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We study the rare-earth magnets on a honeycomb lattice, and are particularly interested in the experimental consequences of the highly anisotropic spin interaction due to the spin-orbit entanglement. We perform a high-temperature series…

Strongly Correlated Electrons · Physics 2020-10-06 Zhu-Xi Luo , Gang Chen

Searching for Kitaev quantum spin liquid (QSL) is a fascinating and challenging problem. Much effort has been devoted to honeycomb lattice candidates with strong spin-orbit coupling in 5d-electron iridates and 4delectron RuCl3. Recently,…

Strongly Correlated Electrons · Physics 2021-10-20 L. Y. Shi , X. M. Wang , R. D. Zhong , Z. X. Wang , T. C. Hu , S. J. Zhang , Q. M. Liu , T. Dong , F. Wang , N. L. Wang

We report on the results of 23Na NMR in the honeycomb lattice magnet Na2Co2TeO6 which has been nominated as a Kitaev material. Measurements of magnetic shift and width of the NMR line as functions of temperature and magnetic field show that…

Strongly Correlated Electrons · Physics 2022-12-21 Jun Kikuchi , Takayuki Kamoda , Nobuyoshi Mera , Yodai Takahashi , Kouji Okumura , Yukio Yasui

The layered honeycomb iridate $\alpha$-Li$_2$IrO$_3$ displays an incommensurate magnetic structure with counterrotating moments on nearest-neighbor sites, proposed to be stabilized by strongly-frustrated anisotropic Kitaev interactions…

Strongly Correlated Electrons · Physics 2019-03-06 Sungkyun Choi , S. Manni , J. Singleton , C. V. Topping , T. Lancaster , S. J. Blundell , D. T. Adroja , V. Zapf , P. Gegenwart , R. Coldea

Detailed magnetization, specific heat, and $^7$Li nuclear magnetic resonance (NMR) measurements on single crystals of the hyperhoneycomb Kitaev magnet $\beta$-Li$_2$IrO$_3$ are reported. At high temperatures, {\cred anisotropy of the…

Strongly Correlated Electrons · Physics 2019-07-30 M. Majumder , F. Freund , T. Dey , M. Prinz-Zwick , N. Büttgen , Y. Skourski , A. Jesche , A. A. Tsirlin , P. Gegenwart

A polymorph of RuI$_3$ synthesized under high pressure was found to have a two-layered honeycomb structure. The resistivity of RuI$_3$ exhibits a semimetallic behavior, in contrast to insulating properties in $\alpha$-RuCl$_3$. In addition,…

In the quest for realizations of quantum spin liquids, the exploration of Kitaev materials - spin-orbit entangled Mott insulators with strong bond-directional exchanges - has taken center stage. However, in these materials the local…

Ruthenium trichloride is the subject of many recent experimental and theoretical studies. Johnson et al. infer a candidate for the magnetic structure (Cc2/m) from results gathered in an extensive set of experiments on an untwined sample of…

Strongly Correlated Electrons · Physics 2022-11-01 S W Lovesey

The Mott insulator $\alpha$-RuCl$_3$ has generated great interest in the community due to its possible field-induced Kitaev quantum spin liquid state. Despite enormous effort spent trying to obtain the form of the low energy Hamiltonian,…

Spin-phonon coupling, the interaction of spins with surrounding lattice is a key parameter to understand the underlying physics of multiferroics and engineer their magnetization dynamics. Elementary excitations in multiferroic materials are…

Materials Science · Physics 2020-11-05 Bommareddy Poojitha , Anjali Rathore , Ankit Kumar , Surajit Saha

We discuss magnetically ordered states, arising in Heisenberg-Kitaev and related spin models, on three-dimensional (3D) harmonic honeycomb lattices. For large classes of ordered states, we show that they can be mapped onto two-dimensional…

Strongly Correlated Electrons · Physics 2020-01-29 Wilhelm G. F. Krüger , Matthias Vojta , Lukas Janssen

