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We study the effect of resonances associated with complex molecular interaction of Rydberg atoms on Rydberg blockade. We show that densely-spaced molecular potentials between doubly-excited atomic pairs become unavoidably resonant with the…

Atomic Physics · Physics 2016-10-05 Andrei Derevianko , Péter Kómár , Turker Topcu , Ronen M. Kroeze , Mikhail D. Lukin

We explore one-dimensional (1-D) samples of ultracold polar molecules with attractive dipole-dipole interactions and show the existence of a repulsive barrier due to a strong quadrupole interaction between molecules. This barrier can…

Chemical Physics · Physics 2015-06-05 Jason N. Byrd , John A. Montgomery , Robin Côté

It is shown that the two-step excitation scheme typically used to create an ultracold Rydberg gas can be described with an effective two-level rate equation, greatly reducing the complexity of the optical Bloch equations. This allows us to…

Atomic Physics · Physics 2015-06-26 Cenap Ates , Thomas Pohl , Thomas Pattard , Jan M. Rost

We perform a comprehensive investigation of the coupling between a Rydberg-dressed atomic gas and an ultra-cold plasma. Using simultaneous time-resolved measurements of both neutral atoms and ions, we show that plasma formation occurs via a…

Atomic Physics · Physics 2019-09-04 A. D. Bounds , N. C. Jackson , R. K. Hanley , E. M. Bridge , P. Huillery , M. P. A. Jones

The dipole blockade effect at laser excitation of mesoscopic ensembles of Rydberg atoms lies in the fact that the excitation of one atom to a Rydberg state blocks the excitation of other atoms due to the shift in the collective energy…

Atomic Physics · Physics 2020-04-22 E. A. Yakshina , D. B. Tretyakov , V. M. Entin , I. I. Beterov , I. I. Ryabtsev

Two ultracold atom clouds, each separately in a dipole-blockade regime, realize a source of entangled atom pairs that can be ejected on demand. Entanglement generation and ejection is due to resonant dipole-dipole interactions, while…

Atomic Physics · Physics 2015-06-17 S. Wüster , S. Möbius , M. Genkin , A. Eisfeld , J. M. Rost

We predict that ultralong-range Rydberg bi-molecules form in collisions between polar molecules in cold and ultracold settings. The collision of $\Lambda$-doublet nitric oxide (NO) with long-lived Rydberg NO($nf$, $ng$) molecules forms…

Atomic Physics · Physics 2021-02-03 Rosario Gonzalez-Ferez , Janine Shertzer , H. R. Sadeghpour

We calculate pair potential curves for interacting Rydberg atoms in a constant electric field and use them to determine the effective $C_3$ dipole-dipole and $C_6$ van der Waals coefficients. We compare the $C_3$ and $C_6$ with experiments…

Rydberg molecule, formed by one or more Rydberg atoms, exhibits remarkable properties, including an exceptionally large spatial extent, rich rovibrational level structures, permanent electric dipole moments, and a pronounced sensitivity to…

Atomic Physics · Physics 2026-03-11 Jingxu Bai , Yuechun Jiao , Xiao-Qiang Shao , Weibin Li , Jianming Zhao

Rydberg blockade sphere persists an intriguing picture by which a number of collective many-body effects caused by the strong Rydberg-Rydberg interactions can be clearly understood and profoundly investigated. In the present work, we…

Atomic Physics · Physics 2015-06-17 Jing Qian , Xing-Dong Zhao , Lu Zhou , Weiping Zhang

In the laser excitation of ultracold atoms to Rydberg states, we observe a dramatic suppression caused by van der Waals interactions. This behavior is interpreted as a local excitation blockade: Rydberg atoms strongly inhibit excitation of…

Atomic Physics · Physics 2009-11-10 D. Tong , S. M. Farooqi , J. Stanojevic , S. Krishnan , Y. P. Zhang , R. Côté , E. E. Eyler , P. L. Gould

Recently, several femtosecond laser techniques have been developed that are capable of bringing gas molecules to extremely fast rotation in a very short time, while keeping their translational motion intact and relatively slow. We…

Chemical Physics · Physics 2015-03-11 Yuri Khodorkovsky , Uri Steinitz , Jean-Michel Hartmann , Ilya Sh. Averbukh

We propose an experimentally realizable scheme to produce triatomic ultralong-range Rydberg molecules (TURM), formed in ultracold KRb traps. A near resonant coupling of the non-zero quantum defect Rydberg levels with the KRb molecule in N=0…

We investigate a long-range interaction between $64D_{5/2}$ Rydberg-atom pairs and antiblockade effect employing a two-color excitation scheme. The first color (pulse A) is set to resonantly excite the Rydberg transition and prepare a few…

Atomic Physics · Physics 2020-02-25 Suying Bai , Xuedong Tian , Xiaoxuan Han , Yuechun Jiao , Jinhui Wu , Jianming Zhao , Suotang Jia

Sufficiently high densities in Bose-Einstein condensates provide favorable conditions for the production of ultralong-range polyatomic molecules consisting of one Rydberg atom and a number of neutral ground state atoms. The chemical binding…

Atomic Physics · Physics 2017-05-10 Matthew T Eiles , Jesus Perez-Rios , F Robicheaux , Chris H Greene

The dipole blockade between Rydberg atoms has been proposed as a basic tool in quantum information processing with neutral atoms. Here we demonstrate experimentally the Rydberg blockade of two individual atoms separated by 4 $\mu$m.…

Quantum Physics · Physics 2010-06-09 A. Gaëtan , Y. Miroshnychenko , T. Wilk , A. Chotia , M. Viteau , D. Comparat , P. Pillet , A. Browaeys , P. Grangier

We consider ultralong-range polyatomic Rydberg molecules formed by combining a Rydberg cesium atom and a ground-state RbCs molecule. We explore the regime where the charge-dipole interaction due to the Rydberg electron with the diatomic…

Rydberg states of atoms are of great current interest for quantum manipulation of mesoscopic samples of atoms. Long-range Rydberg-Rydberg interactions can inhibit multiple excitations of atoms under the appropriate conditions. These…

Atomic Physics · Physics 2009-11-10 Thad G. Walker , Mark Saffman

The laser-excitation of Rydberg atoms in ultracold gases is often described assuming that the atomic motion is frozen during the excitation time. We show that this frozen gas approximation can break down for atoms that are held in optical…

Atomic Physics · Physics 2013-05-23 W. Li , C. Ates , I. Lesanovsky

The anisotropic Dicke model reveals the important role that counter-rotating wave terms play in the coupling between light and two level atoms. It is intriguing to generate the model to the strongly correlated many body case, where the…

Quantum Physics · Physics 2025-03-19 Bao-Yun Dong , Yanhua Zhou , Wei Wang , Tao Wang