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We report a comparative neutron single crystal diffraction study of the structural and magnetic properties of layered halides CrCl$_3$ and $\alpha$-RuCl$_3$, which host a honeycomb arrangement of transition metal ions with distinct…

Strongly Correlated Electrons · Physics 2026-05-13 Zachary Morgan , Iris Ye , Jiasen Guo , Michael A McGuire , Jiaqiang Yan

The layered honeycomb magnet $\alpha$-RuCl$_3$ has attracted intense scrutiny as a prime candidate for realizing the Kitaev quantum spin liquid, yet a consensus on its microscopic Hamiltonian remains elusive due to the material's extreme…

We consider the exchange couplings present in an effective Hamiltonian of $\alpha$-RuCl$_3$, known as the K-$\Gamma$ model. This material has a honeycomb lattice, and is expected to be a representative of the Kitaev materials (which can…

Strongly Correlated Electrons · Physics 2022-04-19 Ipsita Mandal

Mott insulators with strong spin-orbit coupling have been proposed to host unconventional magnetic states, including the Kitaev quantum spin liquid. The 4$d$ system $\alpha$-RuCl$_3$ has recently come into view as a candidate Kitaev system,…

$\alpha$-RuCl$_3$ has been proposed recently as an excellent playground for exploring Kitaev physics on a two-dimensional (2D) honeycomb lattice. However, structural clarification of the compound has not been completed, which is crucial in…

Materials Science · Physics 2016-04-27 Heung-Sik Kim , Hae-Young Kee

The magnetic insulator $\alpha$-RuCl$_{3}$ is a promising candidate to realize Kitaev interactions on a quasi-2D honeycomb lattice. We perform extensive susceptibility measurements on single crystals of $\alpha$-RuCl$_{3}$, including…

Honeycomb lattice Kitaev magnets exhibit exotic magnetic properties governed by the Kitaev interaction. This study delves into $\alpha$-RuCl$_3$, a prototypical example described by effective Hamiltonians encompassing bond-dependent Kitaev…

Strongly Correlated Electrons · Physics 2025-05-29 Hamid Mosadeq , Mohammad-Hossein Zare

Kitaev-type interactions between neighbouring magnetic moments emerge in the honeycomb material ${\alpha}$-RuCl3. It is debated however whether these Kitaev interactions are ferromagnetic or antiferromagnetic. With electron energy loss…

We report X-ray diffraction and magnetic susceptibility studies of the structural phase transition in $\alpha$-RuCl$_{3}$. By utilizing a single crystal sample with predominantly single twin domain, we show that $\alpha$-RuCl$_{3}$ goes…

Strongly Correlated Electrons · Physics 2023-11-08 Subin Kim , Ezekiel Horsley , Jacob P. C. Ruff , Beatriz D. Moreno , Young-June Kim

The combination of electronic correlation and spin-orbit coupling is thought to precipitate a variety of highly unusual electronic phases in solids, including topological and quantum spin liquid states. We report a Raman scattering study…

Strongly Correlated Electrons · Physics 2015-04-22 Luke J. Sandilands , Yao Tian , Kemp W. Plumb , Young-June Kim , Kenneth S. Burch

We report on the unusual behavior of the in-plane thermal conductivity ($\kappa$) and torque ($\tau$) response in the Kitaev-Heisenberg material $\alpha$-RuCl$_3$. $\kappa$ shows a striking enhancement with linear growth beyond H = 7 T,…

Strongly Correlated Electrons · Physics 2017-05-10 Ian A. Leahy , Christopher A. Pocs , Peter E. Siegfried , David Graf , S. -H. Do , Kwang-Yong Choi , B. Normand , Minhyea Lee

We report magnetic and thermodynamic properties of single crystal $\alpha$-RuCl$_3$, in which the Ru$^{3+}$ ($4d^5$) ion is in its low spin state and forms a honeycomb lattice. Two features are observed in both magnetic susceptibility and…

Strongly Correlated Electrons · Physics 2015-04-27 J. A. Sears , M. Songvilay , K. W. Plumb , J. P. Clancy , Y. Qiu , Y. Zhao , D. Parshall , Young-June Kim

We report a muon spin rotation/relaxation ($\mu$SR) study of single-crystalline samples of the $\alpha$-RuCl$_3$ honeycomb magnet, which is presumed to be a model compound for the Kitaev-Heisenberg interaction. It is inferred from magnetic…

We report magnetic, thermodynamic, thermal expansion, and on detailed optical experiments on the layered compound $\alpha$-RuCl$_3$ focusing on the THz and sub-gap optical response across the structural phase transition from the monoclinic…

Strongly Correlated Electrons · Physics 2018-11-09 S. Reschke , F. Mayr , S. Widmann , H. -A. Krug von Nidda , V. Tsurkan , M. V. Eremin , Seung-Hwan Do , K. -Y. Choi , Zhe Wang , A. Loidl

We present first-principles results on the magnetoelastic coupling in $\alpha$-RuCl$_3$ and uncover a striking dependence of the magnetic coupling constants on strain effects. Different magnetic interactions are found to respond very…

Strongly Correlated Electrons · Physics 2021-04-14 David A. S. Kaib , Sananda Biswas , Kira Riedl , Stephen M. Winter , Roser Valenti

We have investigated the longitudinal thermal conductivity of $\alpha$-RuCl$_{3}$, the magnetic state of which is considered to be proximate to a Kitaev honeycomb model, along with the spin susceptibility and magnetic specific heat. We…

Strongly Correlated Electrons · Physics 2017-06-28 Daichi Hirobe , Masahiro Sato , Yuki Shiomi , Hidekazu Tanaka , Eiji Saitoh

We investigate the effects of hydrostatic pressure on $\alpha$-RuCl$_3$, a prototypical material for the Kitaev spin model on a honeycomb lattice with a possible spin-liquid ground state. Using ultrasound measurements at pressures up to…

Strongly Correlated Electrons · Physics 2025-03-07 A. Hauspurg , Susmita Singh , T. Yanagisawa , V. Tsurkan , J. Wosnitza , Wolfram Brenig , Natalia B. Perkins , S. Zherlitsyn

In RuCl$_3$, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the…

The layered compound $\alpha$-RuCl$_3$ is composed of a honeycomb lattice of magnetic Ru$^{3+}$ ions with the $4d^5$ electronic state. We have investigated the magnetic properties of $\alpha$-RuCl$_3$ via magnetization and specific heat…

Strongly Correlated Electrons · Physics 2015-06-24 Yumi Kubota , Hidekazu Tanaka , Toshio Ono , Yasuo Narumi , Koichi Kindo

Single crystals of the Kitaev spin-liquid candidate $\alpha$-RuCl$_3$ have been studied to determine low-temperature bulk properties, structure and the magnetic ground state. Refinements of x-ray diffraction data show that the low…

Strongly Correlated Electrons · Physics 2016-04-27 H. B. Cao , A. Banerjee , J. -Q. Yan , C. A. Bridges , M. D. Lumsden , D. G. Mandrus , D. A. Tennant , B. C. Chakoumakos , S. E. Nagler
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