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Drawing inspiration from a remarkable chiral force found in nature, we show that a static electric field combined with an optical lin$\perp$lin polarization standing wave can exert a chiral optical force on a small chiral molecule that is…

Optics · Physics 2023-08-16 Robert P. Cameron , Duncan McArthur , Alison M. Yao

We calculate optical forces and torques exerted on a chiral dipole by chiral light fields and reveal genuinely chiral forces in combining the chiral contents of both light field and dipolar matter. Here, the optical chirality is…

Modern optical nano-elements pursue ever-smaller sizes and individualized functionalities. Those elements that can efficiently manipulate the magnetic field of light boast promising future applications with a great challenge: the magnetic…

Circular Dichroism (CD) can distinguish the handedness of chiral molecules. However, it is typically very weak due to vanishing absorption at low molecular concentrations. Here, we suggest Thermal Circular Dichroism (TCD) for chiral…

Optics · Physics 2024-07-19 Ershad Mohammadi , Giulia Tagliabue

We put forward a novel, twofold scheme that enables at the same time all-optical enantioselection and sorting of single multipolar chiral microspheres based on optical pulling forces exerted by two non-collinear, nonstructured,…

Optics · Physics 2021-03-04 R. Ali , R. S. Dutra , F. A. Pinheiro , P. A. Maia Neto

We propose an enantioselective scheme to sort homogeneous chiral particles using optical tweezers. For a certain range of material parameters, we show that a highly focused circularly-polarized laser beam traps particles of a specific…

Optics · Physics 2023-07-19 R. Ali , F. A. Pinheiro , R. S. Dutra , F. S. S. Rosa , P. A. Maia Neto

Chiroptical enantioselective sensing is gaining traction across various applications. However, intrinsic molecular chiroptical responses are weak, and existing amplification approaches add synthesis, manufacturing, or operational complexity…

Chiral discrimination that is efficient to tiny amounts of chiral substances, especially at the single-molecule level, is highly demanded. Here, we propose a single-shot nondestructive quantum sensing method addressing such an issue. Our…

Quantum Physics · Physics 2023-10-05 Chong Ye , Yifan Sun , Yong Li , Xiangdong Zhang

Enantiodetection is an important and challenging task across natural science. Nowadays, some chiroptical methods of enantiodetection based on decoherence-free cyclic three-level models of chiral molecules can reach the ultimate limit of the…

Quantum Physics · Physics 2022-11-29 Chong Ye , Xiaowei Mu , Yifan Sun , Libin Fu , Xiangdong Zhang

Enantioselective interactions of chiral molecules include distinct absorptions to opposite-handed circularly polarized light, known as chiral absorption. Traditionally, chiral absorption has been primarily attributed to electric dipole and…

Optics · Physics 2024-06-03 Hanwei Wang , Yang Zhao

Strong light-matter coupling in chiral cavities has been proposed as an effective way to selectively interact with an enantiomer that shares the same handedness as the cavity's chiral mode. We show that surface plasmons supported by a…

Chiral nanophotonic structures have garnered considerable interest in recent years due to their potential to enhance the efficacy of chirality-sensitive biomolecular detection. Designing metaplatforms to enhance chiroptical signals under…

When light illuminates the junction formed between a sharp metal tip and a sample, different mechanisms can con-tribute to the measured photo-induced force simultaneously. Of particular interest are the instantaneous force be-tween the…

We present a unified description of several methods of chiral discrimination based exclusively on electric-dipole interactions. It includes photoelectron circular dichroism (PECD), enantio-sensitive microwave spectroscopy (EMWS),…

Atomic Physics · Physics 2019-01-02 Andres F. Ordonez , Olga Smirnova

Chiral discrimination, a problem of vital importance, has recently become an emerging frontier in ultrafast physics, with remarkable progress achieved in multiphoton and strong-field regimes. Rydberg excitations, unavoidable in the…

We predict a discriminatory interaction between a chiral molecule and an achiral molecule which is mediated by a chiral body. To achieve this, we generalize the van der Waals interaction potential between two ground-state molecules with…

Quantum Physics · Physics 2017-05-19 Pablo Barcellona , Hassan Safari , A. Salam , Stefan Yoshi Buhmann

We show that the optical force exerted on a finite size chiral sphere by a surface plasmon mode has a component along a direction perpendicular to the plasmon linear momentum. We reveal how this chiral lateral force, pointing in opposite…

Optics · Physics 2016-01-20 Antoine Canaguier-Durand , Cyriaque Genet

Developing effective methods to measure the enantiomeric excess of the chiral mixture is one of the major topics in chiral molecular researches, yet remains challenging. Enantiodetection method via two-dimensional (2D) spectroscopy based on…

Chemical Physics · Physics 2023-05-05 Mao-Rui Cai , Chong Ye , Yong Li , Hui Dong

Sculpting sub-cycle temporal structures of optical waveforms allows one to image and even control electronic clouds in atoms, molecules and solids. Here we show how the transverse spin component arising upon spatial confinement of such…

Optics · Physics 2020-11-17 David Ayuso , Andres Ordonez , Misha Ivanov , Olga Smirnova

Transverse spin angular momentum (SAM) of light and associated transverse chiral optical forces have received tremendous attention recently as the latter may lead to an optical separation of chiral biomolecules. In this context, the…

Optics · Physics 2016-11-03 M. H. Alizadeh , B. M. Reinhard