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Ultracold polar molecules offer the possibility of exploring quantum gases with interparticle interactions that are strong, long-range, and spatially anisotropic. This is in stark contrast to the dilute gases of ultracold atoms, which have…

Atomic Physics · Physics 2015-05-18 K. -K. Ni , S. Ospelkaus , D. Wang , G. Quemener , B. Neyenhuis , M. H. G. de Miranda , J. L. Bohn , J. Ye , D. S. Jin

High resolution laser Stark excitation of np (60 < n < 85) Rydberg states of ultra-cold cesium atoms shows an efficient blockade of the excitation attributed to long-range dipole-dipole interaction. The dipole blockade effect is observed as…

We probe resonant dipolar interactions between ultracold $^{40}$K$^{87}$Rb molecules and Rydberg $^{87}$Rb atoms in an optically trapped ensemble. Through state-selective ionization detection of the KRb molecules, we observe resonant energy…

Atomic Physics · Physics 2025-04-10 Lingbang Zhu , Jeshurun Luke , Roy Shaham , Yi-Xiang Liu , Kang-Kuen Ni

We show that microwave spectroscopy of a dense Rydberg gas trapped on a superconducting atom chip in the dipole blockade regime reveals directly the dipole-dipole many-body interaction energy spectrum. We use this method to investigate the…

We study the long-range interaction of a single ion with a highly excited ultracold Rydberg atom and report on the direct observation of ion-induced Rydberg excitation blockade mediated over tens of micrometer distances. Our hybrid ion-atom…

Van der Waals interactions are interactions between dipoles. Similarly, quadrupole-quadrupole interactions are interactions between quadrupoles. In this article, we focus on the interactions between two dipoles or two quadrupoles.…

Atomic and Molecular Clusters · Physics 2022-07-18 Jianing Han , Juliet Michell , Morgan Umstead

Optically trapped Rydberg atoms are a suitable platform to explore quantum many-body physics mediated by long-range atom--atom interactions that can be engineered through externally applied light fields. However, this approach is limited to…

We describe a technique for manipulating quantum information stored in collective states of mesoscopic ensembles. Quantum processing is accomplished by optical excitation into states with strong dipole-dipole interactions. The resulting…

Quantum Physics · Physics 2009-11-06 M. D. Lukin , M. Fleischhauer , R. Cote , L. M. Duan , D. Jaksch , J. I. Cirac , P. Zoller

We propose a scheme for controlling interactions between Rydberg-excited neutral atoms in order to perform a fast high-fidelity quantum gate. Unlike dipole-blockade mechanisms already found in the literature, we drive resonantly the atoms…

Quantum Physics · Physics 2009-11-11 M. Cozzini , T. Calarco , A. Recati , P. Zoller

Over the past few years we have built an apparatus to demonstrate the entanglement of neutral Rb atoms at optically resolvable distances using the strong interactions between Rydberg atoms. Here we review the basic physics involved in this…

Quantum Physics · Physics 2025-11-18 Thad G. Walker , Mark Saffman

The spatial evolution of the Rydberg blockade is studied taking into account Stark-split energy levels across several manifolds. We find that the unexpected restoration of a blockaded Rydberg excitation at small interatomic distances, e.g.,…

Atomic Physics · Physics 2017-05-09 Yurii V. Dumin , Jan M. Rost

Ultracold polar molecules possess long-range, anisotropic, and tunable dipolar interactions, providing the opportunities to probe quantum phenomena inaccessible with existing cold gas platforms. However, experimental progress has been…

Experimental control over the strength and angular dependence of interactions between atoms is a key capability for advancing quantum technologies. Here, we use microwave dressing to manipulate and enhance Rydberg-Rydberg interactions in an…

When ground state atoms are excited to a Rydberg state, van der Waals interactions among them can lead to a strong suppression of the excitation. Despite the strong interactions the evolution can still be reversed by a simple phase shift in…

Quantum Physics · Physics 2011-11-10 Ulrich Raitzsch , Vera Bendkowsky , Rolf Heidemann , Björn Butscher , Robert Löw , Tilman Pfau

We discuss techniques to engineer effective long-range interactions between polar molecules using external static electric and microwave fields. We consider a setup where molecules are trapped in a two-dimensional pancake geometry by a…

Quantum Physics · Physics 2009-11-13 A. Micheli , G. Pupillo , H. P. Büchler , P. Zoller

We present a novel binding mechanism where a neutral Rydberg atom and an atomic ion form a molecular bound state at large internuclear distance. The binding mechanism is based on Stark shifts and level crossings which are induced in the…

Atomic Physics · Physics 2021-12-28 Markus Deiß , Shinsuke Haze , Johannes Hecker Denschlag

Long-range metastable molecules consisting of two cesium atoms in high Rydberg states have been observed in an ultracold gas. A sequential three-photon two-color photoassociation scheme was employed to form these molecules in states which…

Atomic Physics · Physics 2016-11-17 Heiner Saßmannshausen , Johannes Deiglmayr

We investigate a possible mechanism for the autoionization of ultracold Rydberg gases, based on the resonant coupling of Rydberg pair states to the ionization continuum. Unlike an atomic collision where the wave functions begin to overlap,…

Atomic Physics · Physics 2015-05-13 T. Amthor , J. Denskat , C. Giese , N. N. Bezuglov , A. Ekers , L. Cederbaum , M. Weidemüller

We present a new mechanism contributing to the detection of photoassociated long-range Rydberg molecules via pulsed-field ionization: ionic products, created by the decay of a long-range Rydberg molecule, modify the excitation spectrum of…

Atomic Physics · Physics 2023-01-26 Michael Peper , Martin Trautmann , Johannes Deiglmayr

A Rydberg and a ground-state atom can form ultralong range diatomic molecules provided the interaction between the ground-state atom and the Rydberg electron is attractive [C. H. Greene, et al., Phys. Rev. Lett. 85, 2458 (2000)]. A…

Atomic Physics · Physics 2008-07-15 Ivan C. H. Liu , Jovica Stanojevic , Jan M. Rost