Related papers: AC Stark Effect in Ultracold Polar RbCs Molecules
By leveraging the hyperfine interaction between the rotational and nuclear spin degrees of freedom, we demonstrate extensive magnetic control over the electric dipole moments, electric dipolar interactions, and ac Stark shifts of…
Cold and ultracold polar molecules with nonzero electronic angular momentum are of great interest for studies in quantum chemistry and control, investigations of novel quantum systems, and precision measurement. However, in mixed electric…
The ac Stark shift (or light shift) of the 6$^{2}$S$_{1/2}$ (F $=$ 3 $\leftrightarrow $ 4) transition in $^{133}$Cs, as observed through coherent population trapping under pulsed excitation, is measured using a $^{133}$Cs gas cell and the…
We suggest that Bose-Einstein condensates in optical lattices subjected to ac forcing with a smooth envelope may provide detailed experimental access to multiphoton-like transitions between ac-Stark-shifted Bloch bands. Such transitions…
We present a non-perturbative numerical technique for calculating strong light shifts in atoms under the influence of multiple optical fields with arbitrary polarization. We confirm our technique experimentally by performing spectroscopy of…
We present precision spectroscopy on electrically trapped formaldehyde (H$_2$CO), demonstrating key attributes which will enable molecular spectroscopy with unprecedented precision. Our method makes use of a microstructured electric trap…
Precise measurement of the particle number, spatial distribution and internal state is fundamental to all proposed experiments with ultracold molecules both in bulk gases and optical lattices. Here, we demonstrate in-situ detection of…
We demonstrate electrical control of the A-exciton interband transition in mono- and few-layer $MoS_{2}$ crystals embedded into photocapacitor devices via the DC Stark effect. Electric field dependent low-temperature photoluminescence…
Trapping ultracold molecules in conservative traps is essential for applications -- such as quantum state-controlled chemistry, quantum simulations, and quantum information processing. These applications require high densities or…
We propose a scheme for state-insensitive trapping of neutral atoms by using light with two independent wavelengths. In particular, we describe the use of trapping and control lasers to minimize the variance of the potential experienced by…
We report on a method for measuring ac Stark shifts observed in stored light experiments while simultaneously determining the energetic splitting between the electronic ground states involved in the two-photon transition. To this end we…
We prepare mixtures of ultracold CaF molecules and Rb atoms in a magnetic trap and study their inelastic collisions. When the atoms are prepared in the spin-stretched state and the molecules in the spin-stretched component of the first…
We perform one- and two-photon high resolution spectroscopy on ultracold samples of RbCs Feshbach molecules with the aim to identify a suitable route for efficient ground-state transfer in the quantum-gas regime to produce quantum gases of…
Heavy polar molecules can be used to measure the electric dipole moment of the electron, which is a sensitive probe of physics beyond the Standard Model. The value is determined by measuring the precession of the molecule's spin in a plane…
We theoretically study collisions between ultracold polar molecules that are polarized by microwave or static electric fields. We systematically study the dependence on field strength, microwave polarization, and detuning from rotational…
Rotational transitions of $iso$-propyl cyanide, (CH$_3$)$_2$CHCN, also known as $iso$-butyronitrile, were recorded using long-path absorption spectroscopy in selected regions between 37 and 600 GHz. Further measurements were carried out…
We explore the rich internal structure of Cs_2 Feshbach molecules. Pure ultracold molecular samples are prepared in a CO_2-laser trap, and a multitude of weakly bound states is populated by elaborate magnetic-field ramping techniques. Our…
The ac Stark shift of hyperfine levels of neutral atoms can be calculated using the third order perturbation theory(TOPT), where the third order corrections are quadratic in the atom-photon interaction and linear in the hyperfine…
The static and dynamic electric-dipole polarizabilities and tune-out wavelengths for the ground state of Cs atoms are calculated by using a semiempirical relativistic configuration interaction plus core polarization approach. By considering…
We report the observation of microwave coherent control of rotational states of ultracold $^{85}$Rb$^{133}$Cs molecules formed in their vibronic ground state by short-range photoassociation. Molecules are formed in the single rotational…