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Fractionalized excitations are of considerable interest in recent condensed-matter physics. Fractionalization of the spin degrees of freedom into localized and itinerant Majorana fermions are predicted for the Kitaev spin liquid, an exactly…

Strongly Correlated Electrons · Physics 2019-03-18 S. Widmann , V. Tsurkan , D. A. Prishchenko , V. G. Mazurenko , A. A. Tsirlin , A. Loidl

We report magnetization and neutron diffraction studies on crystal and magnetic structures of Ir- and Rh-substituted honeycomb lattice $\alpha$-RuCl$_3$. The iridium or rhodium atoms are distributed at the Ru site with little structural…

Materials Science · Physics 2023-10-05 Zachary Morgan , Iris Ye , Colin L. Sarkis , Xiaoping Wang , Stephen Nagler , Jiaqiang Yan

The honeycomb Kitaev model in a magnetic field is a source of a topological quantum spin liquid with Majorana fermions and gauge flux excitations as fractional quasiparticles. We present experimental results for the thermal Hall effect of…

Strongly Correlated Electrons · Physics 2019-03-06 Richard Hentrich , Maria Roslova , Anna Isaeva , Thomas Doert , Wolfram Brenig , Bernd Büchner , Christian Hess

In this work, we study magnetoelastic interactions by means of ultrasound experiments in $\alpha$-RuCl$_3$ -- a prototypical material for the Kitaev spin model on the honeycomb lattice, with a possible spin-liquid state featuring Majorana…

Strongly Correlated Electrons · Physics 2023-03-17 A. Hauspurg , S. Zherlitsyn , T. Helm , V. Felea , J. Wosnitza , V. Tsurkan , K. -Y. Choi , S. -H. Do , Mengxing Ye , Wolfram Brenig , Natalia B. Perkins

The honeycomb Kitaev-Heisenberg model is a source of a quantum spin liquid with Majorana fermions and gauge flux excitations as fractional quasiparticles. In the quest of finding a pertinent material, $\alpha$-RuCl$_{3}$ recently emerged as…

The ruthenium halide $\alpha$-RuCl$_{3}$ is a promising candidate for a Kitaev spin liquid. However, the microscopic model describing $\alpha$-RuCl$_{3}$ is still debated partly because of a lack of analogue materials for…

The honeycomb compound $\alpha$-RuCl$_3$ is widely discussed as a proximate Kitaev spin-liquid material. This scenario builds on spin-orbit entangled $j = 1/2$ moments arising for a $t_{2g}^5$ electron configuration with strong spin-orbit…

Strongly Correlated Electrons · Physics 2020-10-21 P. Warzanowski , N. Borgwardt , K. Hopfer , T. C. Koethe , P. Becker , V. Tsurkan , A Loidl , M. Hermanns , P. H. M. van Loosdrecht , M. Grüninger

The honeycomb Mott insulator $\alpha$-RuCl$_3$ loses its low-temperature magnetic order by pressure. We report clear evidence for a dimerized structure at $P>1$ GPa and observe the breakdown of the relativistic $j_{\rm eff}$ picture in this…

The majority of research on $\alpha$-RuCl$_3$ has focused on applying in-plane magnetic fields to suppress antiferromagnetic order and induce a quantum spin liquid (QSL). However, this effort has been complicated by the materials…

Strongly Correlated Electrons · Physics 2026-05-14 Hamza Nasir Daniel Balazs , Muhammad Nauman , Ezekiel Horsley , Subin Kim , Young-June Kim , K. A. Modic

The sample quality of the hyperhoneycomb lattice Kitaev magnet $\beta$-ZnIrO$_3$ was successfully improved by removing the maximum amount of moisture from the reaction ampoule. The X-ray diffraction structural analysis of the high-quality…

Strongly Correlated Electrons · Physics 2023-10-24 Yuya Haraguchi , Hiroko Aruga Katori

A quantum spin-liquid might be realized in $\alpha$-RuCl$_{3}$, a honeycomb-lattice magnetic material with substantial spin-orbit coupling. Moreover, $\alpha$-RuCl$_{3}$ is a Mott insulator, which implies the possibility that novel exotic…

Novel ground states might be realized in honeycomb lattices with strong spin-orbit coupling. Here we study the electronic structure of ${\alpha}$-RuCl$_3$, in which the Ru ions are in a d5 configuration and form a honeycomb lattice, by…

Strongly Correlated Electrons · Physics 2016-09-21 A. Koitzsch , C. Habenicht , E. Mueller , M. Knupfer , B. Buechner , H. Kandpal , J. van den Brink , D. Nowak , A. Isaeva , Th. Doert

The Kitaev model predicts that quantum spin liquids (QSLs) will form at low temperatures under certain special conditions, and materials hosting the QSL state are frequently sought. The layered honeycomb lattice material {\alpha}-RuCl3 has…

Materials Science · Physics 2022-01-24 Danrui Ni , Xin Gui , Kelly M. Powderly , R. J. Cava

In the search for experimental realizations of bond-anisotropic Kitaev interactions and resulting spin-liquid phases, the layered magnet $\alpha$-RuCl$_3$ is a prime candidate. Its modelling typically involves Heisenberg, Kitaev, and…

Strongly Correlated Electrons · Physics 2020-06-01 Lukas Janssen , Stefan Koch , Matthias Vojta

Recent theoretical studies have suggested that Kitaev physics and such effects as formation of a mysterious spin-liquid state can be expected not only in RuCl3 and iridates, but also in conventional $3d$ transition metal compounds. Using DC…

Strongly Correlated Electrons · Physics 2023-02-22 E. Vavilova , T. Vasilchikova , A. Vasiliev , D. Mikhailova , V. Nalbandyan , E. Zvereva , S. V. Streltsov

The layered honeycomb magnet $\alpha$-RuCl$_3$ is the most promising candidate for a Kitaev quantum spin liquid (KQSL) that can host charge-neutral Majorana fermions. Recent studies have shown significant sample dependence of thermal…

Layered {\alpha}-RuCl3 is a promising material to potentially realize the long-sought Kitaev quantum spin liquid with fractionalized excitations. While evidence of this exotic state has been reported under a modest in-plane magnetic field,…

The honeycomb magnet $\alpha-$RuCl$_3$ is a prime candidate material for realizing the Kitaev quantum spin liquid (QSL), but it shows long-range magnetic order at low temperature. Nevertheless, its broad inelastic neutron scattering (INS)…

Strongly Correlated Electrons · Physics 2022-11-23 Oliver Franke , Dumitru Călugăru , Andreas Nunnenkamp , Johannes Knolle

Inelastic neutron scattering experiments with a large set of comounted Na$_2$IrO$_3$ crystals reveal the low-energy magnon dispersion in this candidate material for Kitaev physics. The magnon gap amounts to 1.7(1) meV and can be interpreted…

Strongly Correlated Electrons · Physics 2026-03-06 Alexandre Bertin , Hengdi Zhao , Gang Cao , Andrea Piovano , Paul Steffens , Alexandre Ivanov , Markus Braden

We report X-ray diffraction and resonant elastic X-ray scattering (REXS) studies on two $\alpha$-RuCl$_{3}$ crystals with distinct magnetic transition temperatures: T$_{N}$=7.3K and 6.5K. We find that the sample with T$_{N}$=6.5K exhibits a…

Strongly Correlated Electrons · Physics 2024-03-08 Subin Kim , Ezekiel Horsley , Christie Nelson , Jacob Ruff , Young-June Kim