Related papers: Geometrical optimization approach to isomerization…
We propose to create a biexciton by a coherent optical process using a frequency-sweeping (chirped) laser pulse. In contrast to the two-photon Rabi flop scheme, the present method uses the state transfer through avoided level crossing and…
We address the challenge of configuring a fiber laser cavity to enable efficient access to multi-pulse structures such as dissipative soliton molecules. We theoretically compare multi-pulsing routes in the parameter space of the laser. By…
Laser-plasma accelerators offer a compact means of producing high-energy electron beams, but their performance is fundamentally limited by dephasing between the accelerated electrons and the plasma wave. To overcome this limitation, we…
Modeling non-empirical and highly flexible interatomic potential energy surfaces (PES) using machine learning (ML) approaches is becoming popular in molecular and materials research. Training an ML-PES is typically performed in two stages:…
We consider self-pulsing in lasers with a gain section and an absorber section via a mechanism known as Q-switching, as described mathematically by the Yamada ordinary differential equation model for the gain, the absorber and the laser…
The geometric phase (GP) is a fundamental quantum effect arising from conical intersections (CIs), with profound consequences for vibronic energy levels. Standard imaginary-time path integral molecular dynamics (PIMD) based on the…
In reaction path optimization, such as the calculation of a minimum energy path (MEP) between given reactant and product configurations of atoms, it is advantageous to start with an initial guess where close proximity of atoms is avoided…
The process of ionization of a hydrogen atom by a short infrared laser pulse is studied in the regime of very large pulse intensity, in the dipole approximation. Let $A$ denote the integral of the electric field of the pulse over time at…
After an accolade to Joshua Jortner, we trace the influences of his Chemistry background in his Physics writings. On the way, we note the richness of Physics in principles (or large-scale laws) and the fact-orientedness of Chemistry. Next…
A strong inhomogeneous static electric field is used to spatially disperse a supersonic beam of polar molecules, according to their quantum state. We show that the molecules residing in the lowest-lying rotational states can be selected and…
We report our investigation on ultrashort laser pulse optimization using an AI algorithm in a system consisting of a mode-locked oscillator, a spectral phase shaper, and a highly nonlinear amplifier. We analyzed the performance of the pulse…
Preparation of quantum state lies at the heart of quantum information processing. The greedy algorithm provides a potential method to effectively prepare quantum states. However, the standard greedy algorithm, in general, cannot take the…
Ultra-intense laser-matter interaction experiments (>10$^{18}$ W/cm$^{2}$) with dense targets are highly sensitive to the effect of laser "noise" (in the form of pre-pulses) preceding the main ultra-intense pulse. These system-dependent…
Adiabatic pumping is a fundamental concept in the time-dependent transport of mesoscopic devices. To maximize pumping performance, i.e., the amount of pumping per unit time, it is necessary to carefully manage the driving speed, which…
We introduce and implement an interferometric technique based on chirped femtosecond laser pulses and nonlinear optics. The interference manifests as a high-visibility (> 85%) phase-insensitive dip in the intensity of an optical beam when…
Study on a rectified current induced by active particles has received a great attention due to its possible application to a microscopic motor in biological environments. Insertion of an {\em asymmetric} passive object amid many active…
We demonstrate for the first time coherent control of bond making, a milestone on the way to coherent control of photo-induced bimolecular chemical reactions. In strong-field multiphoton femtosecond photoassociation experiments, we find the…
Using three-dimensional kinetic simulations, we examine the emission of collimated gamma-ray beams from structured laser-irradiated targets with a pre-filled cylindrical channel. The channel guides the incident laser pulse, enabling…
In structural optimization, both parameters and shape are relevant for the model performance. Yet, conventional optimization techniques usually consider either parameters or the shape separately. This work addresses this problem by…
Laser-driven plasma accelerators can generate accelerating gradients three orders of magnitude larger than radio-frequency accelerators and have achieved beam energies above 1 GeV in centimetre long stages. However, the pulse repetition…