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Related papers: Unconventional spin dynamics in the honeycomb-latt…

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We present comprehensive electron spin resonance (ESR) studies of in-plane oriented single crystals of $\alpha$-RuCl$_3$, a quasi-two-dimensional material with honeycomb structure, focusing on its high-field spin dynamics. The measurements…

High-frequency ESR results on the S=1/2 Heisenberg hexagonal antiferromagnet InCu2/3V1/3O3 are reported. This compound appears to be a rare model substance for the honeycomb lattice antiferromagnet with very weak interlayer couplings. The…

Strongly Correlated Electrons · Physics 2015-03-17 Susumu Okubo , Hideo Wada , Hitoshi Ohta , Takahiro Tomita , Masashi Fujisawa , Takahiro Sakurai , Eiji Ohmichi , Hikomitsu Kikuchi

We report a $^{35}$Cl nuclear magnetic resonance study in the honeycomb lattice, $\alpha$-RuCl$_3$, a material that has been suggested to potentially realize a Kitaev quantum spin liquid (QSL) ground state. Our results provide direct…

Strongly Correlated Electrons · Physics 2017-07-26 S. -H. Baek , S. -H. Do , K. -Y. Choi , Y. S. Kwon , A. U. B. Wolter , S. Nishimoto , Jeroen van den Brink , B. Büchner

The Kitaev quantum spin liquid (KSL) is a theoretically predicted state of matter whose fractionalized quasiparticles are distinct from bosonic magnons, the fundamental excitation in ordered magnets. The layered honeycomb antiferromagnet…

We report a muon spin rotation/relaxation ($\mu$SR) study of single-crystalline samples of the $\alpha$-RuCl$_3$ honeycomb magnet, which is presumed to be a model compound for the Kitaev-Heisenberg interaction. It is inferred from magnetic…

We report an electron spin resonance (ESR) study of the s=1/2-Heisenberg pseudo-ladder magnet CaCu2O3 in pulsed magnetic fields up to 40 T. At sub-Terahertz frequencies we observe an ESR signal originating from a small amount of…

Strongly Correlated Electrons · Physics 2009-11-11 M. Goiran , M. Costes , J. M. Broto , F. C. Chou , R. Klingeler , E. Arushanov , S. -L. Drechsler , B. Büchner , V. Kataev

Mott insulators with strong spin-orbit coupling have been proposed to host unconventional magnetic states, including the Kitaev quantum spin liquid. The 4$d$ system $\alpha$-RuCl$_3$ has recently come into view as a candidate Kitaev system,…

Using quantum chemistry calculations we shed fresh light on the electronic structure and magnetic properties of RuCl3, a proposed realization of the honeycomb Kitaev spin model. It is found that the nearest-neighbor Kitaev exchange K is…

Strongly Correlated Electrons · Physics 2017-01-19 Ravi Yadav , Nikolay A. Bogdanov , Vamshi M. Katukuri , Satoshi Nishimoto , Jeroen van den Brink , Liviu Hozoi

The material $\alpha$-RuCl$_3$, with a two-dimensional Ru-honeycomb sublattice, has attracted considerable attention because it may be a realization of the Kitaev quantum spin liquid (QSL). Recently, a new honeycomb material,…

Strongly Correlated Electrons · Physics 2022-02-08 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Elbio Dagotto

The pursuit of quantum spin liquid (QSL) in the Kitaev honeycomb magnets has drawn intensive attention recently. In particular, $\alpha$-RuCl$_3$ has been widely recognized as a promising candidate for the Kitaev QSL. Although the compound…

Strongly Correlated Electrons · Physics 2023-03-29 Han Li , Wei Li , Gang Su

High-resolution thermal expansion and magnetostriction measurements were performed on single crystals of $\alpha$-RuCl$_3$ in magnetic fields applied parallel to the Ru-Ru bonds. The length changes were measured in the direction…

