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We report measurements of 19F nuclear spin-lattice relaxation 1/T1 as a function of temperature and external magnetic field in LiY0.998Ho0.002F4 single crystal, a single-ion magnet exhibiting interesting quantum effects. The 19F 1/T1 is…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 M. J. Graf , A. Lascialfari , F. Borsa , A. M. Tkachuk , B. Barbara

The ground state of a molecular diamond-lattice compound (ET)Ag$_4$(CN)$_5$ is investigated by the magnetization and nuclear magnetic resonance spectroscopy. We found that the system exhibits antiferromagnetic long-range ordering with weak…

We investigate magnetic properties of the $s$ = 1/2 compound K$_{2}$Cu$_{3}$(MoO$_{4}$)$_{4}$ by combining magnetic susceptibility, magnetization, specific heat, and electron spin resonance (ESR) with density functional calculations. Its…

NiGa$_2$S$_4$ is a triangular lattice S=1 system with strong two-dimensionality of the lattice, actively discussed as a candidate to host spin-nematic order brought about by strong quadrupole coupling. Using Raman scattering spectroscopy we…

GeCo$_2$O$_4$ is a unique system in the family of cobalt spinels ACo$_2$O$_4$ (A= Sn, Ti, Ru, Mn, Al, Zn, Fe, etc.) in which magnetic Co ions stabilize on the pyrochlore lattice exhibiting a large degree of orbital frustration. Due to the…

We derive a spin-orbital Hamiltonian for a triangular lattice of e_g orbital degenerate (Ni^{3+}) transition metal ions interacting via 90 degree superexchange involving (O^{2-}) anions, taking into account the on-site Coulomb interactions…

Strongly Correlated Electrons · Physics 2009-11-11 Albert J. W. Reitsma , Louis F. Feiner , Andrzej M. Oles'

Motivated by experiments on the double perovskites La2ZnIrO6 and La2MgIrO6, we study the magnetism of spin-orbit coupled j=1/2 iridium moments on the three-dimensional, geometrically frustrated, face-centered cubic lattice. The…

Strongly Correlated Electrons · Physics 2015-09-30 A. M. Cook , S. Matern , C. Hickey , A. A. Aczel , A. Paramekanti

In this study, we have performed the magnetocaloric effect and the specific heat measurements of chromium spinel oxide HgCr$_2$O$_4$, wherein the magnetic Cr$^{3+}$ ions form a highly frustrated pyrochlore lattice with significant…

Strongly Correlated Electrons · Physics 2022-05-25 Shojiro Kimura , Shusaku Imajo , Masaki Gen , Tsutomu Momoi , Masayuki Hagiwara , Hiroaki Ueda , Yoshimitsu Kohama

We have investigated polycrystalline samples of the zigzag chain system BaTb$_2$O$_4$ with a combination of magnetic susceptibility, heat capacity, neutron powder diffraction, and muon spin relaxation measurements. Despite the onset of…

Strongly Correlated Electrons · Physics 2015-10-27 A. A. Aczel , L. Li , V. O. Garlea , J. -Q. Yan , F. Weickert , V. S. Vapf , R. Movshovich , M. Jaime , P. J. Baker , V. Keppens , D. Mandrus

The structure and magnetic properties of rare-earth ions Tm$^{3+}$ kagom\'{e} lattice Tm$_3$Sb$_3$Mg$_2$O$_{14}$ are studied by X-ray diffraction, magnetic susceptibility and muon spin relaxation ($\mu$SR) experiments. The existence of a…

Strongly Correlated Electrons · Physics 2023-10-02 Yanxing Yang , Kaiwen Chen , Zhaofeng Ding , Adrian D. Hillier , Lei Shu

We discuss the ground state properties of a spin 1/2 magnetic ion with threefold $t_{2g}$ orbital degeneracy on a highly frustrated pyrochlore lattice, like Ti$^{3+}$ ion in B-spinel MgTi$_2$O$_4$. We formulate an effective spin-orbital…

