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Kitaev materials often order magnetically at low temperatures due to the presence of non-Kitaev interactions. Torque magnetometry is a very sensitive technique for probing the magnetic anisotropy, which is critical in understanding the…

Strongly Correlated Electrons · Physics 2024-12-17 John S. Pearce , David A. S. Kaib , Zeyu Ma , Danrui Ni , R. J. Cava , Roser Valenti , Radu Coldea , Amalia I. Coldea

The Kitaev spin liquid, a ground state of the bond-dependent Kitaev model in a honeycomb lattice has been a centre of attraction, since a microscopic theory to realize such an interaction in solid-state materials was discovered. A challenge…

Strongly Correlated Electrons · Physics 2022-05-20 Jiefu Cen , Hae-Young Kee

The magnetic field response of the Mott-insulating honeycomb iridate Na$_{2}$IrO$_{3}$ is investigated using torque magnetometry measurements in magnetic fields up to 60 tesla. A peak-dip structure is observed in the torque response at…

Magnetic dilution of a well-established Kitaev candidate system is realized in the substitutional Ru$_{1-x}$Rh$_x$Cl$_3$ series ($x = 0.02-0.6$). Optimized syntheses protocols yield uniformly-doped single crystals and polycrystalline…

Strongly Correlated Electrons · Physics 2023-01-10 G. Bastien , E. Vinokurova , M. Lange , K. K. Bestha , L. T. Corredor , G. Kreutzer , A. Lubk , Th. Doert , B. Buchner , A. Isaeva , A. U. B. Wolter

Magnetism in strongly correlated honeycomb systems with $d^5$ electronic configuration has garnered significant attention due to its potential to realize the Kitaev spin liquid state, characterized by exotic properties. However, real…

Strongly Correlated Electrons · Physics 2025-11-18 Ritwik Das , Indra Dasgupta

Single layer $\alpha$-ruthenium trichloride ($\rm\alpha-RuCl_3$) has been proposed as a potential quantum spin liquid. Graphene/$\rm RuCl_3$ heterobilayers have been extensively studied with a focus on the large interlayer electron transfer…

Strongly Correlated Electrons · Physics 2023-08-02 Jingtian Shi , A. H. MacDonald

The so-called "Kitaev candidate" materials based on $4d^5$ and $5d^5$ metals have recently emerged as magnetic systems displaying strongly anisotropic exchange interactions reminiscent of the Kitaev's honeycomb model. Recently, these…

Strongly Correlated Electrons · Physics 2019-05-17 Kira Riedl , Ying Li , Stephen M. Winter , Roser Valenti

Thermomagnetic and inelastic neutron scattering measurements on Na2PrO3 are reported. This material is an antiferromagnetic honeycomb magnet based on the tetravalent lanthanide Pr4+ and has been proposed to host dominant antiferromagnetic…

Strongly Correlated Electrons · Physics 2021-03-17 Marcus J. Daum , Arun Ramanathan , Alexander I. Kolesnikov , Stuart A. Calder , Martin Mourigal , Henry S. La Pierre

We investigate the thermal Hall effect in a Kitaev-Heisenberg system, a model for Kitaev candidate $\alpha$-RuCl$_3$, in the presence of the coupling between spin and phonon arising from chlorine atoms' vibration. We observe that the…

Strongly Correlated Electrons · Physics 2022-07-27 Shaozhi Li , Satoshi Okamoto

We study the nature of the debated thermal Hall effect in the candidate Kitaev material $\alpha$-RuCl$_3$. Without assuming the existence of a gapped spin liquid, we show that a realistic minimal spin model in the canted zigzag phase…

Strongly Correlated Electrons · Physics 2023-01-27 Shuyi Li , Han Yan , Andriy H. Nevidomskyy

Insulating quantum magnets lie at the forefront both of fundamental research into quantum matter and of technological exploitation in the increasingly applied field of spintronics. In this context, the magnetic thermal transport is a…

Strongly Correlated Electrons · Physics 2020-01-22 Christopher A. Pocs , Ian A. Leahy , Hao Zheng , Gang Cao , Eun-Sang Choi , S. -H. Do , Kwang-Yong Choi , B. Normand , Minhyea Lee

In the pursuit of developing routes to enhance magnetic Kitaev interactions in {\alpha}-RuCl3, as well as probing doping effects, we investigate the electronic properties of {\alpha}-RuCl3 in proximity to graphene. We study…

Strongly Correlated Electrons · Physics 2019-12-11 Sananda Biswas , Ying Li , Stephen M. Winter , Johannes Knolle , Roser Valenti

Topological states of matter such as quantum spin liquids (QSLs) are of great interest because of their remarkable predicted properties including protection of quantum information and the emergence of Majorana fermions. Such QSLs, however,…

$\alpha$-RuCl$_{3}$ is a major candidate for the realization of the Kitaev quantum spin liquid, but its zigzag antiferromagnetic order at low temperatures indicates deviations from the Kitaev model. We have quantified the spin Hamiltonian…

We provide analytical and numerical insights into the phase diagram and other properties of the extended Kitaev-Heisenberg model on the honeycomb lattice in the {\it easy-plane} limit, in which interactions are only between spin components…

Strongly Correlated Electrons · Physics 2023-01-20 P. A. Maksimov , A. L. Chernyshev

The low-temperature magnetic phases in the layered honeycomb lattice material $\alpha$-RuCl$_3$ have been studied as a function of in-plane magnetic field. In zero field this material orders magnetically below 7 K with so-called zigzag…

Strongly Correlated Electrons · Physics 2017-06-07 J. A. Sears , Y. Zhao , Z. Xu , J. W. Lynn , Young-June Kim

The discovery of ordered magnetism in two-dimensional van der Waals materials at the monolayer limit challenges the Mermin-Wagner theorem, which forbids spontaneous breaking of continuous symmetries in two dimensions at finite temperatures.…

$\alpha$-RuCl$_3$ has been extensively studied recently because of potential bond-dependent Kitaev magnetic exchange interactions and the resulting quantum spin liquid phase that can be realized therein. It has been known that the covalency…

Strongly Correlated Electrons · Physics 2022-01-13 Heung-Sik Kim

We present a theoretical study of field-induced magnetic phases in the honeycomb Kitaev-Heisenberg model, which is believed to describe the essential physics of Mott insulators with strong spin-orbit coupling such as $A_2$IrO$_3$ and…

Strongly Correlated Electrons · Physics 2017-04-26 Gia-Wei Chern , Yuriy Sizyuk , Craig Price , Natalia B. Perkins

Motivated by recent experiments on $\alpha$-RuCl$_3$, we investigate a possible quantum spin liquid ground state of the honeycomb-lattice spin model with bond-dependent interactions. We consider the $K-\Gamma$ model, where $K$ and $\Gamma$…

Strongly Correlated Electrons · Physics 2018-02-15 Matthias Gohlke , Gideon Wachtel , Youhei Yamaji , Frank Pollmann , Yong Baek Kim