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Bicontinuous Pickering emulsions (bijels) are a physically interesting class of soft materials with many potential applications including catalysis, microfluidics and tissue engineering. They are created by arresting the spinodal…

Soft Condensed Matter · Physics 2022-03-07 M. Reeves , J. H. J. Thijssen

Biomolecular condensates are small droplets forming spontaneously in biological cells via phase separation. They play a role in many cellular processes, but it is unclear how cells control them. Cellular regulation often relies on…

Soft Condensed Matter · Physics 2024-03-15 Jan Kirschbaum , David Zwicker

We consider an emulsion whose droplets contain a trapped species (insoluble in the continuous phase), and study the emulsion's stability against coarsening via Lifshitz-Slyozov dynamics (Ostwald Ripening). Extending an earlier treatment by…

Soft Condensed Matter · Physics 2007-05-23 A. J. Webster , M. E. Cates

Biolasers made of biological materials have attracted a great of research attention due to their biocompatibility and biodegradability, which have the potential for biosensors and biointegration. However, the current fabrication method of…

Using controlled spinodal decomposition, we have created a fluid-bicontinuous structure stabilized by colloidal particles. We present confocal microscopy studies of these structures and their variation with kinetic pathway. Our studies…

Soft Condensed Matter · Physics 2007-06-13 P. S. Clegg , E. M. Herzig , A. B. Schofield , S. U. Egelhaaf , T. S. Horozov , B. P. Binks , M. E. Cates , W. C. K. Poon

This study explores the stabilization mechanisms of concentrated emulsions with tunable morphology using amphiphilic polymer-grafted nanoparticles (PGNPs). We employ coarse-grained molecular simulations to investigate concentrated…

Soft Condensed Matter · Physics 2024-10-24 Kojiro Suzuki , Yusei Kobayashi , Takashi Yamazaki , Toshikazu Tsuji , Noriyoshi Arai

Liquid-liquid phase separation is important across biology, physics, and materials science. Although usually studied at equilibrium, active components - such as motor proteins, enzymes, and synthetic microswimmers - are increasingly…

Soft Condensed Matter · Physics 2026-01-06 Kan Chang , Yulin Li , Ming Yuan , Masaki Sano , Zhihong You , H. P. Zhang

We propose an approach to measure surface elastic constants of soft solids. Generally, this requires one to probe interfacial mechanics at around the elastocapillary length scale, which is typically microscopic. Deformations of microscopic…

Soft Condensed Matter · Physics 2022-03-02 Stefanie Heyden , Petia M. Vlahovska , Eric R. Dufresne

In this study, we analyze the various arrangements that droplets can form within dispersed buoyant emulsions, which we refer to as the study of microstructure. To this end, we have developed a novel algorithm that effectively prevents…

Fluid Dynamics · Physics 2024-07-11 Nicolas Fintzi , Jean-Lou Pierson , Stéphane Popinet

The aggregation of protein-stabilised emulsions leads to the formation of emulsion gels. These soft solids are classically envisioned as droplet-filled matrices. Here however, it is assumed that protein-coated sub-micron droplets contribute…

Soft Condensed Matter · Physics 2020-10-06 Marion Roullet , Paul S. Clegg , William J. Frith

We demonstrate that the formation of bicontinuous emulsions stabilized by interfacial particles (bijels) is more robust when nanoparticles rather than microparticles are used. Emulsification via spinodal demixing in the presence of nearly…

Soft Condensed Matter · Physics 2015-09-30 M. Reeves , A. T. Brown , A. B. Schofield , M. E. Cates , J. H. J. Thijssen

Protein nanoparticles have been proven to be highly effective stabilizers of water-in-water emulsions obtained from a number of different types of aqueous two-phase systems (ATPS). The stabilizing efficiency of such particles is attributed…

Soft Condensed Matter · Physics 2025-02-14 Andrzej Balis , Georgi Gochev , Domenico Truzzolillo , Dawid Lupa , Liliana Szyk-Warszynska , Jan Zawala

Bicontinuous, interfacially jammed emulsion gels (bijels) represent a class of soft solid materials in which interpenetrating domains of two immiscible fluids are stabilized by an interfacial colloidal monolayer. Such structures can be…

Soft Condensed Matter · Physics 2011-01-18 E. Kim , K. Stratford , M. E. Cates

The issue of the buckling mechanism in droplets stabilized by solid particles (armored droplets) is tackled at a mesoscopic level using dissipative particle dynamics simulations. We consider spherical water droplet in a decane solvent…

Soft Condensed Matter · Physics 2017-02-10 François Sicard , Alberto Striolo

Protein-stabilised emulsion gels can be studied in the theoretical framework of colloidal gels, because both protein assemblies and droplets may be considered as soft colloids. These particles differ in their nature, size and softness, and…

Soft Condensed Matter · Physics 2020-07-10 Marion Roullet , Paul S. Clegg , William J. Frith

Conventional phase segregation is controlled by a positive interfacial tension, which implies that the system relaxes towards a state in which the interfacial area (or length) is minimized, typically manifesting as a single droplet that…

Soft Condensed Matter · Physics 2025-09-24 Kathrin Hertäg , Joshua F. Robinson , Thomas Speck

Producing food-grade soft particles with controlled structure is of interest to elucidate the structure-properties relationship in soft-particles suspensions. The aim of this work is to evaluate the ability of two elaboration processes to…

Soft Condensed Matter · Physics 2022-06-30 Alban Lacroix , Murielle Hayert , Veronique Bosc , Paul Menut

Porous materials possess numerous useful functions because of their high surface area and ability to modulate the transport of heat, mass, fluids, and electromagnetic waves. Unlike highly ordered structures, disordered porous structures…

Soft Condensed Matter · Physics 2022-11-21 Tiancheng Wang , Robert A. Riggleman , Daeyeon Lee , Kathleen J. Stebe

We demonstrate that emulsion droplets stabilized by interfacial particles become unstable beyond a size threshold set by gravity. This holds not only for colloids but supra-colloidal glass beads, using which we directly observe the ejection…

Soft Condensed Matter · Physics 2012-11-26 Joe W. Tavacoli , Gijs Katgert , E. Grace Kim , Michael E. Cates , Paul S. Clegg

Bacterial attachment to a fluid interface can lead to the formation of a film with physicochemical properties that evolve with time. We study the time evolution of interface (micro)mechanics for interfaces between oil and bacterial…

Soft Condensed Matter · Physics 2015-03-26 Liana Vaccari , Daniel Allan , Nima Sharifi-Mood , Aayush Singh , Robert Leheny , Kathleen Stebe