Strongly Correlated Electrons · Physics 2007-05-23 S. Di Matteo , G. Jackeli , N. B. Perkins

In frustrated spinel antiferromagnets, dilution with non-magnetic ions can be a powerful strategy for probing unconventional spin states or uncovering interesting phenomena. Here, we present X-ray, neutron scattering and thermodynamic…

Strongly Correlated Electrons · Physics 2018-06-20 A. V. Zakrzewski , S. Gangopadhyay , A. A. Aczel , S. Calder , T. J. Williams , G. J. MacDougall

We present a theoretical analysis of the electron spin decoherence in single Nitrogen-Vacancy defects in ultra-pure diamond. The electron spin decoherence is due to the interactions with Carbon-13 nuclear spins in the diamond lattice. Our…

Other Condensed Matter · Physics 2009-11-13 J. R. Maze , J. M. Taylor , M. D. Lukin

We report measurements performed on a polycrystalline sample of the pyrochlore compound Nd2Sn2O7. It undergoes a second order magnetic phase transition at Tc ~ 0.91 K to a noncoplanar all-in-all-out magnetic structure of the Nd3+ magnetic…

Strongly Correlated Electrons · Physics 2015-11-04 A. Bertin , P. Dalmas de Reotier , B. Fak , C. Marin , A. Yaouanc , A. Forget , D. Sheptyakov , B. Frick , C. Ritter , A. Amato , C. Baines , P. J. C. King

We report magnetization, electron spin resonance (ESR), and muon spin relaxation ($\mu $SR) measurements on single crystals of the $S=1/2$ (Cu$% ^{+2}$) kagom\'{e} compound Cu(1,3-benzendicarboxylate). The $\mu $SR is carried to…

Strongly Correlated Electrons · Physics 2015-06-18 Oren Ofer , Lital Marcipar , V. Ravi Chandra , Snir Gazit , Daniel Podolsky , Daniel P. Arovas , Amit Keren

Neutron scattering studies on a single crystal of the highly-correlated electron system, La1-xSrxMnO3 with x~0.3, have been carried out elucidating both the spin and lattice dynamics of this metallic ferromagnet. We report a large measured…

Condensed Matter · Physics 2009-10-28 Michael C. Martin , G. Shirane , Y. Endoh , K. Hirota , Y. Moritomo , Y. Tokura

Cs2CoBr4 is a triangular-lattice antiferromagnet which can be viewed as weakly interacting spin chains due to spatially anisotropic frustrating exchange couplings. The spin-orbit interaction in Co(2+) spin-3/2 ions leads to a strong…

Strongly Correlated Electrons · Physics 2023-09-06 T. A. Soldatov , A. I. Smirnov , A. V. Syromyatnikov

The synergistic interplay between spin correlations, spin-orbit coupling, and competing exchange interactions provides a promising route to realize exotic quantum states with nontrivial excitations in rare-earth based frustrated magnets.…

Strongly Correlated Electrons · Physics 2026-05-25 J. Khatua , D. Tay , T. Shiroka , M. Pregelj , K. Kargeti , S. K. Panda , G. B. G. Stenning , P. Manuel , M. D. Le , D. T. Adroja , P. Khuntia

Neutron inelastic scattering has been used to probe the spin dynamics of the quantum (S=1/2) ferromagnet on the pyrochlore lattice Lu2V2O7. Well-defined spin waves are observed at all energies and wavevectors, allowing us to determine the…

Strongly Correlated Electrons · Physics 2015-06-19 M. Mena , R. S. Perry , T. G. Perring , M. D. Le , S. Guerrero , M. Storni , D. T. Adroja , Ch. Ruegg , D. F. McMorrow

The crystal and magnetic structures and underlying magnetic interactions of Bi4Fe5O13F, a model system for studying the physics of the Cairo pentagonal spin lattice, are investigated by transmission electron microscopy, low-temperature…