We report a resonant inelastic X-ray scattering study on a single crystal of a non-stoichiometric pyrochlore iridate Tb2+xIr2−xO7−y (x≃0.25) that magnetically orders at TN≃50 K. We find that the strength of the spin-orbit coupling and the trigonal distortion of the IrO6 octahedra are comparable with the ones obtained in other pyrochlore iridates. We observe a propagating gapped magnon mode at low energy, and model it using a Hamiltonian consisting of a Heisenberg exchange [J=16.2(9) meV] and Dzyaloshinskii-Moriya interactions [D=5.2(3) meV], which shows the robustness of interactions despite Tb-stuffing at the Ir-site. Strikingly, the ratio D/J=0.32(3) supports possible non-trivial topological magnon band crossing. This material may thus host coexisting fermionic and bosonic topology, with potential for manipulating electronic and magnonic topological bands thanks to the d−f interaction.
@article{arxiv.2404.03829,
title = {Spin dynamics and possible topological magnons in non-stoichiometric pyrochlore iridate Tb$_2$Ir$_2$O$_7$ studied by RIXS},
author = {Q. Faure and A. Toschi and J. R. Soh and E. Lhotel and B. Detlefs and D. Prabhakaran and D. F. McMorrow and C. J. Sahle},
journal= {arXiv preprint arXiv:2404.03829},
year = {2024}
}