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The thermodynamic stabilities of various phases of the nitrides of the platinum metal elements are systematically studied using density functional theory. It is shown that for the nitrides of Rh, Pd, Ir and Pt two new crystal structures, in…

Materials Science · Physics 2010-09-03 Daniel Åberg , Babak Sadigh , Jonathan Crowhurst , Alexander F. Goncharov

Ab initio random structure searching with density functional theory was used to determine the zero-temperature structures of atomic metallic hydrogen from 500 GPa to 5 TPa. Including zero point motion in the harmonic approximation, we…

Materials Science · Physics 2015-05-20 Jeffrey M. McMahon , David M. Ceperley

The phase diagram of model anisotropic particles with four attractive patches in a tetrahedral arrangement has been computed at two different values for the range of the potential, with the aim of investigating the conditions under which a…

Materials Science · Physics 2013-06-26 Eva G. Noya , Carlos Vega , Jonathan P. K. Doye , Ard A. Louis

We present results predicting experimentally measurable structural quantities from molecular dynamics studies of hydrogen. In doing this, we propose a paradigm shift for experimentalists -- that the predictions from such calculations should…

Materials Science · Physics 2020-03-25 Graeme J. Ackland , John S. Loveday

The stability of ($R$, Zr)(Fe, Co, Ti)$_{12}$ with a ThMn$_{12}$ structure is investigated using first-principles calculations. We consider energetic competition with multiple phases that have the Th$_2$Zn$_{17}$ structure and the unary…

Materials Science · Physics 2022-03-29 Taro Fukazawa , Yosuke Harashima , Takashi Miyake

Water exhibits rich polymorphism, where more than 20 crystalline phases have been experimentally reported. Five of them are metastable and form at low temperatures by either heating amorphous ice or degassing clathrate hydrates. However,…

A number of transition metal hydrides with close-packed metal sublattices of fcc or hcp structures with hydrogen in octahedral interstitial positions were obtained by the high-pressure hydrogen technique described by Ponyatovskii et al,…

Materials Science · Physics 2014-12-18 Valentina F Degtyareva

According to previous interpretations of experimental data, sodium-scandium double-cation borohydride NaSc(BH$_4$)$_4$ crystallizes in the crystallographic space group $Cmcm$ where each sodium (scandium) atom is surrounded by six scandium…

Materials Science · Physics 2014-04-01 Tran Doan Huan , Maximilian Amsler , Silvana Botti , Miguel A. L. Marques , Stefan Goedecker

Recent breakthroughs in vacancy-ordered double perovskite hydride materials have underscored their significant potential for integration into next-generation high-capacity hydrogen energy storage systems. We perform extensive first…

Materials Science · Physics 2025-07-29 R. Zosiamliana , Lalhriat Zuala , Shivraj Gurung , R. Lalmalsawma , A. Laref , A. Yvaz , D. P. Rai

Based on density functional calculations we predict water ice to attain two new crystal structures with Pbca and Cmcm symmetry at 7.6 and 15.5 Mbar, respectively. The known high pressure ice phases VII, VIII, X, and Pbcm as well as the Pbca…

Materials Science · Physics 2015-05-20 Burkhard Militzer , Hugh F. Wilson

New crystal structures of fully hydrogenated borophene (borophane) have been predicted by first principles calculation. Comparing with the chair-like borophane (C-boropane) that has been reported in literature, we obtained four new…

Materials Science · Physics 2017-05-24 Zhi-Qiang Wang , Tie-Yu Lü , Hui-Qiong Wang , Yuan Ping Feng , Jin-Cheng Zheng

Ternary hydrides have emerged as the primary focus of the new wave of research into superconducting hydrides. In this work, Mg-Ti-H ternary hydrides are explored under high pressures up to 300 GPa using the prediction method of the particle…

Materials Science · Physics 2026-02-10 Pan Min , Wang Yujie , Hu Kaige , Deng Huiqiu

Single crystals of ZrAs1.4Se0.5 (PbFCl type structure) were grown by chemical vapour transport. While their thermodynamic and transport properties are typical for ordinary metals, the electrical resistivity exhibits a shallow minimum at low…

Strongly Correlated Electrons · Physics 2015-06-25 M. Schmidt , T. Cichorek , R. Niewa , A. Schlechte , Y. Prots , F. Steglich , R. Kniep

Using the WIEN2K code, the hydrogen storage capabilities of lithium compositions like LiXH$_3$ (X = Pd, Ag, Cd) hydrides are examined. Structural, electrical, mechanical, thermoelectric, and hydrogen storage properties of these hydrides are…

Materials Science · Physics 2024-12-10 Anupam , Shyam Lal Gupta , Sumit Kumar , Samjeet Singh Thakur , Sanjay Panwar , Diwaker

Compositionally tunable vanadium oxyhydrides Sr2VO4-xHx (x = 0 - 1) without considerable anion vacancy were synthesized by high-pressure solid state reaction. The crystal structures and their properties were characterized by powder neutron…

Density Functional Theory (DFT) calculations, within the virtual crystal alloy approximation, are performed, along with the development of a Landau-type model employing a symmetry-allowed analytical expression of the internal energy and…

The D2O ice VI to ice XV hydrogen ordering phase transition at ambient pressure is investigated in detail with neutron diffraction. The lattice constants are found to be sensitive indicators for hydrogen ordering. The a and b lattice…

Deuteride phases in the zirconium-deuterium system in the temperature range 25-286$\celsius$ have been studied in-situ by high resolution neutron diffraction. The study primarily focused on observations of $\delta \rightarrow \gamma$…

Materials Science · Physics 2017-01-12 T. Maimaitiyili , A. Steuwer , C. Bjerkén , J. Blomqvist , M. Hoelzel , J. C. Ion , O. Zanellato

Following long-standing predictions associated with hydrogen, high-temperature superconductivity has recently been observed in several hydride-based materials. Nevertheless, these high-$T_c$ phases only exist at extremely high pressures,…

Mg$_2$IrH$_6$ is a metastable complex metal hydride with a predicted superconducting transition temperature as high as 170 K at ambient pressure. Following the synthesis of isomorphic, insulating Mg$_2$IrH$_5$ at low pressure,…