiro-optical phenomena have been investigated by…

Optics · Physics 2023-08-21 Junsuke Yamanishi , Hyo-Yong Ahn , Hiromi Okamoto

Enantiodetection of chiral molecules is important to pharmaceutical drug production, chemical reaction control, and biological function designs. Traditional optical methods of enantiodetection rely on the weak magnetic-dipole or…

Chemical Physics · Physics 2022-09-14 Mao-Rui Cai , Chong Ye , Hui Dong , Yong Li

Today we are witnessing the electric-dipole revolution in chiral measurements. Here we reflect on its lessons and outcomes, such as the perspective on chiral measurements using the complementary principles of "chiral reagent" and "chiral…

Optics · Physics 2022-11-30 David Ayuso , Andres F. Ordonez , Olga Smirnova

We derived an analytical formula for the optical force acting on a small anisotropic chiral particle. The behavior of chiral particles is qualitatively different from achiral particles due to new chirality dependent terms which couple…

Optics · Physics 2015-06-16 Kun Ding , Jack Ng , Lei Zhou , C. T. Chan

Optical enantioseparation of nanoscale matter is fundamentally limited by the intrinsic weakness of chiroptical forces compared to the dominant achiral gradient forces and thermal fluctuations. Conventional plasmonic approaches typically…

Optics · Physics 2026-02-11 Guillermo Serrera , Pablo Albella

Chiroptical techniques for detecting and characterizing the chirality of matter and artificial nanostructures are traditionally based on their interaction with chiral light, typically circularly-polarized fields propagating in free space.…

Chiral near fields possessing enhanced asymmetry (superchirality), created by the interaction of light with (chiral) nanostructures, potentially provide a route to novel sensing and metrology technologies for biophysical applications.…

Enantio-conversion with the help of electromagnetic fields is an essential issue due to the chirality-dependence of many chemical, biological, and pharmaceutical processes. Here, we propose a method for this issue based on a five-level…

Quantum Physics · Physics 2021-03-03 Chong Ye , Bo Liu , Yu-Yuan Chen , Yong Li

Up to now, in the literature of optical manipulation, optical force due to chirality usually coexists with the non-chiral force and the chiral force usually takes a very small portion of the total force. In this work, we investigate a case…

Chiral optical forces exhibit opposite signs for the two enantiomeric versions of a chiral molecule or particle. If large enough, these forces might be able to separate enantiomers all optically, which would find numerous applications in…

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