English

Spin dynamics and possible topological magnons in non-stoichiometric pyrochlore iridate Tb$_2$Ir$_2$O$_7$ studied by RIXS

Strongly Correlated Electrons 2024-09-18 v2

Abstract

We report a resonant inelastic X-ray scattering study on a single crystal of a non-stoichiometric pyrochlore iridate Tb2+x_{2+x}Ir2x_{2-x}O7y_{7-y} (x0.25x \simeq 0.25) that magnetically orders at TN50T_{\rm{N}}\simeq 50 K. We find that the strength of the spin-orbit coupling and the trigonal distortion of the IrO6_6 octahedra are comparable with the ones obtained in other pyrochlore iridates. We observe a propagating gapped magnon mode at low energy, and model it using a Hamiltonian consisting of a Heisenberg exchange [J=16.2(9)J = 16.2(9) meV] and Dzyaloshinskii-Moriya interactions [D=5.2(3)D = 5.2(3) meV], which shows the robustness of interactions despite Tb-stuffing at the Ir-site. Strikingly, the ratio D/J=0.32(3)D/J = 0.32(3) supports possible non-trivial topological magnon band crossing. This material may thus host coexisting fermionic and bosonic topology, with potential for manipulating electronic and magnonic topological bands thanks to the dfd-f interaction.

Keywords

Cite

@article{arxiv.2404.03829,
  title  = {Spin dynamics and possible topological magnons in non-stoichiometric pyrochlore iridate Tb$_2$Ir$_2$O$_7$ studied by RIXS},
  author = {Q. Faure and A. Toschi and J. R. Soh and E. Lhotel and B. Detlefs and D. Prabhakaran and D. F. McMorrow and C. J. Sahle},
  journal= {arXiv preprint arXiv:2404.03829},
  year   = {2024}
}

Comments

manuscript: 7 pages, 4 figures; Supplemental Material: 6 pages, 7 figures, 1 table. Accepted at PRB Letters (2024)