Related papers: Geometrical optimization approach to isomerization…
We demonstrate how the shape of femtosecond laser pulses can be tailored in order to obtain maximal ionization of atoms or molecules. For that purpose, we have overlayed a direct-optimization scheme on top of a fully unconstrained…
We propose a methodology to design optimal pulses for achieving quantum optimal control on molecular systems. Our approach constrains pulse shapes to linear combinations of a fixed number of experimentally relevant pulse functions. Quantum…
How fast can a laser pulse ionize an atom? We address this question by considering pulses that carry a fixed time-integrated energy per-area, and finding those that achieve the double requirement of maximizing the ionization that they…
Cis-trans isomerization in retinal, the first step in vision, is often computationally studied from a time dependent viewpoint. Motivation for such studies lies in coherent pulsed laser experiments that explore the isomerization dynamics.…
The new capacity of X-ray free-electron laser (XFEL) facilities to produce multi-color X-ray femtosecond pulses paves the way to explore ultrafast phenomena in matter induced by X-ray photons. In the present study, we exploit the site…
Manipulating at will the propagation dynamics of high power laser pulses is a long-standing dream whose accomplishment would lead to the control of a plethora of fascinating physical phenomena emerging from laser-matter interaction. The…
The first step in the coherent control of a photoinduced binary reaction is bond making or photoassociation. We have recently demonstrated coherent control of bond making in multi-photon femtosecond photoassociation of hot magnesium atoms,…
We investigate the potential of numerical algorithms to decipher the kinetic parameters involved in multi-step chemical reactions. To this end we study a dimerization kinetics of protein as a model system. We follow the dimerization…
In this work we studied polymerization-induced self-assembly by means of computer simulations. Using this model, phase diagrams of the micelle states were constructed depending on the polymer concentration and the asymmetry of the…
Recent studies of the dynamically assisted Schwinger effect have shown that particle production is significantly enhanced by a proper choice of the electric field. We demonstrate that optimal control theory provides a systematic means of…
This paper studies a bulk-surface reaction-diffusion system for cell polarization in two-dimensional domains. The model describes the formation of localized patterns through the wave-pinning mechanism, while explicitly incorporating the…
Dipole spin-wave states of atomic ensembles with wave vector ${\bf k}(\omega)$ mismatched from the dispersion relation of light are difficult to access by far-field excitation but may support rich phenomena beyond the traditional…
We investigate computationally a method for ultrafast preparation of alkali metal atoms in their Rydberg states using a three-dimensional model potential in the single active electron approximation. By optimizing laser pulse shapes that can…
A theoretical study of laser and plasma based electron acceleration is presented. An effective model has been used, in which the presence of an underdense plasma has been taken account via its index of refraction $n_{m}$. In the confines of…
For many applications of pulsed radiation, the time-history of the radiation intensity must be optimized to induce a desired time-history of conditions. This optimization is normally performed using multi-physics simulations of the system.…
We proposed a method to engineer the light matter interaction while initializing a qubit in presence of physical constraints utilizing the inverse engineering. Combining the multiple degrees of freedom in the pulse parameters with the…
The possibility of achieving highly selective excitation of low metastable states of hydrogen and helium atoms by using short laser pulses with reasonable parameters is demonstrated theoretically. Interactions of atoms with the laser field…
We consider the formation of cold ground-state polar molecules in a low vibrational level by laser fields. Starting from a pair of cold colliding atoms of dissimilar species, we propose a strategy consisting of three steps. In the first…
We present and discuss a new computationally inexpensive method to study, within the single active electron approximation, the interaction of a complex system with an intense ultrashort laser pulse. As a first application, we consider the…
At the core of attosecond science lies the ability to generate laser pulses of sub-femtosecond duration. In tabletop devices the process relies on high-harmonic generation, where a major challenge is to obtain high yields and high cutoff…