The local magnetic properties of Yb$^{3+}$ in the layered honeycomb material YbCl$_{3}$ were investigated by electron spin resonance on single crystals. For in-plane and out-of-plane field orientations the $g$-factor shows a clear…

Strongly Correlated Electrons · Physics 2023-08-15 Jörg Sichelschmidt , Ellen Häußler , Ekaterina Vinokurova , M. Baenitz , Thomas Doert

In $\alpha$-RuCl$_3$, an external magnetic field applied within the honeycomb plane can induce a transition from a magnetically ordered state to a disordered state that is potentially related to the Kitaev quantum spin liquid. In zero…

The Kitaev model predicts that quantum spin liquids (QSLs) will form at low temperatures under certain special conditions, and materials hosting the QSL state are frequently sought. The layered honeycomb lattice material {\alpha}-RuCl3 has…

Materials Science · Physics 2022-01-24 Danrui Ni , Xin Gui , Kelly M. Powderly , R. J. Cava

YbOCl is a representative member of the van der Waals layered honeycomb rare-earth chalcohalide REChX (RE = rare earth, Ch = O, S, Se, and Te, and X = F, Cl, Br, and I) family reported recently. Its spin ground state remains to be explored…

Strongly Correlated Electrons · Physics 2024-09-13 Zheng Zhang , Yanzhen Cai , Jinlong Jiao , Jing Kang , Dehong Yu , Bertrand Roessli , Anmin Zhang , Jianting Ji , Feng Jin , Jie Ma , Qingming Zhang

Novel ground states might be realized in honeycomb lattices with strong spin-orbit coupling. Here we study the electronic structure of ${\alpha}$-RuCl$_3$, in which the Ru ions are in a d5 configuration and form a honeycomb lattice, by…

Strongly Correlated Electrons · Physics 2016-09-21 A. Koitzsch , C. Habenicht , E. Mueller , M. Knupfer , B. Buechner , H. Kandpal , J. van den Brink , D. Nowak , A. Isaeva , Th. Doert

Cu2(pymca)3(ClO4) (pymca: pyrimidine-2-carboxylate) consists of a slightly distorted honeycomb lattice of Cu2+ spins, which shows no long-range magnetic order down to 0.6 K. A magnetization study revealed 1/3 and 2/3 plateau phases [A.…

Strongly Correlated Electrons · Physics 2025-08-11 Masaaki Matsuda , Alexander I. Kolesnikov , Zentaro Honda , Tokuro Shimokawa , Sho Inoue , Yasuo Narumi , Masayuki Hagiwara

The low-temperature magnetic phases in the layered honeycomb lattice material $\alpha$-RuCl$_3$ have been studied as a function of in-plane magnetic field. In zero field this material orders magnetically below 7 K with so-called zigzag…

Strongly Correlated Electrons · Physics 2017-06-07 J. A. Sears , Y. Zhao , Z. Xu , J. W. Lynn , Young-June Kim

$^7$Li nuclear magnetic resonance (NMR) and terahertz (THz) spectroscopies are used to probe magnetic excitations and their field dependence in the hyperhoneycomb Kitaev magnet $\beta$-Li$_2$IrO$_3$. Spin-lattice relaxation rate ($1/T_1$)…

Strongly Correlated Electrons · Physics 2020-06-16 M. Majumder , M. Prinz-Zwick , S. Reschke , A. Zubtsovskii , T. Dey , F. Freund , N. Büttgen , A. Jesche , I. Kézsmárki , A. A. Tsirlin , P. Gegenwart

We investigate the effects of hydrostatic pressure on $\alpha$-RuCl$_3$, a prototypical material for the Kitaev spin model on a honeycomb lattice with a possible spin-liquid ground state. Using ultrasound measurements at pressures up to…

Strongly Correlated Electrons · Physics 2025-03-07 A. Hauspurg , Susmita Singh , T. Yanagisawa , V. Tsurkan , J. Wosnitza , Wolfram Brenig , Natalia B. Perkins , S. Zherlitsyn
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