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We report 7Li-NMR studies on LiInCr4O8 and LiGaCr4O8, in which Cr3+ ions with spin 3/2 form a breathing pyrochlore lattice, a network of tetrahedra with alternating sizes. In LiInCr4O8 with large alternation, the nuclear relaxation rate…

Strongly Correlated Electrons · Physics 2015-06-23 Yu Tanaka , Makoto Yoshida , Masashi Takigawa , Yoshihiko Okamoto , Zenji Hiroi

By means of nuclear spin-lattice relaxation rate 1/T1, we follow the spin dynamics as a function of the applied magnetic field in two gapped one-dimensional quantum antiferromagnets: the anisotropic spin-chain system NiCl2-4SC(NH2)2 and the…

We present an analytical model of orbital ordering in vanadium spinel MnV2O4. The model is based on recent first-principles calculation indicating a strong trigonal distortion at the vanadium sites of this compound [Phys. Rev. Lett. 102,…

Strongly Correlated Electrons · Physics 2010-07-13 Gia-Wei Chern , Natalia Perkins , Zhihao Hao

We report on the properties of SrTb2O4, a frustrated zigzag ladder antiferromagnet, studied by single crystal neutron diffraction (with polarised neutrons in zero field and unpolarised neutrons in an applied magnetic field), as well as by…

We report a neutron diffraction study of the multiferroic mechanism in (ND4)2FeCl5D2O, a molecular compound that exhibits magnetically induced ferroelectricity. This material exhibits two successive magnetic transitions on cooling: a…

We report a comprehensive investigation of the structural and magnetic properties of Na$_5$Yb(MoO$_4$)$_4$, a member of the stretched diamond magnetic lattice family. Neutron powder diffraction at 3.3~K confirms that the compound…

We re-investigate the magnetically frustrated, {\it diamond-lattice-antiferromagnet} spinels FeAl$_2$O$_4$ and MnAl$_2$O$_4$ using magnetization measurements and diffuse scattering of polarized neutrons. In FeAl$_2$O$_4$, macroscopic…

Disordered Systems and Neural Networks · Physics 2015-06-19 Harikrishnan S. Nair , Zhendong Fu , Jörg Voigt , Yixi Su , Th. Brückel

The phase diagram of the quasi-one-dimensional magnet NaCuMoO$_4$(OH) is established through single-crystal NMR and heat-capacity measurements. The $^{23}$Na and $^1$H NMR experiments indicate a spiral and a collinear spin-density-wave…

Strongly Correlated Electrons · Physics 2017-11-27 Kazuhiro Nawa , Makoto Yoshida , Masashi Takigawa , Yoshihiko Okamoto , Zenji Hiroi

We report a resonant inelastic X-ray scattering study on a single crystal of a non-stoichiometric pyrochlore iridate Tb$_{2+x}$Ir$_{2-x}$O$_{7-y}$ ($x \simeq 0.25$) that magnetically orders at $T_{\rm{N}}\simeq 50$ K. We find that the…

Strongly Correlated Electrons · Physics 2024-09-18 Q. Faure , A. Toschi , J. R. Soh , E. Lhotel , B. Detlefs , D. Prabhakaran , D. F. McMorrow , C. J. Sahle

Geometrical frustration is a central challenge in contemporary condensed matter physics, a crucible favourable to the emergence of novel physics. The pyrochlore magnets, with rare earth magnetic moments localized at the vertices of…

Strongly Correlated Electrons · Physics 2015-05-30 Sylvain Petit , Pierre Bonville , Isabelle Mirebeau , Hannu Mutka , Julien Robert

We report positive muon spin relaxation measurements on the triangular lattice magnetic system FeGa2S4. A magnetic transition not previously detected by specific heat and magnetic susceptibility measurements is found in zero field at T^*…

Strongly Correlated Electrons · Physics 2012-04-25 P. Dalmas de Reotier , A. Yaouanc , D. E. MacLaughlin , Songrui Zhao , T. Higo , S. Nakatsuji , Y. Nambu , C. Marin , G. Lapertot , A. Amato , C. Baines

Continuous spin excitations are widely recognized as one of the hallmarks of novel spin states in quantum magnets, such as quantum spin liquids (QSLs). Here, we report the observation of such kind of excitations in K2Ni2(SO4)3, which…

Na4Ir3O8 is a unique case of a hyperkagome 3D corner sharing triangular lattice which can be decorated with quantum spins. It has spurred a lot of theoretical interest as a spin liquid candidate. We present a comprehensive set of NMR data…

Strongly Correlated Electrons · Physics 2015-07-29 A. C. Shockley , F. Bert , J-C Orain , Y. Okamoto , P. Mendels

A novel metallic and magnetic transition metal oxide Ag2NiO2 is studied by means of resistivity, magnetic susceptibility, specific heat and X-ray diffraction. The crystal structure is characterized by alternating stacking of a Ni3+O2 layer…

Strongly Correlated Electrons · Physics 2009-11-11 H. Yoshida , Y. Muraoka , T. Soergel , M. Jansen , Z. Hiroi

We investigate the structural and magnetic properties of BaNi$_3$(AsO$_4$)$_2$(OH)$_2$, focusing on its spin-1 kagome lattice and the intricate coexistence of ferromagnetic and antiferromagnetic interactions. Powder x-ray diffraction…

Strongly Correlated Electrons · Physics 2025-08-14 Yuya Haraguchi , Jun-ichi Yamaura , Akira Matsuo , Koichi Kindo , Hiroko Aruga Katori

We perform a general study of spin ordering on the pyrochlore lattice with a 3:1 proportionality of two spin polarizations. Equivalently, this describes valence bond solid conformations of a quantum dimer model on the diamond lattice. We…

Strongly Correlated Electrons · Physics 2007-05-23 Doron L. Bergman , Gregory A. Fiete , Leon Balents

The stretched diamond lattice material LiYbO2 has recently been reported to exhibit two magnetic transitions ($T_{N1} = 1.1 K$, $T_{N2} = 0.45 K$) via specific heat, magnetization, and neutron scattering measurements [Bordelon et al., Phys.…

Strongly Correlated Electrons · Physics 2022-10-19 Eric M. Kenney , Mitchell M. Bordelon , Chennan Wang , Hubertus Luetkens , Stephen D. Wilson , Michael J. Graf

The ferrimagnetic spinels MnB2O4 (B = Mn,V) exhibit a similar series of closely spaced magnetic and structural phase transitions at low temperatures, reflecting both magnetic frustration and a strong coupling between the spin and lattice…

Strongly Correlated Electrons · Physics 2015-01-28 S. L. Gleason , T. Byrum , Y. Gim , A. Thaler , P. Abbamonte , G. J. MacDougall , L. W. Martin , H. D. Zhou , S. L. Cooper

At room temperature, the normal oxide spinels NiCr_2O_4 and CuCr_2O_4 are tetragonally distorted and crystallize in the I4_1/amd space group due to cooperative Jahn-Teller ordering driven by the orbital degeneracy of tetrahedral Ni$^{2+}$…

Materials Science · Physics 2012-09-11 Matthew R. Suchomel , Daniel P. Shoemaker , Lynn Ribaud , Moureen C. Kemei , Ram Seshadri

Tetragonal distorted spinel of CuMn2-xTixO4 (x = 0, 0.25 and 0.50) was prepared by solid state reaction method followed by neutron diffraction, FTIR spectroscopy, dielectric spectroscopy and magnetization measurements. The neutron…

Materials Science · Physics 2020-12-01 P. Patra , I. Naik , S. D. Kaushik , S. Mohanta
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