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$\alpha$-RuCl$_3$ has been studied extensively because of its proximity to the Kitaev quantum-spin-liquid (QSL) phase and the possibility of approaching it by tuning the competing interactions. Here we present the first polarized inelastic…

We apply the numerical linked cluster expansion (NLCE) to study thermodynamic properties of the proximate Kitaev magnet $\alpha$-RuCl$_3$ on the honeycomb lattice in the presence of a magnetic field. Using the extended spin-1/2…

Strongly Correlated Electrons · Physics 2026-05-05 Alexander Schwenke , Wolfram Brenig

We report the discovery of an intriguing pressure-driven phase transformation in the layered Kitaev-material $\alpha$-RuCl$_3$. By analyzing both the Bragg scattering as well as the diffuse scattering of high-quality single crystals, we…

Strongly Correlated Electrons · Physics 2022-09-20 Quirin Stahl , Tobias Ritschel , Gaston Garbarino , Frederico Cova , Anna Isaeva , Thomas Doert , Jochen Geck

In recent years, the increasing level of control over van der Waals (vdW) heterostructures has opened new routes to tune the properties of quantum materials. Motivated by these developments, we examine the potential consequences of…

Strongly Correlated Electrons · Physics 2026-03-17 Pedro M. Cônsoli , Ezra Day-Roberts , Johannes Knolle , Antia S. Botana , Onur Erten

Maximizing the ratio between Kitaev and residual Heisenberg interactions is a major goal in nowadays research on Kitaev-Heisenberg quantum magnets. Here we investigate Kitaev-Heisenberg exchange in a recently discovered crystalline phase of…

Strongly Correlated Electrons · Physics 2023-12-15 Pritam Bhattacharyya , Liviu Hozoi , Quirin Stahl , Jochen Geck , Nikolay A. Bogdanov

Pressure evolution of the crystal structure and magnetism of the honeycomb $\alpha$-RuBr$_3$ is studied using high-pressure x-ray diffraction, magnetometry, and density-functional band-structure calculations. Hydrostatic compression…

We present initial Raman spectroscopy experiments on exfoliated flakes of $\alpha$-RuCl$_3$, from tens of nm thick down to single layers. Besides unexpectedly finding this material to be air stable, in the thinnest layers we observe the…

Strongly Correlated Electrons · Physics 2019-12-11 Boyi Zhou , Yiping Wang , Gavin B. Osterhoudt , Paige Kelly , David Mandrus , Rui He , Kenneth S. Burch , Erik A. Henriksen

$\alpha$-RuCl$_3$ is a leading material for proximate Kitaev magnetism. We address the origin of the broad, $\Gamma$-point centered excitation continuum observed by inelastic neutron scattering at elevated temperatures in this compound.…

Materials Science · Physics 2026-02-12 Chaebin Kim , Martin Mourigal

Raman spectroscopy together with density functional calculations were used to study lattice dynamics in a layered honeycomb cobaltite Na$_3$Co$_2$SbO$_6$, which can host a field-induced phase related with the Kitaev physics. We show that…

Strongly Correlated Electrons · Physics 2024-05-10 Yu. S. Ponosov , E. V. Komleva , E. A. Pankrushina , D. Mikhailova , S. V. Streltsov

Fine-tuning chemistry by doping with transition metals enables new perspectives for exploring Kitaev physics on a two-dimensional (2D) honeycomb lattice of {\alpha}-RuCl3, which is promising in the field of quantum information protection…

A new-type structural transition has been found in Li2RuO3 with honeycomb lattice of edge-sharing RuO6-octahedra. With decreasing temperature T, the electrical resistivity exhibits an anomalous increase at T=Tc~540 K, suggesting the (metal…

Strongly Correlated Electrons · Physics 2015-06-25 Yoko Miura , Yukio Yasui , Masatoshi Sato , Naoki Igawa , Kazuhisa Kakurai

We report on THz, infrared reflectivity and transmission experiments for wave numbers from 10 to 8000 cm$^{-1}$ ($\sim$ 1 meV - 1 eV) and for temperatures from 5 to 295 K on the Kitaev candidate material {\alpha}-RuCl$_3$. As reported…

Strongly Correlated Electrons · Physics 2017-10-18 S. Reschke , F. Mayr , Zhe Wang , Seung-Hwan Do , K. -Y. Choi , A. Loidl

Intensive studies of the interplay between spin-orbit coupling (SOC) and electronic correlations in transition metal compounds have recently been undertaken. In particular, $j_{\rm eff}$ = 1/2 bands on a honeycomb lattice provide a pathway…

Strongly Correlated Electrons · Physics 2015-06-24 Heung-Sik Kim , V. Vijay Shankar , Andrei Catuneanu , Hae-Young Kee

The spin-orbit assisted Mott insulator $\alpha$-RuCl3 is proximate to the coveted quantum spin liquid (QSL) predicted by the Kitaev model. In the search for the pure Kitaev QSL, reducing the dimensionality of this frustrated magnet by…

The fractionalization of elementary excitations in quantum spin systems is a central theme in current condensed matter physics. The Kitaev honeycomb spin model provides a prominent example of exotic fractionalized quasiparticles, composed…

Strongly Correlated Electrons · Physics 2016-09-21 A. Glamazda , P. Lemmens , S. -H. Do , Y. S. Choi , K. -Y. Choi

Magnetic insulators in the regime of strong spin-orbit coupling exhibit intriguing behaviors in external magnetic fields, reflecting the frustrated nature of their effective interactions. We review the recent advances in understanding the…

Strongly Correlated Electrons · Physics 2019-07-30 Lukas Janssen , Matthias Vojta

We report a comprehensive single-crystal neutron diffraction investigation of the Kitaev quantum magnet $\alpha$-RuCl$_{3}$ under hydrostatic pressure. Utilizing a He-gas pressure cell, we successfully applied an ideal hydrostatic pressure…

Strongly Correlated Electrons · Physics 2023-04-04 Xiao Wang , Fengfeng Zhu , Navid Qureshi , Ketty Beauvois , Junda Song , Thomas Mueller , Thomas Brückel , Yixi Su

The insulating honeycomb magnet $\alpha$-RuCl$_{3}$ exhibits fractionalized excitiations that signal its proximity to a Kitaev quantum spin liquid (QSL) state, however, at $T=0$, fragile long-range magnetic order arises from non-Kitaev…

Strongly Correlated Electrons · Physics 2017-12-12 P. Lampen-Kelley , A. Banerjee , A. A. Aczel , H. B. Cao , M. B. Stone , C. A. Bridges , J. -Q. Yan , S. E. Nagler , D. Mandrus

Topologically ordered states of matter are generically characterized by excitations with quantum number fractionalization. A prime example is the spin liquid realized in Kitaev's honeycomb-lattice compass model where spin-flip excitations…

Strongly Correlated Electrons · Physics 2018-11-12 C. Wellm , J. Zeisner , A. Alfonsov , A. U. B. Wolter , M. Roslova , A. Isaeva , T. Doert , M. Vojta , B. Büchner , V. Kataev

A range of honeycomb-lattice compounds has been proposed and investigated in the search for a topological Kitaev spin liquid. However, sizable Heisenberg interactions and additional symmetry-allowed exchange anisotropies in the magnetic…

Strongly Correlated Electrons · Physics 2018-10-18 Ravi Yadav , Stephan Rachel , Liviu Hozoi , Jeroen van den Brink , George Jackeli