Material realization of the non-Abelian Kitaev spin liquid phase - an example of Ising topological order (ITO) - has been the subject of intense research in recent years. The $4d$ honeycomb Mott insulator $\alpha$-RuCl$_3$ has emerged as a…

Strongly Correlated Electrons · Physics 2021-02-26 Jacob S. Gordon , Hae-Young Kee

We report low-temperature (down to $\sim$5 K) Raman signatures of the recently discovered intercalated honeycomb magnet Ag$_3$LiIr$_2$O$_6$, a putative Kitaev quantum spin liquid (QSL) candidate. The Kitaev QSL is predicted to host Majorana…

Strongly Correlated Electrons · Physics 2022-07-05 Srishti Pal , Vinod Kumar , Debendra Prasad Panda , A. Sundaresan , Avinash V. Mahajan , D. V. S. Muthu , A. K. Sood

We report a $^{35}$Cl nuclear magnetic resonance (NMR) study of the diluted Kitaev material $\alpha$-Ru$_{1-x}$Ir$_x$Cl$_3$ ($x=0.1$ and $0.2$) where non-magnetic Ir$^{3+}$ dopants substitute Ru$^{3+}$ ions. Upon dilution, the $^{35}$Cl…

Strongly Correlated Electrons · Physics 2020-09-16 Seung-Ho Baek , Hyeon Woo Yeo , Seung-Hwan Do , Kwang-Yong Choi , Lukas Janssen , Matthias Vojta , Bernd Büchner

We show that the topological Kitaev spin liquid on the honeycomb lattice is extremely fragile against the second-neighbor Kitaev coupling $K_2$, which has recently been shown to be the dominant perturbation away from the nearest-neighbor…

Strongly Correlated Electrons · Physics 2015-12-08 Ioannis Rousochatzakis , Johannes Reuther , Ronny Thomale , Stephan Rachel , N. B. Perkins

Na2Co2TeO6 is a proposed approximate Kitaev magnet, yet its actual magnetic interactions are elusive due to a lack of knowledge on the full excitation spectrum. Here, using inelastic neutron scattering and single crystals, we determine the…

Strongly Correlated Electrons · Physics 2022-10-04 Weiliang Yao , Kazuki Iida , Kazuya Kamazawa , Yuan Li

Motivated by the growing interest in spin liquids and topological phases, as well as the rise of deformation engineering, we study the combined effects of deformation and magnetic fields on the honeycomb Kitaev model. The Kitaev model, as…

Strongly Correlated Electrons · Physics 2026-05-20 Abdullah AlJishi , Ali AlSwaid , Moayad Ekhwan , Hocine Bahlouli , Raditya Weda Bomantara , Michael Vogl

To study the relationship between the properties of low-dimensional spin systems with weakly coupled Cu-triangles and their crystal structure, single crystals of $Cs_3Cu_3Cl_8OH$ (1) and the new $Cs_3Cu_3Cl_{7.6}Br_{0.4}OH$ (2) were grown.…

$\alpha$-RuCl$_3$ is a Mott insulator with a honeycomb lattice with strong spin-orbit coupling. We report dielectric measurements on $\alpha$-RuCl$_3$ single crystals under field. At zero field, the dielectric constant, $\epsilon$, drops…

Strongly Correlated Electrons · Physics 2018-02-20 Jia-Cheng Zheng , Yi Cui , Tian-Run Li , Ke-Jing Ran , Jinsheng Wen , Weiqiang Yu

As a candidate Kitaev material, Na$_2$Co$_2$TeO$_6$ exhibits intriguing magnetism on a honeycomb lattice that is believed to be $C_3$-symmetric. Here we report a neutron diffraction study of high quality single crystals under $a$-axis…

Strongly Correlated Electrons · Physics 2023-06-06 Weiliang Yao , Yang Zhao , Yiming Qiu , Christian Balz , J. Ross Stewart , Jeffrey W. Lynn , Yuan Li
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