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We present confocal microscopy studies of novel particle-stabilized emulsions. The novelty arises because the immiscible fluids have an accessible upper critical solution temperature. The emulsions have been created by beginning with…

Soft Condensed Matter · Physics 2009-11-11 P. S. Clegg , E. M. Herzig , A. B. Schofield , T. S. Horozov , B. P. Binks , M. E. Cates , W. C. K. Poon

We present a quantitative confocal-microscopy study of the transient and final microstructure of particle-stabilised emulsions formed via demixing in a binary liquid. To this end, we have developed an image-analysis method that relies on…

Soft Condensed Matter · Physics 2010-11-04 Job H J Thijssen , Paul S Clegg

The stability of shapes formed by three viscoelastic droplets during their arrested coalescence has been investigated using micromanipulation experiments. Addition of a third droplet to arrested droplet doublets is shown to be controlled by…

Particle stabilized emulsions have received an enormous interest in the recent past, but our understanding of the dynamics of emulsion formation is still limited. For simple spherical particles, the time dependent growth of fluid domains is…

Soft Condensed Matter · Physics 2015-02-10 Florian Günther , Stefan Frijters , Jens Harting

Motivated by the buckling of glassy crusts formed on evaporating droplets of polymer and colloid solutions, we numerically model the deformation and buckling of spherical elastic caps controlled by varying the volume between the shell and…

Materials Science · Physics 2009-11-11 D. A. Head

The issue of the stability of Pickering emulsions is tackled at a mesoscopic level using dissipative particle dynamics simulations within the Adiabatic Biased Molecular Dynamics framework. We consider the early stage of the coalescence…

Soft Condensed Matter · Physics 2017-02-08 François Sicard , Alberto Striolo

We study the thermodynamics of binary mixtures with the volume fraction of the minority component less than the amount required to form a flat interface and show that the surface tension dominated equilibrium phase of the mixture forms a…

Soft Condensed Matter · Physics 2023-03-07 Subhadip Biswas , Biswaroop Mukherjee , Buddhapriya Chakrabarti

Recent large-scale computer simulations suggest that it may be possible to create a new class of soft solids, called `bijels', by stabilizing and arresting the bicontinuous interface in a binary liquid demixing via spinodal decomposition…

Soft Condensed Matter · Physics 2007-12-14 E. M. Herzig , K. A. White , A. B. Schofield , W. C. K. Poon , P. S. Clegg

Micro- and nanogels are widely used to stabilise emulsions and simultaneously implement their responsiveness to the external stimuli. One of the factors that improves the emulsion stability is the nanogel softness. Here, we study how the…

Soft Condensed Matter · Physics 2023-02-08 Alexander V. Petrunin , Steffen Bochenek , Walter Richtering , Andrea Scotti

Forming an interface between immiscible fluids incurs a free-energy cost that usually favors minimizing the interfacial area. An emulsion droplet of fixed volume therefore tends to form a sphere, and pairs of droplets tend to coalesce.…

Soft Condensed Matter · Physics 2025-04-15 Jatin Abacousnac , Wenjun Chen , Jasna Brujic , David G. Grier

The freeze-thaw cycling of particle-stabilised emulsions can alter the emulsion structure and stability. This could have significant consequences for using particle stabilisation in industrial applications where increased stability is…

Soft Condensed Matter · Physics 2019-02-25 Katy L. Dickinson , Ulrich K. Wiegand , Job H. J. Thijssen

Particle-stabilised emulsions are a cornerstone of soft matter science due to their broad application and fundamental relevance. Computer simulations provide key insights into the formation and behaviour of these emulsions, yet current…

Soft Condensed Matter · Physics 2026-02-19 Elisabeth C. Eij , Joost de Graaf , Martin F. Haase , Jesse M. Steenhoff

Droplet-based microfluidics has emerged as a powerful technology for the miniaturization and automation of biochemical assays. The replacement of surfactants by nanoparticles as interfacial stabilizers has gained increasing interest.…

Soft Condensed Matter · Physics 2019-06-21 Laura Andreina Chacon Orellana , Jean-Christophe Baret

We introduce a new experimental approach to study the structural transitions of large numbers of nanoparticle-coated droplets as their volume is reduced. We use an emulsion system where the dispersed phase is slightly soluble in the…

Soft Condensed Matter · Physics 2012-09-28 Sujit S. Datta , Ho Cheung Shum , David A. Weitz

Nanostructured materials formed via kinetically controlled self-assembly processes gather more interest nowadays. Bicontinuous emulsion gels stabilized by colloidal particles, called bijels, are attractive materials in soft-matter as they…

Drying of biologically-relevant sessile droplets, including passive systems (like DNA and proteins), as well as active microbial systems comprising bacteria and algae, have garnered considerable attention over the last decades. Distinct…

Soft Condensed Matter · Physics 2023-11-07 Anusuya Pal , Amalesh Gope , Anupam Sengupta

Protein-stabilised emulsions can be seen as mixtures of unadsorbed proteins and of protein-stabilised droplets. To identify the contributions of these two components to the overall viscosity of sodium caseinate o/w emulsions, the…

Soft Condensed Matter · Physics 2019-01-30 Marion Roullet , Paul S. Clegg , William J. Frith

The stable configurations formed by two viscoelastic, ellipsoid-shaped droplets during their arrested coalescence has been investigated using micromanipulation experiments. Ellipsoidal droplets are produced by millifluidic emulsification of…

Soft Condensed Matter · Physics 2018-08-14 Chen Hao , Zhaoyu Xie , Timothy J. Atherton , Patrick T. Spicer

Emulsion fuels have the potential to reduce both particulate matter and NOx emissions and can potentially improve the efficiency of combustion engines. However, their limited stability remains a critical barrier to practical use as an…

Carefully tuned composite materials can have properties wholly unlike their separate constituents. We review the development of one example: colloid-stabilized emulsions with bicontinuous liquid domains. These non-equilibrium structures…

Soft Condensed Matter · Physics 2008-02-25 P. S. Clegg
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